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Register a new userIntrapulse Impact Processes in Dense-Gas Femtosecond Laser Filamentation
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The processes of energy gain and redistribution in a dense gas subject to an intense ultrashort laser pulse are investigated theoretically for the case of high-pressure argon. The electrons released via strong-field ionization and driven by oscillating laser field collide with neutral neighbor atoms, thus effecting the energy gain in the emerging electron gas via a short-range inverse Bremsstrahlung interaction. These collisions also cause excitation and impact ionization of the atoms thus reducing the electron-gas energy. A kinetic model of these competing processes is developed which predicts the prevalence of excited atoms over ionized atoms by the end of the laser pulse. The creation of a significant number of excited atoms during the pulse in high-pressure gases is consistent with the delayed ionization dynamics in the pulse wake, recently discovered by Gao et al.[1] This energy redistribution mechanism offers an approach to manage effectively the excitation vs. ionization patterns in dense gases interacting with intense laser pulses and thus opens new avenues for diagnostics and control in these settings.
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In magnetoplasmonics, it is possible to tailor the magneto-optical properties of nanostructures by exciting surface plasmon polaritons (SPPs). Thus far, magnetoplasmonic effects have been considered static. Here, we describe ultrafast manifestations of magnetoplasmonics by observing the non-trivial evolution of the transverse magneto-optic Kerr effect within 45-fs pulses reflected from an iron-based magnetoplasmonic crystal. The effect occurs for resonant SPP excitations, displays opposite time derivative signs for different slopes of the resonance, and is explained with the magnetization-dependent dispersion relation of SPPs.
We present experimental measurements of the femtosecond time-scale generation of strong magnetic-field fluctuations during the interaction of ultrashort, moderately relativistic laser pulses with solid targets. These fields were probed using low-emittance, highly relativistic electron bunches from a laser wakefield accelerator, and a line-integrated $B$-field of $2.70 pm 0.39,rm kT,mu m$ was measured. Three-dimensional, fully relativistic particle-in-cell simulations indicate that such fluctuations originate from a Weibel-type current filamentation instability developing at submicron scales around the irradiated target surface, and that they grow to amplitudes strong enough to broaden the angular distribution of the probe electron bunch a few tens of femtoseconds after the laser pulse maximum. Our results highlight the potential of wakefield-accelerated electron beams for ultrafast probing of relativistic laser-driven phenomena.
While filaments are generally interpreted as a dynamic balance between Kerr focusing and plasma defocusing, the role of the higher-order Kerr effect (HOKE) is actively debated as a potentially dominant defocusing contribution to filament stabilization. In a pump-probe experiment supported by numerical simulations, we demonstrate the transition between two distinct filamentation regimes at 800,nm. For long pulses (1.2 ps), the plasma substantially contributes to filamentation, while this contribution vanishes for short pulses (70 fs). These results confirm the occurrence, in adequate conditions, of filamentation driven by the HOKE rather than by plasma.
We disclose an unanticipated link between plasmonics and nonlinear frequency down-conversion in laser-induced gas-plasmas. For two-color femtosecond pump pulses, a plasmonic resonance is shown to broaden the terahertz emission spectra significantly. We identify the resonance as a leaky mode, which contributes to the emission spectra whenever electrons are excited along a direction where the plasma size is smaller than the plasma wavelength. As a direct consequence, such resonances can be controlled by changing the polarization properties of elliptically-shaped driving laser pulses. Both, experimental results and 3D Maxwell consistent simulations confirm that a significant terahertz pulse shortening and spectral broadening can be achieved by exploiting the transverse driving laser beam shape as an additional degree of freedom.
In [I.R. Khairulin et al., submitted to Phys. Rev. Lett.] we propose a method for amplifying a train of sub-femtosecond pulses of circularly or elliptically polarized extreme ultraviolet (XUV) radiation, constituted by high-order harmonics of an infrared (IR) laser field, in a neon-like active medium of a plasma-based X-ray laser, additionally irradiated with a replica of a fundamental frequency laser field used to generate harmonics, and show the possibility of maintaining or enhancing the ellipticity of high-harmonic radiation during its amplification. In the present paper we describe this process in detail both for a single harmonic component and a sub-femtosecond pulse train formed by a set of harmonics. We derive the analytical theory and describe both analytically and numerically the evolution of the high-harmonic field during its propagation through the medium. We discuss also the possibility of an experimental implementation of the suggested technique in an active medium of an X-ray laser based on neon-like Ti^{12+} ions irradiated by an IR laser field with a wavelength of 3.9 microns.
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