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Chalcogenide-glass polarization-maintaining photonic crystal fiber for mid-infrared supercontinuum generation

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 Added by Thibaut Sylvestre
 Publication date 2019
  fields Physics
and research's language is English




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In this paper, we report the design and fabrication of a highly birefringent polarization-maintaining photonic crystal fiber (PM-PCF) made from chalcogenide glass, and its application to linearly-polarized supercontinuum (SC) generation in the mid-infrared region. The PM fiber was drawn using the casting method from As38Se62 glass which features a transmission window from 2 to 10 $mu m$ and a high nonlinear index of 1.13.10$^{-17}$m$^{2}$W$^{-1}$. It has a zero-dispersion wavelength around 4.5 $mu m$ and, at this wavelength, a large birefringence of 6.10$^{-4}$ and consequently strong polarization maintaining properties are expected. Using this fiber, we experimentally demonstrate supercontinuum generation spanning from 3.1-6.02 $mu m$ and 3.33-5.78 $mu m$ using femtosecond pumping at 4 $mu m$ and 4.53 $mu m$, respectively. We further investigate the supercontinuum bandwidth versus the input pump polarization angle and we show very good agreement with numerical simulations of the two-polarization model based on two coupled generalized nonlinear Schrodinger equations.



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We demonstrate the generation of a low-noise, octave-spanning mid-infrared supercontinuum from 1700 to 4800 nm by injecting femtosecond pulses into the normal dispersion regime of a multimode step-index chalcogenide fiber with 100 $mu$m core diameter. We conduct a systematic study of the intensity noise across the supercontinuum spectrum and show that the initial fluctuations of the pump laser are at most amplified by a factor of three. We also perform a comparison with the noise characteristics of an octave-spanning supercontinuum generated in the anomalous dispersion regime of a multimode fluoride fiber with similar core size and show that the all-normal dispersion supercontinuum in the multimode chalcogenide fiber has superior noise characteristics. Our results open up novel perspective for many practical applications such as long-distance remote sensing where high power and low noise are paramount.
Improved long-wavelength transmission and supercontinuum (SC) generation is demonstrated by anti-reflective (AR) nanoimprinting and tapering of chalcogenide photonic crystal fibers (PCF). Using a SC source input spanning from 1-4.2 {mu}m, the total transmission of a 15 {mu}m core diameter PCF was improved from ~53 % to ~74 % by nanoimprinting of AR structures on both input- and output facets of the fiber. Through a combined effect of reduced reflection and red-shifting of the spectrum to 5 {mu}m, the relative transmission of light >3.5 {mu}m in the same fiber was increased by 60.2 %. Further extension of the spectrum to 8 {mu}m was achieved using tapered fibers. The spectral broadening dynamics and output power was investigated using different taper parameters and pulse repetition rates.
We investigate supercontinuum generation in several suspended-core soft-glass photonic crystal fibers pumped by an optical parametric oscillator tunable around 1550 nm. The fibers were drawn from lead-bismuth-gallium-cadmium-oxide glass (PBG-81) with a wide transmission window from 0.5-2.7 micron and a high nonlinear refractive index up to 4.3.10^(-19) m^2/W. They have been specifically designed with a microscale suspended hexagonal core for efficient supercontinuum generation around 1550 nm. We experimentally demonstrate two supercontinuum spectra spanning from 1.07-2.31 micron and 0.89-2.46 micron by pumping two PCFs in both normal and anomalous dispersion regimes, respectively. We also numerically model the group velocity dispersion curves for these fibers from their scanning electron microscope images. Results are in good agreement with numerical simulations based on the generalized nonlinear Schrodinger equation including the pump frequency chirp.
We present numerical results of supercontinuum (SC) generation in the mid-IR spectral region, specifically addressing the molecular fingerprint window ranging from 2.5 to 25 um. By solving the Generalized Nonlinear Schrodinger Equation (GNLSE) in a chalcogenide waveguide, we demonstrate low-power SC generation beyond 10 um from a pump at 5 um. Further, we investigate the short-pulse and CW regimes, and show that a simple linear dispersion profile, applicable to a broad range of chalcogenide media, is sufficient to account for the broad SC generation, and yield rich pulse dynamics leading to the frequent occurrence of rogue wave events. Results are encouraging as they point to the feasibility of producing bright and coherent light, by means of single low-power tabletop laser pumping schemes, in a spectral region that finds applications in such diverse areas as molecular spectroscopy, metrology and tomography, among others, and that is not easily addressable with other light sources
Although supercontinuum sources are readily available for the visible and near infrared, and recently also for the mid-IR, many areas of biology, chemistry and physics would benefit greatly from the availability of compact, stable and spectrally bright deep ultraviolet (DUV) and vacuum ultraviolet (VUV) supercontinuum sources. Such sources have however not yet been developed. Here we report the generation of a bright supercontinuum, spanning more than three octaves from 124 nm to beyond 1200 nm, in hydrogen-filled kagome-style hollow-core photonic crystal fiber (kagome-PCF). Few-{mu}J, 30 fs pump pulses at wavelength 805 nm are launched into the fiber, where they undergo self-compression via the Raman-enhanced Kerr effect. Modeling indicates that before reaching a minimum sub-cycle pulse duration of ~1 fs, much less than one period of molecular vibration (8 fs), nonlinear reshaping of the pulse envelope, accentuated by self-steepening and shock formation, creates an ultrashort feature that causes impulsive excitation of long-lived coherent molecular vibrations. These phase-modulate a strong VUV dispersive wave (at 182 nm or 6.8 eV) on the trailing edge of the pulse, further broadening the spectrum into the VUV. The results also show for the first time that kagome-PCF guides well in the VUV.
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