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Register a new userUnscrambling Structured Chirality with Structured Light at Nanoscale Using Photo-induced Force
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We introduce a microscopy technique that facilitates the prediction of spatial features of chirality of nanoscale samples by exploiting photo-induced optical force exerted on an achiral tip in the vicinity of the test specimen. The tip-sample interactive system is illuminated by structured light to probe both the transverse and longitudinal (with respect to the beam propagation direction) components of the sample magnetoelectric polarizability as the manifestation of its sense of handedness, i.e., chirality. We specifically prove that although circularly polarized waves are adequate to detect the transverse polarizability components of the sample, they are unable to probe the longitudinal component. To overcome this inadequacy, we propose a judiciously engineered combination of radially and azimuthally polarized beams, as optical vortices possessing pure longitudinal electric and magnetic field components along their vortex axis, respectively, hence probing longitudinal chirality. The proposed technique may benefit branches of science like stereochemistry, biomedicine, physical and material science, and pharmaceutics
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Many nanophotonic applications require precise control and characterization of electromagnetic field properties at the nanoscale. The chiral properties of the field are among its key characteristics, yet measurement of optical chirality at dimensions beyond the diffraction limit has proven difficult. Here we theoretically show that the chiral properties of light can be characterized down to the nanometer scale by means of force detection. We demonstrate that the photo-induced force exerted on a sharp chiral tip, subjected to sequential illumination by two circularly polarized beams of opposite handedness, provides a useful probe of the chirality of the electromagnetic field. The gradient force difference $Deltalangle$textit{$F_{grad, z}$}$rangle$ is found to have exclusive correspondence to the time-averaged helicity density, whereas the differential scattering force provides information about the spin angular momentum density of light. We further characterize and quantify the helicity-dependent $Deltalangle$textit{$F_{grad, z}$}$rangle$ using a Mie scattering formalism complemented with full wave simulations, underlining that the magnitude of the difference force is within an experimentally detectable range.
Optical trapping describes the interaction between light and matter to manipulate micro-objects through momentum transfer. In the case of 3D trapping with a single beam, this is termed optical tweezers. Optical tweezers are a powerful and non-invasive tool for manipulating small objects, which have become indispensable in many fields, including physics, biology, soft condensed matter, amongst others. In the early days, optical trapping were typically used with a single Gaussian beam. In recent years, we have witnessed the rapid progress in the use of structured light beams with customized phase, amplitude and polarization in optical trapping. Unusual beam properties, such as phase singularities on-axis, propagation invariant nature, have opened up novel capabilities to the study of micromanipulation in liquid, air and vacuum. In this review, we summarize the recent advances in the field of optical trapping using structured light beams.
The structural versatility of light underpins an outstanding collection of optical phenomena where both geometrical and topological states of light can dictate how matter will respond or display. Light possesses multiple degrees of freedom such as amplitude, and linear, spin angular, and orbital angular momenta, but the ability to adaptively engineer the spatio-temporal distribution of all these characteristics is primarily curtailed by technologies used to impose any desired structure to light. We describe a foundational demonstration that examines a laser architecture offering integrated spatio-temporal field control and programmability, thereby presenting unique opportunities for generating light by design to exploit its topology.
Optical communication is an integral part of the modern economy, having all but replaced electronic communication systems. Future growth in bandwidth appears to be on the horizon using structured light, encoding information into the spatial modes of light, and transmitting them down fibre and free-space, the latter crucial for addressing last mile and digitally disconnected communities. Unfortunately, patterns of light are easily distorted, and in the case of free-space optical communication, turbulence is a significant barrier. Here we review recent progress in structured light in turbulence, first with a tutorial style summary of the core concepts, before highlighting the present state-of-the-art in the field. We support our review with new experimental studies that reveal which types of structured light are best in turbulence, the behaviour of vector versus scalar light in turbulence, the trade-off of diversity and multiplexing, and how turbulence models can be exploited for enhanced optical signal processing protocols. This comprehensive treatise will be invaluable to the large communities interested in free-space optical communication with spatial modes of light.
We demonstrate the coherent frequency conversion of structured light, optical beams in which the phase varies in each point of the transverse plane, from the near infrared (803nm) to the visible (527nm). The frequency conversion process makes use of sum-frequency generation in a periodically poled lithium niobate (ppLN) crystal with the help of a 1540-nm Gaussian pump beam. We perform far-field intensity measurements of the frequency-converted field, and verify the sought-after transformation of the characteristic intensity and phase profiles for various input modes. The coherence of the frequency-conversion process is confirmed using a mode-projection technique with a phase mask and a single-mode fiber. The presented results could be of great relevance to novel applications in high-resolution microscopy and quantum information processing.
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