No Arabic abstract
We have investigated the metamagnetic-like transition in the triple layer ruthenate Sr4Ru3O10 by means of neutron diffraction from single crystals. The magnetic structure of the compound appears to be determined in a complex way by the two substructures of inequivalent ruthenium ions. At Tc=105K the system has a sharp transition into a ferromagnetic state along the c-axis which is driven by the ruthenium atoms in the central octahedra of the triple layers whereas the substructure of the outer ruthenium atoms tend to align in the ab plane achieving an antiferromagnetic order at the metamagnetic transition T*~50K. Below T* the strong anisotropy along c prevails, the outer ruthenium tend to align along the c-axis and the in-plane antiferromagnetic order disappears. This finding confirms the delicate balance between antiferro and ferromagnetic couplings in the (Sr,Ca)n+1RunO3n+1 family of compounds, and proves the layer dependence of the magnetic anisotropy in Sr4Ru3O10.
We show that the metamagnetic transition in Sr$_4$Ru$_3$O$_{10}$ bifurcates into two transitions as the field is rotated away from the conducting planes. This two-step process comprises partial or total alignment of moments in ferromagnetic bands followed by an itinerant metamagnetic transition whose critical field increases with rotation. Evidence for itinerant metamagnetism is provided by the Shubnikov-de Hass effect which shows a non-trivial evolution of the geometry of the Fermi surface and an enhancement of the quasiparticles effective-mass across the transition. The metamagnetic response of Sr$_4$Ru$_3$O$_{10}$ is orbital-dependent and involves ferromagnetic and metamagnetic bands.
The local spectroscopic signatures of metamagnetic criticality in Sr3Ru2O7 were explored using scanning tunneling microscopy (STM). Singular features in the tunneling spectrum were found close to the Fermi level, as would be expected in a Stoner picture of itinerant electron metamagnetism. These features showed a pronounced magnetic field dependence across the metamagnetic critical point, which cannot be understood in terms of a naive Stoner theory. In addition, a pseudo-gap structure was observed over several tens of meV, accompanied by a c(2x2) superstructure in STM images. This result represents a new electronic ordering at the surface in the absence of any measurable surface reconstruction.
We investigate the behavior of ultrasharp metamagnetic transitions in La(5/8-y)Nd(y)Ca(3/8)MnO(3) manganites. These compounds change from a low temperature ferromagnetic metallic state at low Nd doping to a charge-ordered antiferromagnetic insulator for high Nd content. At an intermediate doping a phase-separated state is established. At low temperatures (2 K), we observe an avalanche-like field-induced metamagnetic transition, when the entire compound changes abruptly from one phase to the other. We investigate the signatures of this ultrasharp transition using magnetization and specific heat measurements. We observe a first order transition in the specific heat associated with discontinuous jumps in the magnetization. A strong increase of the sample temperature is simultaneously observed. The results are interpret in terms of latent heat release from the field induced enhancement of the ferromagnetic fraction, triggering the avalanche process.
We report on the electronic and thermodynamic properties of the antiferromagnetic metal uranium mononitride with a Neel temperature $T_Napprox 53,$K. The fabrication of microstructures from single crystals enables us to study the low-temperature metamagnetic transition at approximately $58,$T by high-precision magnetotransport, Hall-effect, and magnetic-torque measurements. We confirm the evolution of the high-field transition from a broad and complex behavior to a sharp first-order-like step, associated with a spin flop at low temperature. In the high-field state, the magnetic contribution to the temperature dependence of the resistivity is suppressed completely. It evolves into an almost quadratic dependence at low temperatures indicative of a metallic character. Our detailed investigation of the Hall effect provides evidence for a prominent Fermi-surface reconstruction as the system is pushed into the high-field state.
We report detailed investigation of quantum oscillations in Sr3Ru2O7, observed inductively (the de Haas-van Alphen effect) and thermally (the magnetocaloric effect). Working at fields from 3 T to 18 T allowed us to straddle the metamagnetic transition region and probe the low- and high-field Fermi liquids. The observed frequencies are strongly field-dependent in the vicinity of the metamagnetic transition, and there is evidence for magnetic breakdown. We also present the results of a comprehensive rotation study. The most surprising result concerns the field dependence of the measured quasiparticle masses. Contrary to conclusions previously drawn by some of us as a result of a study performed with a much poorer signal to noise ratio, none of the five Fermi surface branches for which we have good field-dependent data gives evidence for a strong field dependence of the mass. The implications of these experimental findings are discussed.