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Register a new userThermal chiral anomaly in the magnetic-field induced ideal Weyl phase of Bi1-xSbx topological insulators
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The chiral anomaly is the predicted break down of chiral symmetry in a Weyl semimetal with monopoles of opposite chirality when an electric field parallel to a magnetic field is applied. It occurs because of charge pumping from a positive chirality to a negative chirality monopole. Experimental observation of this fundamental effect has been plagued by concerns about the pathways of the current. Here, we unambiguously demonstrate the thermal analog of the chiral anomaly in topological insulator bismuth-antimony alloys driven into an ideal Weyl semimetal state by a Zeeman field, with the chemical potential pinned at the Weyl points, and in which the Fermi surface has no trivial pockets. The experimental signature is a large enhancement of the thermal conductivity in an applied magnetic field parallel to the thermal gradient that follows the Wiedemann-Franz law above 60 K. Absence of current flow avoids extrinsic effects that plague electrical measurements.
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The discovery of Weyl semimetals (WSMs) has fueled tremendous interest in condensed matter physics. WSMs require breaking of either inversion symmetry (IS) or time-reversal symmetry (TRS); they can be categorized into type-I and type-II WSMs, characterized by un-tilted and strongly tilted Weyl cones respectively. Type-I WSMs with breaking of IS or TRS and type-II WSMs with IS breaking have been realized experimentally, but TRS-breaking type-II WSM still remains elusive. In this article, we report an ideal TRS-breaking type-II WSM with only one pair of Weyl nodes observed in the antiferromagnetic topological insulator Mn(Bi1-xSbx)2Te4 under magnetic fields. This state is manifested by a large intrinsic anomalous Hall effect, a non-trivial $mathrm{{pi}}$ Berry phase of the cyclotron orbit and a large positive magnetoresistance in the ferromagnetic phase at an optimal sample composition. Our results establish a promising platform for exploring the physics underlying the long-sought, ideal TRS breaking type-II WSM.
The electron-phonon interaction (EPI) is instrumental in a wide variety of phenomena in solid-state physics, such as electrical resistivity in metals, carrier mobility, optical transition and polaron effects in semiconductors, lifetime of hot carriers, transition temperature in BCS superconductors, and even spin relaxation in diamond nitrogen-vacancy centers for quantum information processing. However, due to the weak EPI strength, most phenomena have focused on electronic properties rather than on phonon properties. One prominent exception is the Kohn anomaly, where phonon softening can emerge when the phonon wavevector nests the Fermi surface of metals. Here we report a new class of Kohn anomaly in a topological Weyl semimetal (WSM), predicted by field-theoretical calculations, and experimentally observed through inelastic x-ray and neutron scattering on WSM tantalum phosphide (TaP). Compared to the conventional Kohn anomaly, the Fermi surface in a WSM exhibits multiple topological singularities of Weyl nodes, leading to a distinct nesting condition with chiral selection, a power-law divergence, and non-negligible dynamical effects. Our work brings the concept of Kohn anomaly into WSMs and sheds light on elucidating the EPI mechanism in emergent topological materials.
The Seebeck coefficients, electrical resistivities, total thermal conductivities, and magnetization are reported for temperatures between 5 and 350 K for n-type Bi0.88Sb0.12 nano-composite alloys made by Ho-doping at the 0, 1 and 3% atomic levels. The alloys were prepared using a dc hot-pressing method, and are shown to be single phase for both Ho contents with grain sizes on the average of 900 nm. We find the parent compound has a maximum of ZT = 0.28 at 231 K, while doping 1% Ho increases the maximum ZT to 0.31 at 221 K and the 3% doped sample suppresses the maximum ZT = 0.24 at a temperature of 260 K.
After the classification of topological states of matter has been clarified for non-interacting electron systems, the theoretical connection between gapless boundary modes and nontrivial bulk topological structures, and their evolutions as a function of dimensions are now well understood. However, such dimensional hierarchy has not been well established experimentally although some indirect evidences were reported, for example, such as the half-quantized Hall conductance via quantum Hall effect and extrapolation in the quantum-oscillation measurement. In this paper, we report the appearance of the possible chiral edge mode from the surface state of topological insulators under magnetic fields, confirming the dimensional hierarchy in three dimensional topological insulators. Applying laser pulses to the surface state of Bi1-xSbx, we find that the sign of voltage relaxation in one edge becomes opposite to that in the other edge only when magnetic fields are applied to the topological insulating phase. We show that this sign difference originates from the chirality of edge states, based on coupled time-dependent Poisson and Boltzmann equations.
Chiral anomaly or Adler-Bell-Jackiw anomaly in Weyl semimetals (WSMs) has a significant impact on the electron transport behaviors, leading to remarkable longitudinal or planar electrical and thermoelectric transport phenomena in the presence of electromagnetic gauge fields. These phenomena are consequences of the imbalanced chiral charge and energy induced by chiral anomaly in the presence of parallel electric ($mathbf{E}$) and magnetic ($mathbf{B}$) fields ($mathbf{E cdot B } eq 0$) or $(mathbf{B cdot abla }T eq 0)$ ($mathbf{ abla}T$ is the thermal gradient). We here propose another two fascinating transport properties, namely, the nonlinear planar Nernst effect and nonlinear planar thermal Hall effect induced by chiral anomaly in the presence of $mathbf{B cdot abla}T eq 0$ in WSMs. Using the semiclassical Boltzmann transport theory, we derive the analytical expressions for the chiral anomaly induced nonlinear Nernst and thermal Hall transport coefficients and also evaluate the fundamental mathematical relations among them in the nonlinear regime. The formulas we find in this current work are consistent with that predicted for the nonlinear anomalous electrical and thermoelectric effects induced by Berry curvature dipole recently. Additionally, in contrast to the recent work, by utilizing the lattice Weyl Hamiltonian with intrinsic chiral chemical potential, we find that the chiral anomaly induced nonlinear planar effects can exist even for a pair of oppositely tilted or non-tilted Weyl cones in both time reversal and inversion broken WSMs. The chiral anomaly induced nonlinear planar effects predicted here along with the related parameter dependencies are hence possible to be realized in realistic WSMs in experiment.
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