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Visualizing the periodic modulation of Cooper pairing in a severely underdoped cuprate

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 Added by Yayu Wang
 Publication date 2019
  fields Physics
and research's language is English




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A major obstacle in understanding the mechanism of Cooper pairing in the cuprates is the existence of various intertwined orders associated with spin, charge, and Cooper pairs. Of particular importance is the ubiquitous charge order features that have been observed in a variety of cuprates, especially in the underdoped regime of the phase diagram. To explain the origin of the charge order and its implication to the superconducting phase, many theoretical models have been proposed, such as charge stripes, electronic nematicity, and Fermi surface instability. A highly appealing physical picture is the so-called pair density wave (PDW), a periodic modulation of Cooper paring in space, which may also induce a charge order. To elucidate the existence and nature of the PDW order, here we use scanning tunneling microscopy (STM) to investigate a severely underdoped Bi2Sr2CaCu2O8+{delta}, in which superconductivity just emerges on top of a pronounced checkerboard charge order. By analyzing the spatial distribution of the spectral features characteristic of superconductivity, we observe a periodic modulation of both the superconducting coherence peak and gap depth, demonstrating the existence of a density wave order of Cooper pairing. The PDW order has the same spatial periodicity as the charge order, and the amplitudes of the two orders exhibit clear positive correlation. These results shed important new lights on the origin of and interplay between the charge order and Cooper pairing modulation in the cuprates.



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The preformed-pairs theory of pseudogap physics in high-$T_C$ superconductors predicts a nonanalytic $T$-dependence for the $ab$-plane superfluid fraction, $rho_S$, at low temperatures in underdoped cuprates. We report high-precision measurements of $rho_S(T)$ on severely underdoped YBa$_2$Cu$_3$O$_{6+x}$ and Y$_{0.8}$Ca$_{0.2}$Ba$_2$Cu$_3$O$_{6+x}$ films. At low $T$, $rho_S$ looks more like $1 - T^2$ than $1 - T^{3/2}$, in disagreement with theory.
Recent angle resolved photoemission cite{yang-nature-08} and scanning tunneling microscopy cite{kohsaka-nature-08} measurements on underdoped cuprates have yielded new spectroscopic information on quasiparticles in the pseudogap phase. New features of the normal state such as particle-hole asymmetry, maxima in the energy dispersion and accompanying drops in the spectral weight of quasiparticles agree with the ansatz of Yang textit{et al.} for the single particle propagator in the pseudogap phase. The coherent quasiparticle dispersion and reduced asymmetry in the tunneling density of states in the superconducting state can also be described by this propagator.
176 - Louis Taillefer 2010
The origin of the exceptionally strong superconductivity of cuprates remains a subject of debate after more than two decades of investigation. Here we follow a new lead: The onset temperature for superconductivity scales with the strength of the anomalous normal-state scattering that makes the resistivity linear in temperature. The same correlation between linear resistivity and Tc is found in organic superconductors, for which pairing is known to come from fluctuations of a nearby antiferromagnetic phase, and in pnictide superconductors, for which an antiferromagnetic scenario is also likely. In the cuprates, the question is whether the pseudogap phase plays the corresponding role, with its fluctuations responsible for pairing and scattering. We review recent studies that shed light on this phase - its boundary, its quantum critical point, and its broken symmetries. The emerging picture is that of a phase with spin-density-wave order and fluctuations, in broad analogy with organic, pnictide, and heavy-fermion superconductors.
The electrical resistivity rho_c of the underdoped cuprate superconductor YBCO was measured perpendicular to the CuO_2 planes on ultra-high quality single crystals in magnetic fields large enough to suppress superconductivity. The incoherent insulating-like behavior of rho_c at high temperature, characteristic of all underdoped cuprates, is found to cross over to a coherent regime of metallic behavior at low temperature. This crossover coincides with the emergence of the small electron pocket detected in the Fermi surface of YBCO via quantum oscillations, the Hall and Seebeck coefficients and with the detection of a unidirectional modulation of the charge density as seen by high-field NMR measurements. The low coherence temperature is quantitatively consistent with the small hopping integral t_perp inferred from the splitting of the quantum oscillation frequencies. We conclude that the Fermi-surface reconstruction in YBCO at dopings from p = 0.08 to at least p = 0.15, attributed to stripe order, produces a metallic state with 3D coherence deep in the underdoped regime.
We apply a recently-developed low-field technique to inductively measure the critical pair momentum $p_c$ in thin, underdoped films of Y$_{1-x}$Ca$_{x}$Ba$_{2}$Cu$_{3}$O$_{7-delta}$ and Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+delta}$ reflecting a wide range of hole doping. We observe that $p_c propto hbar/xi$ scales with $T_c$ and therefore superfluid density $n_s(Trightarrow0)$ in our two-dimensional cuprate films. This relationship was famously predicted by a universal model of the cuprates with a textit{doping-independent} superconducting gap, but has not been observed by high field measurements of the coherence length $xi$ due to field-induced phenomena not included in the theory.
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