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Register a new userEnergy spectrum of two-dimensional excitons in a non-uniform dielectric medium
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We demonstrate that, in monolayers (MLs) of semiconducting transition metal dichalcogenides, the $s$-type Rydberg series of excitonic states follows a simple energy ladder: $epsilon_n=-Ry^*/(n+delta)^2$, $n$=1,2,ldots, in which $Ry^*$ is very close to the Rydberg energy scaled by the dielectric constant of the medium surrounding the ML and by the reduced effective electron-hole mass, whereas the ML polarizability is only accounted for by $delta$. This is justified by the analysis of experimental data on excitonic resonances, as extracted from magneto-optical measurements of a high-quality WSe$_2$ ML encapsulated in hexagonal boron nitride (hBN), and well reproduced with an analytically solvable Schrodinger equation when approximating the electron-hole potential in the form of a modified Kratzer potential. Applying our convention to other, MoSe$_2$, WS$_2$, MoS$_2$ MLs encapsulated in hBN, we estimate an apparent magnitude of $delta$ for each of the studied structures. Intriguingly, $delta$ is found to be close to zero for WSe$_2$ as well as for MoS$_2$ monolayers, what implies that the energy ladder of excitonic states in these two-dimensional structures resembles that of Rydberg states of a three-dimensional hydrogen atom.
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We propose a robust and efficient way of controlling the optical spectra of two-dimensional materials and van der Waals heterostructures by quantum cavity embedding. The cavity light-matter coupling leads to the formation of exciton-polaritons, a superposition of photons and excitons. Our first principles study demonstrates a reordering and mixing of bright and dark excitons spectral features and in the case of a type II van-der-Waals heterostructure an inversion of intra and interlayer excitonic resonances. We further show that the cavity light-matter coupling strongly depends on the dielectric environment and can be controlled by encapsulating the active 2D crystal in another dielectric material. Our theoretical calculations are based on a newly developed non-perturbative many-body framework to solve the coupled electron-photon Schrodinger equation in a quantum-electrodynamical extension of the Bethe-Salpeter approach. This approach enables the ab-initio simulations of exciton-polariton states and their dispersion from weak to strong cavity light-matter coupling regimes. Our method is then extended to treat van der Waals heterostructures and encapsulated 2D materials using a simplified Mott-Wannier description of the excitons that can be applied to very large systems beyond reach for fully ab-initio approaches.
We report a two-dimensional artificial lattice for dipolar excitons confined in a GaAs double quantum well. Exploring the regime of large fillings per lattice site, we verify that the lattice depth competes with the magnitude of excitons repulsive dipolar interactions to control the degree of localisation in the lattice potential. Moreover, we show that dipolar excitons radiate a narrow-band photoluminescence, with a spectral width of a few hundreds of micro-eV at 340 mK, in both localised and delocalised regimes. This makes our device suitable for explorations of dipolar excitons quasi-condensation in a periodic potential.
The results of experimental study of the magnetoresistivity, the Hall and Shubnikov-de Haas effects for the heterostructure with HgTe quantum well of 20.2 nm width are reported. The measurements were performed on the gated samples over the wide range of electron and hole densities including vicinity of a charge neutrality point. Analyzing the data we conclude that the energy spectrum is drastically different from that calculated in framework of $kP$-model. So, the hole effective mass is equal to approximately $0.2 m_0$ and practically independent of the quasimomentum ($k$) up to $k^2gtrsim 0.7times 10^{12}$ cm$^{-2}$, while the theory predicts negative (electron-like) effective mass up to $k^2=6times 10^{12}$ cm$^{-2}$. The experimental effective mass near k=0, where the hole energy spectrum is electron-like, is close to $-0.005 m_0$, whereas the theoretical value is about $-0.1 m_0$.
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