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Register a new userHeat transfer between two metals through subnanometric vacuum gaps
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We theoretically investigate the heat transfer between two metals across a vacuum gap in extreme near-field regime by quantifying the relative contribution of electrons, phonons and photons. We show that electrons play a dominant role in the heat transfer between two metals at subnanometric distance subject to a temperature gradient. Moreover, we demonstrate that this effect is dramatically amplified in the presence of an applied bias voltage. These results could pave the way to novel strategies for thermal management and energy conversion in extreme near-field regime.
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The non-contact heat transfer between two bodies is more efficient than the Stefan-Boltzmann law, when the distances are on the nanometer scale (shorter than Wiens wavelength), due to contributions of thermally excited near fields. This is usually described in terms of the fluctuation electrodynamics due to Rytov, Levin, and co-workers. Recent experiments in the tip-plane geometry have reported giant heat currents between metallic (gold) objects, exceeding even the expectations of Rytov theory. We discuss a simple model that describes the distance dependence of the data and permits to compare to a plate-plate geometry, as in the proximity (or Derjaguin) approximation. We extract an area density of active channels which is of the same order for the experiments performed by the groups of Kittel (Oldenburg) and Reddy (Ann Arbor). It is argued that mechanisms that couple phonons to an oscillating surface polarisation are likely to play a role.
In this work, we study the near-field heat transfer between composite nanostructures. It is demonstrated that thermally excited surface plasmon polaritons, surface phonon polaritons, and hyperbolic phonon polaritons in such composite nanostructures significantly enhance the near-field heat transfer. To further analyze the underlying mechanisms, we calculate energy transmission coefficients and obtain the near-field dispersion relations. The dispersion relations of composite nanostructures are substantially different from those of isolated graphene, silicon carbide (SiC) films, and SiC nanowire arrays due to the strong coupling effects among surface polaritonic modes. We identify four pairs of strongly coupled polaritonic modes with considerable Rabi frequencies in graphene/SiC film composite structures that greatly broaden the spectral peak. We confirm that near-field strong coupling effects between surface plasmon polaritons and hyperbolic phonon polaritons in the in-plane Reststrahlen band are different from those in the out-of-plane Reststrahlen band due to the different types of hyperbolicity. In addition, we analyze the effective tunability of the near-field heat transfer of graphene/SiC nanowire arrays composite structures by adjusting the chemical potential of graphene, the height and volume filling factor of the SiC nanowire arrays. This work provides a method to manipulate the near-field heat transfer with the use of strongly coupled surface polaritonic modes.
In this Rapid Communication, we theoretically demonstrate that near-field radiative heat transfer (NFRHT) can be modulated and enhanced by a new energy transmission mode of evanescent wave, i.e. the nonreciprocal surface plasmons polaritons (NSPPs). In addition to the well-known coupled surface plasmon polaritons (SPPs), applying a drift current on a graphene sheet leads to an extremely asymmetric photonic transmission model, which has never been noted in the noncontact heat exchanges at nanoscale before. The coupling of plasmons in the infrared bands dominates the NFRHT, associated with low loss (high loss and ultrahigh confinement) traveling along (against) the current. The dependence of NSPPs on the drift-current velocity as well as the vacuum gap is analyzed. It is found that the coupling of NSPPs at smaller and larger gap sizes exhibits different nonreciprocities. Finally, we also demonstrate that the prominent influence of the drift current on the radiative heat flux is found at a low chemical potential. These findings will open a new way to spectrally control NFRHT, which holds great potential for improving the performance of energy systems like near-field thermophotovoltaics and thermal modulator.
Recent experimental measurements for near-field radiative heat transfer between two bodies have been able to approach the gap distance within $2 ; textrm{nm}$, where the contributions of Coulomb fluctuation and electrons tunneling are comparable. Using the nonequilibrium Greens function method in the $G_{0}W_{0}$ approximation, based on a tight-binding model, we obtain for the energy current a Caroli formula from the Meir-Wingreen formula in the local equilibrium approximation. Also, the Caroli formula is consistent with the evanescent part of the heat transfer from the theory of fluctuational electrodynamics. We go beyond the local equilibrium approximation to study the energy transfer in the crossover region from electron tunneling to Coulomb fluctuation based on a numerical calculation.
We show that periodic multilayered structures allow to drastically enhance near-field radiative heat transfer between nanoparticles. In particular, when the two nanoparticles are placed on each side of the multilayered structure, at the same interparticle distance the resulting heat transfer is more than five orders of magnitude higher than that in the absence of the multilayered structure. This enhancement takes place in a broad range of distances and is due to the fact that the intermediate multilayered structure supports hyperbolic phonon polaritons with the key feature that the edge frequencies of the Type I and Type II Reststrahlen bands coincide with each other at a value extremely close to the particle resonance. This allow a very high-k evanescent modes resonating with the nanoparticles. Our predictions can be relevant for effective managing of energy at the nano-scale.
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