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Unidirectional light transmission by two-layer nanostructures interacting via optical near-fields

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 Added by Serge Huant
 Publication date 2019
  fields Physics
and research's language is English




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We experimentally demonstrate unidirectional light transmission through two-layer nanostructured materials considering that the horizontal-to-vertical-polarization conversion efficiency in the forward direction and the vertical-to-horizontal efficiency in the backward direction, which are usually equivalent due to optical reciprocity, are different. The different ways of transferring light momentum in the forward and backward directions via optical near-fields between the layers are responsible for the unidirectionality of light, which was theoretically investigated in our recent work [J. Opt. Soc. Am. B 31, 2404-2413]. With two-layer metal nanostructures experimentally fabricated via a repeated lift-off technique, consistent optical characteristics are observed, verifying the utilization of the large momentum of optical near-fields.

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We theoretically demonstrate direction-dependent polarization conversion efficiency, yielding unidirectional light transmission, through a two-layer nanostructure by using the angular spectrum representation of optical near-fields. The theory provides results that are consistent with electromagnetic numerical simulations. This study reveals that optical near-field interactions among nanostructured matter can provide unique optical properties, such as the unidirectionality observed here, and offers fundamental guiding principles for understanding and engineering nanostructures for realizing novel functionalities.
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We predict a dynamic metallization effect where an ultrafast (single-cycle) optical pulse with a field less or on the order of 1 V/Angstrom causes plasmonic metal-like behavior of a dielectric film with a few-nm thickness. This manifests itself in plasmonic oscillations of polarization and a significant population of the conduction band evolving on a femtosecond time scale. These phenomena are due a combination of both adiabatic (reversible) and diabatic (for practical purposes irreversible) pathways.
We investigate the appearance of pi lapses in the transmission phase theta of a two-level quantum dot with Coulomb interaction U. Using the numerical and functional renormalization group methods we study the entire parameter space for spin-polarized as well as spin-degenerate dots, modeled by spinless or spinful electrons, respectively. We investigate the effect of finite temperatures T. For small T and sufficiently small single-particle spacings delta of the dot levels we find pi phase lapses between two transmission peaks in an overwhelming part of the parameter space of the level-lead couplings. For large delta the appearance or not of a phase lapse between resonances depends on the relative sign of the level-lead couplings in analogy to the U=0 case. We show that this generic scenario is the same for spin-polarized and spin-degenerate dots. We emphasize that in contrast to dots with more levels, for a two-level dot with small delta and generic dot-lead couplings (that is up to cases with special symmetry) the universal phase lapse behavior is already established at U=0. The most important effect of the Coulomb interaction is to increase the separation of the transmission resonances. The relation of the appearance of phase lapses to the inversion of the population of the dot levels is discussed. For the spin-polarized case and low temperatures we compare our results to recent mean-field studies. For small delta correlations are found to strongly alter the mean-field picture.
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