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Register a new userExperimental test of exchange fluctuation relations in an open quantum system
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Elucidating the energy transfer between a quantum system and a reservoir is a central issue in quantum non-equilibrium thermodynamics, which could provide novel tools to engineer quantum-enhanced heat engines. The lack of information on the reservoir inherently limits the practical insight that can be gained on the exchange process of open quantum systems. Here, we investigate the energy transfer for an open quantum system in the framework of quantum fluctuation relations. As a novel toolbox, we employ a nitrogen-vacancy center spin qubit in diamond, subject to repeated quantum projective measurements and a tunable dissipation channel. In the presence of energy fluctuations originated by dissipation and quantum projective measurements, the experimental results, supplemented by numerical simulations, show the validity of the energy exchange fluctuation relation, where the energy scale factor encodes missing reservoir information in the system out-of-equilibrium steady state properties. This result is complemented by a theoretical argument showing that, also for an open three-level quantum system, the existence of an out-of-equilibrium steady state dictates a unique time-independent value of the energy scale factor for which the fluctuation relation is verified. Our findings pave the way to the investigation of energy exchange mechanisms in arbitrary open quantum systems.
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The experimental verification of quantum fluctuation relations for driven open quantum system is currently a challenge, due to the conceptual and operative difficulty of distinguishing work and heat. The Nitrogen-Vacancy center in diamond has been recently proposed as a controlled test bed to study fluctuation relations in the presence of an engineered dissipative channel, in absence of work [Hernandez-Gomez et al., Phys. Rev. Research 2, 023327 (2020)]. Here, we extend those studies to exploring the validity of quantum fluctuation relations in a driven-dissipative scenario, where the spin exchanges energy both with its surroundings because of a thermal gradient, and with an external work source. We experimentally prove the validity of the quantum fluctuation relations in the presence of cyclic driving in two cases, when the spin exchanges energy with an effective infinite-temperature reservoir, and when the total work vanishes at stroboscopic times -- although the power delivered to the NV center is non-null. Our results represent the first experimental study of quantum fluctuation relation in driven open quantum systems.
Research on the out-of-equilibrium dynamics of quantum systems has so far produced important statements on the thermodynamics of small systems undergoing quantum mechanical evolutions. Key examples are provided by the Crooks and Jarzynski relations: taking into account fluctuations in non-equilibrium dynamics, such relations connect equilibrium properties of thermodynamical relevance with explicit non-equilibrium features. Although the experimental verification of such fundamental relations in the classical domain has encountered some success, their quantum mechanical version requires the assessment of the statistics of work performed by or onto an evolving quantum system, a step that has so far encountered considerable difficulties in its implementation due to the practical difficulty to perform reliable projective measurements of instantaneous energy states. In this paper, by exploiting a radical change in the characterization of the work distribution at the quantum level, we report the first experimental verification of the quantum Jarzynski identity and the Tasaki-Crooks relation following a quantum process implemented in a Nuclear Magnetic Resonance (NMR) system. Our experimental approach has enabled the full characterisation of the out-of-equilibrium dynamics of a quantum spin in a statistically significant way, thus embodying a key step towards the grounding of quantum-systems thermodynamics.
As the dimensions of physical systems approach the nanoscale, the laws of thermodynamics must be reconsidered due to the increased importance of fluctuations and quantum effects. While the statistical mechanics of small classical systems is relatively well understood, the quantum case still poses challenges. Here we set up a formalism that allows to calculate the full probability distribution of energy exchanges between a periodically driven quantum system and a thermalized heat reservoir. The formalism combines Floquet theory with a generalized master equation approach. For a driven two-level system and in the long-time limit, we obtain a universal expression for the distribution, providing clear physical insight into the exchanged energy quanta. We illustrate our approach in two analytically solvable cases and discuss the differences in the corresponding distributions. Our predictions could be directly tested in a variety of systems, including optical cavities and solid-state devices.
We investigate the link between information and thermodynamics embodied by Landauers principle in the open dynamics of a multipartite quantum system. Such irreversible dynamics is described in terms of a collisional model with a finite temperature reservoir. We demonstrate that Landauers principle holds, for such a configuration, in a form that involves the flow of heat dissipated into the environment and the rate of change of the entropy of the system. Quite remarkably, such a principle for {it heat and entropy power} can be explicitly linked to the rate of creation of correlations among the elements of the multipartite system and, in turn, the non-Markovian nature of their reduced evolution. Such features are illustrated in two exemplary cases.
Maxwells demon explores the role of information in physical processes. Employing information about microscopic degrees of freedom, this intelligent observer is capable of compensating entropy production (or extracting work), apparently challenging the second law of thermodynamics. In a modern standpoint, it is regarded as a feedback control mechanism and the limits of thermodynamics are recast incorporating information-to-energy conversion. We derive a trade-off relation between information-theoretic quantities empowering the design of an efficient Maxwells demon in a quantum system. The demon is experimentally implemented as a spin-1/2 quantum memory that acquires information, and employs it to control the dynamics of another spin-1/2 system, through a natural interaction. Noise and imperfections in this protocol are investigated by the assessment of its effectiveness. This realization provides experimental evidence that the irreversibility on a non-equilibrium dynamics can be mitigated by assessing microscopic information and applying a feed-forward strategy at the quantum scale.
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