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Register a new userNuclear spin dynamics influenced and detected by electron spin polarization in CdTe/CdMgTe quantum wells
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Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday ellipticity, we generate and detect the coherent spin dynamics of the resident electrons. The photogenerated electron spin polarization is transferred into the nuclear spin system, which becomes polarized and acts back on the electron spins as the Overhauser field. Under the influence of resonant radio frequency pulses, we trace the coherent spin dynamics of the nuclear isotopes $^{111}$Cd, $^{113}$Cd, and $^{125}$Te. We measure nuclear Rabi oscillations, the inhomogeneous dephasing time $T_2^*$, the spin coherence time $T_2$, and the longitudinal relaxation time $T_1$. Furthermore, we investigate the influence of the laser excitation and the corresponding electron spin polarization on the nuclear spin relaxation time and find a weak extension of this time induced by interaction with the electron spins.
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We analyze thermally induced spin and charge transport in HgTe/CdTe quantum wells on the basis of the numerical non-equilibrium Greens function technique in the linear response regime. In the topologically non-trivial regime, we find a clear signature of the gap of the edge states due to their finite overlap from opposite sample boundaries -- both in the charge Seebeck and spin Nernst signal. We are able to fully understand the physical origin of the thermoelectric transport signatures of edge and bulk states based on simple analytical models. Interestingly, we derive that the spin Nernst signal is related to the spin Hall conductance by a Mott-like relation which is exact to all orders in the temperature difference between the warm and the cold reservoir.
We present a detailed analytical and numerical analysis of the nuclear spin dynamics in parabolic quantum wells. The shallow potential of parabolic quantum wells permits substantial modification of the electronic wave function in small electric fields. The nuclear spin relaxation via the hyperfine interaction depends on the electronic local density of states, therefore the local nuclear relaxation time depends sensitively on the electric field. For an inhomogeneous nuclear magnetization, such as generated by dynamic nuclear polarization, the total nuclear magnetization dynamics can similarly be altered. We examine this effect quantitatively and the effect of temperature, field, well thickness, and nuclear spin diffusion.
We study the spin dynamics in charged quantum dots in the situation where the resident electron is coupled to only about 200 nuclear spins and where the electron spin splitting induced by the Overhauser field does not exceed markedly the spectral broadening. The formation of a dynamical nuclear polarization as well as its subsequent decay by the dipole-dipole interaction is directly resolved in time. Because not limited by intrinsic nonlinearities, almost complete nuclear polarization is achieved, even at elevated temperatures. The data suggest a nonequilibrium mode of nuclear polarization, distinctly different from the spin temperature concept exploited on bulk semiconductors
Nuclear-spin diffusion in double quantum wells (QWs) is examined by using dynamic nuclear polarization (DNP) at a Landau level filling factor $ u=2/3$ spin phase transition (SPT). The longitudinal resistance increases during the DNP of one of the two QW (the polarization QW) by means of a large applied current and starts to decrease just after the termination of the DNP. On the other hand, the longitudinal resistance of the other QW (the detection QW) continuously increases for approximately 2h after the termination of the DNP of the polarization QW. It is therefore concluded that the nuclear spins diffuse from the polarization QW to the detection QW. The time evolution of the longitudinal resistance of the polarization QW is explained mainly by the nuclear-spin diffusion in the in-plane direction. In contrast, that of the detection QW manifests much slower nuclear diffusion in the perpendicular direction through the AlGaAs barrier.
We study the spin-dependent transmission through interfaces between a HgTe/CdTe quantum well (QW) and a metal - both for the normal metal and the superconducting case. Interestingly, we discover a new type of spin Hall effect at these interfaces that happens to exist even in the absence of structure and bulk inversion asymmetry within each subsystem (i.e. the QW and the metal). Thus, this is a pure boundary spin Hall effect which can be directly related to the existence of exponentially localized edge states at the interface. We demonstrate how this effect can be measured and functionalized for an all-electric spin injection into normal metal leads.
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