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We study the use of frequency upconversion schemes of near-IR picosecond laser pulses and compare their ability to guide and trigger electric discharges through filamentation in air. Upconversion, such as Second Harmonic Generation, is favorable for triggering electric discharges for given amount of available laser energy, even taking into account the losses inherent to frequency conversion. We focus on the practical question of optimizing the use of energy from a given available laser system and the potential advantage to use frequency conversion schemes.
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An 18-level argon collisional radiative model (CRM) suitable for low pressure was established. The model can be solved by combining the optical emission spectroscopy (OES) with Langmuir probe calibration. In the capacitively coupled plasmas (CCPs) with different frequency and power, the electron temperature and density obtained by the model were compared with those measured by Langmuir probe. It is found that the calibration point at any frequency or power is suitable for the fixed pressure. This method was then applied to the diagnosis of triple-frequency (TF) CCPs, it is shown that the high frequency (HF) power mainly controls the electron density, the low frequency (LF) power mainly controls the electron temperature, and the intermediate frequency (IF) power was between the two. Compared with the dual-frequency (DF) CCPs, it is found that with the increase of IF power, the HF power can control the electron density more independently with less influence on the electron temperature.
Laser frequency can be upconverted in a plasma undergoing ionization. For finite ionization rates, the laser pulse energy is partitioned into a pair of counter-propagating waves and static transverse currents. The wave amplitudes are determined by the ionization rates and the input pulse duration. The strongest output waves can be obtained when the plasma is fully ionized in a time that is shorter than the pulse duration. The static transverse current can induce a static magnetic field with instant ionization, but it dissipates as heat if the ionization time is longer than a few laser periods. This picture comports with experimental data, providing a description of both laser frequency upconverters as well as other laser-plasma interaction with evolving plasma densities.
An overview from the past and an outlook for the future of fundamental laser-plasma interactions research enabled by emerging laser systems.
When a relativistic laser pulse with high photon density interacts with a specially tailored thin foil target, a strong torque is exerted on the resulting spiral-shaped foil plasma, or light fan. Because of its structure, the latter can gain significant orbital angular momentum (OAM), and the opposite OAM is imparted to the reflected light, creating a twisted relativistic light pulse. Such an interaction scenario is demonstrated by particle-in-cell simulation as well as analytical modeling, and should be easily verifiable in the laboratory. As important characters, twisted relativistic light pulse has strong torque and ultra-high OAM density.
In this work, the temporal decay of electrons produced by an atmospheric pin-to-pin nanosecond discharge operating in the spark regime was measured via a combination of microwave Rayleigh scattering (MRS) and laser Rayleigh scattering (LRS). Due to the initial energy deposition of the nanosecond pulse, a variance in local gas density occurs on the timescale of electron decay. Thus, the assumption of a constant collisional frequency is no longer applicable when electron number data is extracted from the MRS measurements. To recalibrate the MRS measurements throughout the electron decay period, temporally-resolved LRS measurements of the local gas density were performed over the event duration. Local gas density was measured to be 30% of the ambient level during the later stages of electron decay and recovers at about 1 ms after the discharge. A shock front traveling approximately 500 m/s was additionally observed. Coupled with plasma volume calibration via temporally-resolved ICCD imaging, the corrected decay curves of the electron number and electron number density are presented with a measured peak electron number density of 4.5*10^15 cm^-3 and decay rate of ~ 0.1-0.35*10^7 s^-1. A hybrid MRS and LRS diagnostic technique can be applied for a broad spectrum of atmospheric-pressure microplasmas where a variation in number gas density is expected due to an energy deposition in the discharge.
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