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Register a new userHeating causes non-linear microwave absorption anomaly in single wall carbon nanotubes
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Added by
Bence G\\'abor M\\'arkus
Publication date
2018
fields
Physics
and research's language is
English
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Microwave impedance measurements indicate a non-linear absorption anomaly in single wall carbon nanotubes at low temperatures (below $20$ K). We investigate the nature of the anomaly using a time resolved microwave impedance measurement technique. It proves that the anomaly has an extremely slow, a few hundred second long dynamics. This strongly suggests that the anomaly is not caused by an intrinsic electronic effect and that it is rather due to a slow heat exchange between the sample and the environment.
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Low field and high field transport properties of carbon nanotubes/polymer composites are investigated for different tube fractions. Above the percolation threshold f_c=0.33%, transport is due to hopping of localized charge carriers with a localization length xi=10-30 nm. Coulomb interactions associated with a soft gap Delta_CG=2.5 meV are present at low temperature close to f_c. We argue that it originates from the Coulomb charging energy effect which is partly screened by adjacent bundles. The high field conductivity is described within an electrical heating scheme. All the results suggest that using composites close to the percolation threshold may be a way to access intrinsic properties of the nanotubes by experiments at a macroscopic scale.
We present a simple technique which uses a self-aligned oxide etch to suspend individual single-wall carbon nanotubes between metallic electrodes. This enables one to compare the properties of a particular nanotube before and after suspension, as well as to study transport in suspended tubes. As an example of the utility of the technique, we study quantum dots in suspended tubes, finding that their capacitances are reduced owing to the removal of the dielectric substrate.
The dynamical conductance of electrically contacted single-walled carbon nanotubes is measured from dc to 10 GHz as a function of source-drain voltage in both the low-field and high-field limits. The ac conductance of the nanotube itself is found to be equal to the dc conductance over the frequency range studied for tubes in both the ballistic and diffusive limit. This clearly demonstrates that nanotubes can carry high-frequency currents at least as well as dc currents over a wide range of operating conditions. Although a detailed theoretical explanation is still lacking, we present a phenomenological model of the ac impedance of a carbon nanotube in the presence of scattering that is consistent with these results.
We compute the tunneling density of states of doped multi-wall nanotubes including disorder and electron-electron interactions. A non-conventional Coulomb blockade reflecting nonperturbative Altshuler-Aronov-Lee power-law zero-bias anomalies is found, in accordance with recent experimental results. The presence of a boundary implies a universal doubling of the boundary exponent in the diffusive limit.
The possibility of low-energy surface plasmon amplification by optically excited excitons in small-diameter single wall carbon nanotubes is theoretically demonstrated. The nonradiative exciton-plasmon energy transfer causes the buildup of the macroscopic population numbers of coherent localized surface plasmons associated with high-intensity coherent local fields formed at nanoscale throughout the nanotube surface. These strong local fields can be used in a variety of new optoelectronic applications of carbon nanotubes, including near-field nonlinear-optical probing and sensing, optical switching, enhanced electromagnetic absorption, and materials nanoscale modification.
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