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We report experimental evidence of a mechanism that supports and intensifies induced magnetization at optical frequencies without the intervention of spin-orbit or spin-spin interactions. Energy-resolved spectra of scattered light, recorded at moderate intensities (108 W/cm2) and short timescales (<150 fs) in a series of non-magnetic molecular liquids, reveal the signature of torque dynamics driven jointly by the electric and magnetic field components of light at the molecular level. While past experiments have recorded radiant magnetization from magneto-electric interactions of this type, no evidence has been provided to date of the inelastic librational features expected in cross-polarized light scattering spectra due to the Lorentz force acting in combination with optical magnetic torque. Here, torque is shown to account for inelastic components in the magnetic scattering spectrum under conditions that produce no such features in electric dipole scattering, in excellent agreement with quantum theoretical predictions
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Modern optical nano-elements pursue ever-smaller sizes and individualized functionalities. Those elements that can efficiently manipulate the magnetic field of light boast promising future applications with a great challenge: the magnetic near field is irretrievable from conventional optical far-field characterization. Here we propose photoinduced magnetic force microscopy to directly and exclusively sense the magnetic field of light at the nanoscale. The proposed instrument exploits a magnetic nanoprobe with exclusive magnetic excitation under structured light illumination. The magnetic nanoprobe detects the photoinduced magnetic force, which is defined as the dipolar Lorentz force exerted on the photoinduced magnetic dipole in the nanoprobe. Since the resulting magnetic force is proportional to the incident magnetic field, the measured force reveals the magnetic near-field distribution at the nanoscale. The proposed instrument represents a fundamental step towards comprehensive electric and magnetic near-field detection and/or manipulation in single nano-element optical devices.
We show that the optical force field in optical tweezers with elliptically polarized beams has the opposite handedness for a wide range of particle sizes and for the most common configurations. Our method is based on the direct observation of the particle equilibrium position under the effect of a transverse Stokes drag force, and its rotation around the optical axis by the mechanical effect of the optical torque. We find overall agreement with theory, with no fitting, provided that astigmatism, which is characterized separately, is included in the theoretical description. Our work opens the way for characterization of the trapping parameters, such as the microsphere complex refractive index and the astigmatism of the optical system, from measurements of the microsphere rotation angle.
A key element in the generation of optical torque in optical traps, which occurs when electromagnetic angular momentum is transferred from the trapping beam to the trapped particle by scattering, is the symmetries of the scattering particle and the trapping beam. We discuss the effect of such symmetries on the generation and measurement of optical torque in optical tweezers, and some consequent general principles for the design of optically-driven micromachines.
We developed an all-optical link system for making remote comparisons of two distant ultra-stable optical clocks. An optical carrier transfer system based on a fiber interferometer was employed to compensate the phase noise accumulated during the propagation through a fiber link. Transfer stabilities of $2times10^{-15}$ at 1 second and $4times10^{-18}$ at 1000 seconds were achieved in a 90-km link. An active polarization control system was additionally introduced to maintain the transmitted light in an adequate polarization, and consequently, a stable and reliable comparison was accomplished. The instabilities of the all-optical link system, including those of the erbium doped fiber amplifiers (EDFAs) which are free from phase-noise compensation, were below $2times10^{-15}$ at 1 second and $7times10^{-17}$ at 1000 seconds. The system was available for the direct comparison of two distant $^{87}$Sr lattice clocks via an urban fiber link of 60 km. This technique will be essential for the measuring the reproducibility of optical frequency standards.
We present a theoretical study of the optical angular momentum transfer from a circularly polarized plane wave to thin metal nanoparticles of different rotational symmetries. While absorption has been regarded as the predominant mechanism of torque generation on the nanoscale, we demonstrate numerically how the contribution from scattering can be enhanced by using multipolar plasmon resonance. The multipolar modes in non-circular particles can convert the angular momentum carried by the scattered field, thereby producing scattering-dominant optical torque, while a circularly symmetric particle cannot. Our results show that the optical torque induced by resonant scattering can contribute to 80% of the total optical torque in gold particles. This scattering-dominant torque generation is extremely mode-specific, and deserves to be distinguished from the absorption-dominant mechanism. Our findings might have applications in optical manipulation on the nanoscale as well as new designs in plasmonics and metamaterials.
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