No Arabic abstract
An elusive goal in the field of driven quantum matter is the induction of long-range order. Here, we demonstrate a mechanism based on light-induced evaporative cooling of holes in a correlated electron system. Since the entropy of a filled narrow band grows rapidly with hole doping, the isentropic transfer of holes from a doped Mott insulator to such a band results in a drop of temperature. Strongly correlated Fermi liquids and symmetry-broken states could thus be produced by dipolar excitations. Using nonequilibrium dynamical mean field theory, we show that suitably designed chirped pulses allow to realize this cooling effect. In particular, we demonstrate the emergence of antiferromagnetic order in a system which is initially in a weakly correlated state above the maximum Neel temperature. Our work suggests a general strategy for inducing strong correlation phenomena and electronic orders in light-driven materials or periodically modulated atomic gases in optical lattice potentials.
We theoretically study the thermal relaxation of many-body systems under the action of oscillating external fields. When the magnitude or the orientation of a field is modulated around values where the pairwise heat-exchange conductances depend non-linearly on this field, we demonstrate that the time symmetry is broken during the evolution of temperatures over a modulation cycle. We predict that this asymmetry enables a pumping of heat which can be used to cool down faster the system. This effect is illustrated through different magneto-optical systems under the action of an oscillating magnetic field.
We investigate the half-filled two-orbital Hubbard model with the crystalline electric field using dynamical mean-field theory combined with the continuous-time quantum Monte Carlo simulations. We systematically study how the interplay of the intra- and interorbital Coulomb interations together with the Hund coupling realizes the diagonal and off-diagonal ordered states. It is found that the antiferroorbital ordered state is realized in the Hubbard model, in addition to the antiferromagnetically ordered and excitonic states. The competition between the antiferroorbital ordered and excitonic states close to the band insulating state is addressed.
The time-dependent exact-diagonalization method is used to study the light-induced phase transition of magnetic orders in the anisotropic triangular-lattice Hubbard model. Calculating the spin correlation function, we confirm that the phase transition from the 120$^{circ}$ order to the N{e}el order can take place due to high-frequency periodic fields. We show that the effective Heisenberg-model Hamiltonian derived from the high-frequency expansion by the Floquet theory describes the present system very well and that the ratio of the exchange interactions expressed in terms of the frequency and amplitude of the external field determines the type of the magnetic orders. Our results demonstrate the controllability of the magnetic orders by tuning the external field.
To shed light on how electronic correlations vary across the phase diagram of the cuprate superconductors, we examine the doping evolution of spin and charge excitations in the single-band Hubbard model using determinant quantum Monte Carlo (DQMC). In the single-particle response, we observe that the effects of correlations weaken rapidly with doping, such that one may expect the random phase approximation (RPA) to provide an adequate description of the two-particle response. In contrast, when compared to RPA, we find that significant residual correlations in the two-particle excitations persist up to $40%$ hole and $15%$ electron doping (the range of dopings achieved in the cuprates). These fundamental differences between the doping evolution of single- and multi-particle renormalizations show that conclusions drawn from single-particle processes cannot necessarily be applied to multi-particle excitations. Eventually, the system smoothly transitions via a momentum-dependent crossover into a weakly correlated metallic state where the spin and charge excitation spectra exhibit similar behavior and where RPA provides an adequate description.
Phase transitions and symmetry are intimately linked. Melting of ice, for example, restores translation invariance. The mysterious hidden order (HO) phase of URu$_2$Si$_2$ has, despite relentless research efforts, kept its symmetry breaking element intangible. Here we present a high-resolution x-ray diffraction study of the URu$_2$Si$_2$ crystal structure as a function of hydrostatic pressure. Below a critical pressure threshold $p_capprox3$ kbar, no tetragonal lattice symmetry breaking is observed even below the HO transition $T_{HO}=17.5$ K. For $p>p_c$, however, a pressure-induced rotational symmetry breaking is identified with an onset temperatures $T_{OR}sim 100$ K. The emergence of an orthorhombic phase is found and discussed in terms of an electronic nematic order that appears unrelated to the HO, but with possible relevance for the pressure-induced antiferromagnetic (AF) phase. Existing theories describe the HO and AF phases through an adiabatic continuity of a complex order parameter. Since none of these theories predicts a pressure-induced nematic order, our finding adds an additional symmetry breaking element to this long-standing problem.