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Velocity selected production of $2^3S$ metastable positronium

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 Added by Ruggero Caravita Dr
 Publication date 2018
  fields Physics
and research's language is English




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Positronium in the $2^3S$ metastable state exhibits a low electrical polarizability and a long lifetime (1140 ns) making it a promising candidate for interferometry experiments with a neutral matter-antimatter system. In the present work, $2^3S$ positronium is produced - in absence of electric field - via spontaneous radiative decay from the $3^3P$ level populated with a 205nm UV laser pulse. Thanks to the short temporal length of the pulse, 1.5 ns full-width at half maximum, different velocity populations of a positronium cloud emitted from a nanochannelled positron/positronium converter were selected by delaying the excitation pulse with respect to the production instant. $ 2^3S $ positronium atoms with velocity tuned between $ 7 cdot 10^4 $ m/s and $ 10 cdot 10^4 $ m/s were thus produced. Depending on the selected velocity, a $2^3S$ production effciency ranging from $sim 0.8 %$ to $sim 1.7%$, with respect to the total amount of emitted positronium, was obtained. The observed results give a branching ratio for the $3^3P$-$2^3S$ spontaneous decay of $(9.7 pm 2.7) % $. The present velocity selection technique could allow to produce an almost monochromatic beam of $sim 1 cdot 10^3 $ $2^3S$ atoms with a velocity spread $ < 10^4 $ m/s and an angular divergence of $sim$ 50 mrad.



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We investigate experimentally the possibility of enhancing the production of $2^3S$ positronium atoms by driving the $1^3S$-$3^3P$ and $3^3P$-$2^3S$ transitions, overcoming the natural branching ratio limitation of spontaneous decay from $3^3P$ to $2^3S$. The decay of $3^3P$ positronium atoms towards the $2^3S$ level has been effciently stimulated by a 1312.2nm broadband IR laser pulse. The dependence of the stimulating transition efficiency on the intensity of the IR pulse has been measured to find the optimal enhancement conditions. A maximum relative increase of $ times (3.1 pm 1.0) $ in the $2^3S$ production efficiency, with respect to the case where only spontaneous decay is present, was obtained.
We characterized the pulsed Rydberg-positronium production inside the AEgIS (Antimatter Experiment: Gravity, Interferometry, Spectroscopy) apparatus in view of antihydrogen formation by means of a charge exchange reaction between cold antiprotons and slow Rydberg-positronium atoms. Velocity measurements on positronium along two axes in a cryogenic environment (10K) and in 1T magnetic field were performed. The velocimetry was done by MCP-imaging of photoionized positronium previously excited to the $n=3$ state. One direction of velocity was measured via Doppler-scan of this $n=3$-line, another direction perpendicular to the former by delaying the exciting laser pulses in a time-of-flight measurement. Self-ionization in the magnetic field due to motional Stark effect was also quantified by using the same MCP-imaging technique for Rydberg positronium with an effective principal quantum number $n_{eff}$ ranging between 14 and 22. We conclude with a discussion about the optimization of our experimental parameters for creating Rydberg-positronium in preparation for an efficient pulsed production of antihydrogen.
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The effect of confinement on the self-annihilation rate of positronium is studied in three levels of approximation. Artificial restriction of the electron-positron separation leads to an increase in the annihilation rate over its vacuum value; this increase is found to diminish exponentially as the maximum separation is increased. Confinement in a hard-wall spherical cavity with the center of mass free to move throughout the cavity also increases the annihilation rate over its vacuum value; the increase depends weakly on the position of the center of mass, being larger when the center of mass is near the cavity wall. Finally, to model confinement in a pore of a microporous material, the hard wall is replaced by physically motivated electron- and positron-wall potentials; it is found that the annihilation rate is larger than its vacuum value, in contradiction to calculations of Marlotti Tanzi et al. [Phys. Rev. Lett. 116, 033401 (2016)] that assumed hard-wall confinement for the electrons, and experimental data.
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