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Register a new userOscillating quadrupole effects in high precision metrology
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The influence of oscillating quadrupole fields on atomic energy levels is examined theoretically and general expressions for the quadrupole matrix elements are given. The results are relevant to any ion-based clock in which one of the clock states supports a quadrupole moment. Clock shifts are estimated for $^{176}$Lu$^+$ and indicate that coupling to the quadrupole field would not be a limitation to clock accuracy at the $lesssim10^{-19}$ level. Nevertheless, a method is suggested that would allow this shift to be calibrated. This method utilises a resonant quadrupole coupling that enables the quadrupole moment of the atom to be measured. A proof-of-principle demonstration is given using $^{138}$Ba$^+$, in which the quadrupole moment of the $D_{5/2}$ state is estimated to be $Theta=3.229(89) e a_0^2$.
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We examine a range of effects arising from ac magnetic fields in high precision metrology. These results are directly relevant to high precision measurements, and accuracy assessments for state-of-the-art optical clocks. Strategies to characterize these effects are discussed and a simple technique to accurately determine trap-induced ac magnetic fields in a linear Paul trap is demonstrated using $^{171}mathrm{Yb}^+$
We show that quantification of the performance of quantum-enhanced measurement schemes based on the concept of quantum Fisher information yields asymptotically equivalent results as the rigorous Bayesian approach, provided generic uncorrelated noise is present in the setup. At the same time, we show that for the problem of decoherence-free phase estimation this equivalence breaks down and the achievable estimation uncertainty calculated within the Bayesian approach is by a $pi$ factor larger than that predicted by the QFI even in the large prior knowledge (small parameter fluctuation) regime, where QFI is conventionally regarded as a reliable figure of merit. We conjecture that the analogous discrepancy is present in arbitrary decoherence-free unitary parameter estimation scheme and propose a general formula for the asymptotically achievable precision limit. We also discuss protocols utilizing states with indefinite number of particles and show that within the Bayesian approach it is legitimate to replace the number of particles with the mean number of particles in the formulas for the asymptotic precision, which as a consequence provides another argument that proposals based on the properties of the QFI of indefinite particle number states leading to sub-Heisenberg precisions are not practically feasible.
In an idealistic setting, quantum metrology protocols allow to sense physical parameters with mean squared error that scales as $1/N^2$ with the number of particles involved---substantially surpassing the $1/N$-scaling characteristic to classical statistics. A natural question arises, whether such an impressive enhancement persists when one takes into account the decoherence effects that are unavoidable in any real-life implementation. In this thesis, we resolve a major part of this issue by describing general techniques that allow to quantify the attainable precision in metrological schemes in the presence of uncorrelated noise. We show that the abstract geometrical structure of a quantum channel describing the noisy evolution of a single particle dictates then critical bounds on the ultimate quantum enhancement. Our results prove that an infinitesimal amount of noise is enough to restrict the precision to scale classically in the asymptotic $N$ limit, and thus constrain the maximal improvement to a constant factor. Although for low numbers of particles the decoherence may be ignored, for large $N$ the presence of noise heavily alters the form of both optimal states and measurements attaining the ultimate resolution. However, the established bounds are then typically achievable with use of techniques natural to current experiments. In this work, we thoroughly introduce the necessary concepts and mathematical tools lying behind metrological tasks, including both frequentist and Bayesian estimation theory frameworks. We provide examples of applications of the methods presented to typical qubit noise models, yet we also discuss in detail the phase estimation tasks in Mach-Zehnder interferometry both in the classical and quantum setting---with particular emphasis given to photonic losses while analysing the impact of decoherence.
Quantum metrology employs quantum effects to attain a measurement precision surpassing the limit achievable in classical physics. However, it was previously found that the precision returns the shot-noise limit (SNL) from the ideal Zeno limit (ZL) due to the photon loss in quantum metrology based on Mech-Zehnder interferometer. Here, we find that not only the SNL can be beaten, but also the ZL can be asymptotically recovered in long-encoding-time condition when the photon dissipation is exactly studied in its inherent non-Markovian manner. Our analysis reveals that it is due to the formation of a bound state of the photonic system and its dissipative noise. Highlighting the microscopic mechanism of the dissipative noise on the quantum optical metrology, our result supplies a guideline to realize the ultrasensitive measurement in practice by forming the bound state in the setting of reservoir engineering.
We present a method that uses radio-frequency pulses to cancel the quadrupole shift in optical clock transitions. Quadrupole shifts are an inherent inhomogeneous broadening mechanism in trapped ion crystals, limiting current optical ion clocks to work with a single probe ion. Cancelling this shift at each interrogation cycle of the ion frequency allows the use of $N>1$ ions in clocks, thus reducing the uncertainty in the clock frequency by $sqrt{N}$ according to the standard quantum limit. Our sequence relies on the tensorial nature of the quadrupole shift, and thus also cancels other tensorial shifts, such as the tensor ac stark shift. We experimentally demonstrate our sequence on three and seven $^{88}mathrm{Sr}^{+}$ ions trapped in a linear Paul trap, using correlation spectroscopy. We show a reduction of the quadrupole shift difference between ions to $approx20$ mHzs level where other shifts, such as the relativistic 2$^{mathrm{nd}}$ order Doppler shift, are expected to limit our spectral resolution. In addition, we show that using radio-frequency dynamic decoupling we can also cancel the effect of 1$^{mathrm{st}}$ order Zeeman shifts.
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