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Register a new userLaser refrigeration using exciplex resonances in gas filled hollow-core fibres
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We theoretically study prospects and limitations of a new route towards macroscopic scale laser refrigeration based on exciplex-mediated frequency up-conversion in gas filled hollow-core fibres. Using proven quantum optical rate equations we model the dynamics of a dopant-buffer gas mixture filling an optically pumped waveguide. In the particular example of alkali-noble gas mixtures, recent high pressure gas cell setup experiments have shown that efficient kinetic energy extraction cycles appear via the creation of transient exciplex excited electronic bound states. The cooling cycle consists of absorption of lower energy laser photons during collisions followed by blue-shifted spontaneous emission on the atomic line of the alkali atoms. For any arbitrary dopant-buffer gas mixture, we derive scaling laws for cooling power, cooling rates and temperature drops with varying input laser power, dopant and buffer gas concentration, fibre geometry and particularities of the exciplex ground and excited state potential landscapes.
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A new configuration for observation of magneto-optical subnatural-linewidth resonances of electromagnetically induced absorption (EIA) in alkali vapor has been verified experimentally. The configuration includes using two counter-propagating pump and probe light waves with mutually orthogonal linear polarizations, exciting an open optical transition of an alkali atom in the presence of a buffer gas. The main advantage of the novel observation scheme consists in the possibility of obtaining simultaneously high-contrast and quite narrow nonlinear signals. Here a 2.5-cm long rubidium-87 vapor cell filled with Ar buffer gas is used, and the excited optical transition is the F$_g$=2 $to$ F$_e$=1 of the D$_1$ line. The signals registered reach a contrast of 57.7% with a FWHM of 7.2 mG. The contrast with respect to a wide Doppler pedestal well exceeds 100%. To our knowledge, to date this is the best result for EIA resonances in terms of contrast-to-width ratio. In general, the results demonstrate that the new magneto-optical scheme has very good prospects for various applications in quantum metrology, nonlinear optics and photonics.
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