No Arabic abstract
The nonlinear frequency conversion of low-temporal-coherent light holds a variety of applications and has attracted considerable interest. However, its physical mechanism remains relatively unexplored, and the conversion efficiency and bandwidth are extremely insufficient. Here, considering the instantaneous broadband characteristic, we establish a model of second harmonic generation (SHG) of low-temporal-coherent pulse, and reveal its differences from the coherent conditions. It is found that the second harmonic (SH) of low-temporal-coherent light is produced by not only the degenerate SH processes but also crossed sum-frequency processes. On the basis of this, we propose a method for realizing low-temporal-coherent SHG with high efficiency and broad bandwidth, and experimentally demonstrate a conversion efficiency up to 70% with a bandwidth of 3.1 THz (2.9 nm centered at 528 nm). To the best of our knowledge, this is the highest efficiency and broadest bandwidth of low-temporal-coherent SHG, and its efficiency is almost the same with that of the narrowband coherent condition. Furthermore, the spectral evolution characteristics of the broadband low-temporal-coherent pulse in SHG process are revealed in experiments, that the SH power spectral density (PSD) is proportional to the self-convolution of the fundamental wave PSD, which is greatly different from that of the coherent process. Our research opens a door for the study of the low-coherent nonlinear optical processes.
We demonstrate second harmonic generation of blue light on an integrated thin-film lithium niobate waveguide and observe a conversion efficiency of $eta_0= 33000%/text{W-cm}^2$, significantly exceeding previous demonstrations.
In this letter we experimentally demonstrate second harmonic conversion in the opaque region of a GaAs cavity with efficiencies of the order of 0.1% at 612nm, using 3ps pump pulses having peak intensities of order of 10MW/cm2. We show that the conversion efficiency of the inhomogeneous, phase-locked second harmonic component is a quadratic function of the cavity factor Q.
Semiconductor nanowires (NWs) are promising for realizing various on-chip nonlinear optical devices, due to their nanoscale lateral confinement and strong light-matter interaction. However, high-intensity pulsed pump lasers are typically needed to exploit their optical nonlinearity because light couples poorly with nanometric-size wires. Here, we demonstrate microwatts continuous-wave light pumped second harmonic generation (SHG) in AlGaAs NWs by integrating them with silicon planar photonic crystal cavities. Light-NW coupling is enhanced effectively by the extremely localized cavity mode at the subwavelength scale. Strong SHG is obtained even with a continuous-wave laser excitation with a pump power down to ~3 uW, and the cavity-enhancement factor is estimated around 150. Additionally, in the integrated device, the NWs SHG is more than two-order of magnitude stronger than third harmonic generations in the silicon slab, though the NW only couple s with less than 1% of the cavity mode. This significantly reduced power-requirement of NWs nonlinear frequency conversion would promote NW-based building blocks for nonlinear optics, specially in chip-integrated coherent light sources, entangled photon-pairs and signal processing devices.
A scheme for active second harmonics generation is suggested. The system comprises $N$ three-level atoms in ladder configuration, situated into resonant cavity. It is found that the system can lase in either superradiant or subradiant regime, depending on the number of atoms $N$. When N passes some critical value the transition from the super to subradiance occurs in a phase-transition-like manner. Stability study of the steady state supports this conclusion.
High-harmonic generation is one of the most fundamental processes in strong laser-field physics that has led to countless achievements in atomic physics and beyond. However, a rigorous quantum electrodynamical picture of the process has never been reported. Here, we prove rigorously and demonstrate experimentally that the quantum state of the driving laser field, as well as that of harmonics, is coherent. Projecting this state on its part corresponding to harmonic generation, it becomes a superposition of a state, amplitude-shifted due to the quantum nature of light, and the initial state of the laser. This superposition interpolates between a Schr{o}dinger kitten, and a genuine Schr{o}dinger cat state. This work opens new paths for ground-breaking investigations in strong laser-field physics and quantum technology. We dedicate the work to the memory of Roy J. Glauber, the inventor of coherent states.