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Register a new userTopological strong field physics on sub-laser cycle time scale
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Added by
Alvaro Jimenez-Galan
Publication date
2018
fields
Physics
and research's language is
English
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Sub-laser cycle time scale of electronic response to strong laser fields enables attosecond dynamical imaging in atoms, molecules and solids. Optical tunneling and high harmonic generation are the hallmarks of attosecond imaging in optical domain, including imaging of phase transitions in solids. Topological phase transition yields a state of matter intimately linked with electron dynamics, as manifested via the chiral edge currents in topological insulators. Does topological state of matter leave its mark on optical tunneling and sub-cycle electronic response? We identify distinct topological effects on the directionality and the attosecond timing of currents arising during electron injection into conduction bands. We show that electrons tunnel across the band gap differently in trivial and topological phases, for the same band structure, and identify the key role of the Berry curvature in this process. These effects map onto topologically-dependent attosecond delays in high harmonic emission and the helicities of the emitted harmonics, which can record the phase diagram of the system and its topological invariants. Thus, the topological state of the system controls its attosecond, highly non-equilibrium electronic response to strong low-frequency laser fields, in bulk. Our findings create new roadmaps in studies of topological systems, building on ubiquitous properties of sub-laser cycle strong field response - a unique mark of attosecond science.
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A nonlinear interferometry scheme is described theoretically to induce and resolve electron wave- function beating on time scales shorter than the optical cycle of the time-delayed pump and probe pulses. By employing two moderately intense few-cycle laser fields with a stable carrier-envelope phase, a large range of the entire electronic level structure of a quantum system can be retrieved. In contrast to single-photon excitation schemes, the retrieved electronic states include levels that are both dipole- and non-dipole-accessible from the ground electronic state. The results show that strong-field interferometry can reveal both high-resolution and broad-band spectral information at the same time with important consequences for quantum-beat spectroscopy on attosecond or even shorter time scales.
We analyze the role of the difference between the central frequencies of the spectral distributions of the vector potential and the electric field of a short laser pulse. The frequency shift arises when the electric field is determined as the derivative of the vector potential to ensure that both quantities vanish at the beginning and end of the pulse. We derive an analytical estimate of the frequency shift and show how it affects various light induced processes, such as excitation, ionization and high harmonic generation. Since observables depend on the frequency spectrum of the electric field, the shift should be taken into account when setting the central frequency of the vector potential to avoid potential misinterpretation of numerical results for processes induced by few-cycle pulses.
When intense laser fields interact with nanoscale targets, strong-field physics meets plasmonic near-field enhancement and sub-wavelength localization of light. Photoemission spectra reflect the associated attosecond optical and electronic response and encode the collisional and collective dynamics of the solid. Nanospheres represent an ideal platform to explore the underlying attosecond nanophysics because of their particularly simple geometry. This review summarizes key results from the last decade and aims to provide the essential stepping stones for students and researchers to enter this field.
Sources of intense, ultra-short electromagnetic pulses enable applications such as attosecond pulse generation, control of electron motion in solids and the observation of reaction dynamics at the electronic level. For such applications both high-intensity and carrier envelope phase~(CEP) tunability are beneficial, yet hard to obtain with current methods. In this work we present a new scheme for generation of isolated CEP-tunable intense sub-cycle pulses with central frequencies that range from the midinfrared to the ultraviolet. It utilizes an intense laser pulse which drives a wake in a plasma, co-propagating with a long-wavelength seed pulse. The moving electron density spike of the wake amplifies the seed and forms a sub-cycle pulse. Controlling the CEP of the seed pulse, or the delay between driver and seed leads to CEP-tunability, while frequency tunability can be achieved by adjusting the laser and plasma parameters. Our 2D and 3D Particle-In-Cell simulations predict laser-to-sub-cycle-pulse conversion efficiencies up to 1%, resulting in relativistically intense sub-cycle pulses.
Topological lasers have been intensively investigated as a strong candidate for robust single-mode lasers. A typical topological laser employs a single-mode topological edge state, which appears deterministically in a designed topological bandgap and exhibits robustness to disorder. These properties seem to be highly attractive in pursuit of high power lasers capable of single mode operation. In this paper, we theoretically analyze a large-scale single-mode laser based on a topological edge state. We consider a sizable array laser consisting of a few hundreds of site resonators, which support a single topological edge mode broadly distributed among the resonators. We build a basic model describing the laser using the tight binding approximation and evaluate the stability of single mode lasing based on the threshold gain difference $Deltaalpha$ between the first-lasing edge mode and the second-lasing competing bulk mode. Our calculations demonstrate that stronger couplings between the cavities and lower losses are advantageous for achieving stable operation of the device. When assuming an average coupling of 100 cm$^{-1}$ between site resonators and other realistic parameters, the threshold gain difference $Deltaalpha$ can reach about 2 cm$^{-1}$, which would be sufficient for stable single mode lasing using a conventional semiconductor laser architecture. We also consider the effects of possible disorders and long-range interactions to assess the robustness of the laser under non-ideal situations. These results lay the groundwork for developing single-mode high-power topological lasers.
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