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Register a new userElectronic properties of type-II Weyl semimetal WTe$_2$. A review perspective
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Currently, there is a flurry of research interest on materials with an unconventional electronic structure, and we have already seen significant progress in their understanding and engineering towards real-life applications. The interest erupted with the discovery of graphene and topological insulators in the previous decade. The electrons in graphene simulate massless Dirac Fermions with a linearly dispersing Dirac cone in their band structure, while in topological insulators, the electronic bands wind non-trivially in momentum space giving rise to gapless surface states and bulk bandgap. Weyl semimetals in condensed matter systems are the latest addition to this growing family of topological materials. Weyl Fermions are known in the context of high energy physics since almost the beginning of quantum mechanics. They apparently violate charge conservation rules, displaying the chiral anomaly, with such remarkable properties recently theoretically predicted and experimentally verified to exist as low energy quasiparticle states in certain condensed matter systems. Not only are these new materials extremely important for our fundamental understanding of quantum phenomena, but also they exhibit completely different transport phenomena. For example, massless Fermions are susceptible to scattering from non-magnetic impurities. Dirac semimetals exhibit non-saturating extremely large magnetoresistance as a consequence of their robust electronic bands being protected by time reversal symmetry. These open up whole new possibilities for materials engineering and applications including quantum computing. In this review, we recapitulate some of the outstanding properties of WTe$_2$, namely, its non-saturating titanic magnetoresistance due to perfect electron and hole carrier balance up to a very high magnetic field observed for the very first time. (Continued. Please see the main article).
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By combining bulk sensitive soft-X-ray angular-resolved photoemission spectroscopy and accurate first-principles calculations we explored the bulk electronic properties of WTe$_2$, a candidate type-II Weyl semimetal featuring a large non-saturating magnetoresistance. Despite the layered geometry suggesting a two-dimensional electronic structure, we find a three-dimensional electronic dispersion. We report an evident band dispersion in the reciprocal direction perpendicular to the layers, implying that electrons can also travel coherently when crossing from one layer to the other. The measured Fermi surface is characterized by two well-separated electron and hole pockets at either side of the $Gamma$ point, differently from previous more surface sensitive ARPES experiments that additionally found a significant quasiparticle weight at the zone center. Moreover, we observe a significant sensitivity of the bulk electronic structure of WTe$_2$ around the Fermi level to electronic correlations and renormalizations due to self-energy effects, previously neglected in first-principles descriptions.
The carrier dynamics and electronic structures of type-II Weyl semimetal candidates MoTe$_2$ and WTe$_2$ have been investigated by using temperature-dependent optical conductivity [$sigma(omega)$] spectra. Two kinds of Drude peaks (narrow and broad) have been separately observed. The width of the broad Drude peak increases with elevating temperature above the Debye temperature of about 130 K in the same way as those of normal metals, on the other hand, the narrow Drude peak becomes visible below 80 K and the width is rapidly suppressed with decreasing temperature. Because the temperature dependence of the narrow Drude peak is similar to that of a type-I Weyl semimetal TaAs, it was concluded to originate from Dirac carriers of Weyl bands. The result suggests that the conductance has the contribution of two kinds of carriers, normal semimetallic and Dirac carriers, and this observation is an evidence of type-II Weyl semimetals of MoTe$_2$ and WTe$_2$. The obtained $sigma(omega)$ spectra in the interband transition region can be explained by band structure calculations with a band renormalization owing to electron correlation.
We perform ultrahigh resolution angle-resolved photoemission experiments at a temperature T=0.8 K on the type-II Weyl semimetal candidate WTe$_{2}$. We find a surface Fermi arc connecting the bulk electron and hole pockets on the (001) surface. Our results show that the surface Fermi arc connectivity to the bulk bands is strongly mediated by distinct surface resonances dispersing near the border of the surface-projected bulk band gap. By comparing the experimental results to first-principles calculations we argue that the coupling to these surface resonances, which are topologically trivial, is compatible with the classification of WTe$_{2}$ as a type-II Weyl semimetal hosting topological Fermi arcs. We further support our conclusion by a systematic characterization of the bulk and surface character of the different bands and discuss the similarity of our findings to the case of topological insulators.
Topological quantum materials, including topological insulators and superconductors, Dirac semimetals and Weyl semimetals, have attracted much attention recently for their unique electronic structure, spin texture and physical properties. Very lately, a new type of Weyl semimetals has been proposed where the Weyl Fermions emerge at the boundary between electron and hole pockets in a new phase of matter, which is distinct from the standard type I Weyl semimetals with a point-like Fermi surface. The Weyl cone in this type II semimetals is strongly tilted and the related Fermi surface undergos a Lifshitz transition, giving rise to a new kind of chiral anomaly and other new physics. MoTe2 is proposed to be a candidate of a type II Weyl semimetal; the sensitivity of its topological state to lattice constants and correlation also makes it an ideal platform to explore possible topological phase transitions. By performing laser-based angle-resolved photoemission (ARPES) measurements with unprecedentedly high resolution, we have uncovered electronic evidence of type II semimetal state in MoTe2. We have established a full picture of the bulk electronic states and surface state for MoTe2 that are consistent with the band structure calculations. A single branch of surface state is identified that connects bulk hole pockets and bulk electron pockets. Detailed temperature-dependent ARPES measurements show high intensity spot-like features that is ~40 meV above the Fermi level and is close to the momentum space consistent with the theoretical expectation of the type II Weyl points. Our results constitute electronic evidence on the nature of the Weyl semimetal state that favors the presence of two sets of type II Weyl points in MoTe2.
We have investigated the magnetoresistance (MR) and Hall resistivity properties of the single crystals of tantalum sulfide, Ta3S2, which was recently predicted to be a new type II Weyl semimetal. Large MR (up to ~8000% at 2 K and 16 T), field-induced metal-insulator-like transition and nonlinear Hall resistivity are observed at low temperatures. The large MR shows a strong dependence on the field orientation, leading to a giant anisotropic magnetoresistance (AMR) effect. For the field applied along the b-axis (B//b), MR exhibits quadratic field dependence at low fields and tends towards saturation at high fields; while for B//a, MR presents quadratic field dependence at low fields and becomes linear at high fields without any trend towards saturation. The analysis of the Hall resistivity data indicates the coexistence of a large number of electrons with low mobility and a small number of holes with high mobility. Shubnikov-de Haas (SdH) oscillation analysis reveals three fundamental frequencies originated from the three-dimensional (3D) Fermi surface (FS) pockets. We find that the semi-classical multiband model is sufficient to account for the experimentally observed MR in Ta3S2.
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