Do you want to publish a course? Click here

Vectorial optical field reconstruction by attosecond spectral interferometry

62   0   0.0 ( 0 )
 Publication date 2019
  fields Physics
and research's language is English




Ask ChatGPT about the research

An electrical pulse E(t) is completely defined by its time-dependent amplitude and polarisation direction. For optical pulses the manipulation and characterisation of the light polarisation state is fundamental due to its relevance in several scientific and technological fields. In this work we demonstrate the complete temporal reconstruction of the electric field of few-cycle pulses with a complex time-dependent polarisation. Our experimental approach is based on extreme ultraviolet interferometry with isolated attosecond pulses and on the demonstration that the motion of an attosecond electron wave packet is sensitive to perturbing fields only along the direction of its motion. By exploiting the sensitivity of interferometric techniques and by controlling the emission and acceleration direction of the wave packet, pulses with energies as low as few hundreds of nanojoules can be reconstructed. Our approach opens the possibility to completely characterise the electric field of the pulses typically used in visible pump-probe spectroscopy.



rate research

Read More

74 - Li Zhang , Fei Lin , Xiaodong Qiu 2018
Nonlinear optical generation has been a well-established way to realize frequency conversion in nonlinear optics, whereas previous studies were just focusing on the scalar light fields. Here we report a concise yet efficient experiment to realize frequency conversion from vector fields to vector fields based on the vectorial nonlinear optical process, e.g., the second-harmonic generation. Our scheme is based on two cascading type-I phase-matching BBO crystals, whose fast axes are configured elaborately to be perpendicular to each other. Without loss of generality, we take the full Poincare beams as the vectorial light fields in our experiment, and visualize the structured features of vectorial second-harmonic fields by using Stokes polarimetry. The interesting doubling effect of polarization topological index, i.e., a low-order full Poincare beam is converted to a high-order one are demonstrated. However, polarization singularities of both C-points and L-lines are found to keep invariant during the SHG process. Our scheme can be straightforwardly generalized to other nonlinear optical effects. Our scheme can offer a deeper understanding on the interaction of vectorial light with media and may find important applications in optical imaging, optical communication and quantum information science.
The coherent exchange of optical near fields between two neighboring dipoles plays an essential role for the optical properties, quantum dynamics and thus for the function of many naturally occurring and artificial nanosystems. These interactions are inherently short-ranged, extending over a few nanometers only, and depend sensitively on relative orientation, detuning and dephasing, i.e., on the vectorial properties of the coupled dipolar near fields. This makes it challenging to analyze them experimentally. Here, we introduce plasmonic nanofocusing spectroscopy to record coherent light scattering spectra with 5-nm spatial resolution from a small dipole antenna, excited solely by evanescent fields and coupled to plasmon resonances in a single gold nanorod. We resolve mode couplings, resonance energy shifts and Purcell effects as a function of dipole distance and relative orientation, and show how they arise from different vectorial components of the interacting optical near-fields. Our results pave the way for using dipolar alignment to control the optical properties and function of nanoscale systems.
430 - J. F. Tao , J. Cai , Q. Z. Xia 2019
In this paper, we propose a new method to characterize the temporal structure of arbitrary optical laser pulses with low pulse energies. This approach is based on strong field photoelectron holography with the glory rescattering effect as the underlying mechanism in the near-forward direction. Utilizing the subfemtosecond glory rescattering process as a fast temporal gate to sample the unknown light pulse, the time-dependent vectorial electric field can be retrieved from the streaking photoelectron momentum spectra. Our method avoids the challenging task of generation or manipulation of attosecond pulses and signifies important progress in arbitrary optical waveform characterization.
The reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) is one of the most widely used techniques for resolving ultrafast electronic dynamics in atomic and molecular systems. As it relies on the interference of photo-electrons in vacuum, similar interference has never been contemplated in the bulk of crystals. Here we show that the interference of two-photon transitions can be recorded directly in the bulk of solids and read out with standard angle-resolved photo-emission spectroscopy. The phase of the RABBIT beating in the photoelectron spectra coming from the bulk of solids is sensitive to the relative phase of the Berry connection between bands and it experiences a shift of $pi$ as one of the quantum paths crosses a band. For resonant interband transitions, the amplitude of the RABBIT oscillation decays as the pump and probe pulses are separated in time due to electronic decoherence, providing a simple interferometric method to extract dephasing times.
We demonstrate a new technique for the experimental measurement of the spectral coherence of microresonator optical frequency combs. Specifically, we use a spectral interference method, typically used in the context of supercontinuum generation, to explore the variation of the complex degree of first order coherence across the full comb bandwidth. We measure the coherence of two different frequency combs, and observe wholly different coherence characteristics. In particular, we find that the observed dynamical regimes are similar to the stable and unstable modulation instability regimes reported in previous theoretical studies. Results from numerical simulations are found to be in good agreement with experimental observations. In addition to demonstrating a new technique to assess comb stability, our results provide strong experimental support for previous theoretical analyses.
comments
Fetching comments Fetching comments
Sign in to be able to follow your search criteria
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا