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Register a new userEffect of Cu doping on superconductivity in TaSe$_3$: Relationship between superconductivity and induced charge density wave
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By measuring the temperature dependence of the resistance, we investigated the effect of Cu doping on superconductivity (SC) in Cu-doped TaSe$_3$ in which the charge density wave (CDW) transition is induced by Cu doping. We observed an emergence of a region where the SC transition temperature ($T_mathrm{C}$) decreased in samples with higher Cu concentrations and found that the region tended to expand with increasing Cu concentration. In addition, the temperature dependence of the upper critical field ($H_mathrm{C2}$) of Cu-doped TaSe$_3$ was found to differ from that of pure TaSe$_3$. Based on these experimental results and the fact that the SC of TaSe$_3$ is filamentary, we conclude that SC is suppressed locally by Cu doping and competes with the CDW in Cu-doped TaSe$_3$. The resistance anomaly due to the CDW transition was extremely small and the size of the anomaly was enhanced with increasing Cu concentration but the temperature at which the anomaly appeared hardly changed. This result of the anomaly and the local suppression of SC imply that the induced CDWs are short-range order in the vicinity of Cu atoms. We also discuss the effect of the pinning of CDWs on the relationship between SC and short-range order CDWs.
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Here we report a systematic investigation on the evolution of the structural and physical properties, including the charge density wave and superconductivity of the polycrystalline CuIr2Te4-xIx. X-ray diffraction results indicate that both of a and c lattice parameters increase linearly. The resistivity measurements indicate that the charge density wave is destabilized with slight x but reappears when x is large than 0.9. Meanwhile, the superconducting transition temperature enhances as x raises and reaches a maximum value of around 2.95 K for the optimal composition CuIr2Te3.9I0.1 followed by a slight decrease with higher iodine doping content. The specific heat jump for the optimal composition CuIr2Te3.9I0.1 is approximately 1.46, which is close to the Bardeen Cooper Schrieffer value which is 1.43, indicating it is a bulk superconductor. The results of thermodynamic heat capacity measurements under different magnetic fields, magnetization and magneto-transport measurements further suggest that CuIr2Te4-xIx bulks are type II superconductors. Finally, an electronic phase diagram for this CuIr2Te4-xIx system has been constructed. The present study provides a suitable material platform for further investigation of the interplay of the CDW and superconductivity.
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