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Register a new userCross section measurements of $^{155,157}$Gd(n,$gamma$) induced by thermal and epithermal neutrons
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Neutron capture measurements on $^{155}$Gd and $^{157}$Gd were performed using the time-of-flight technique at the n_TOF facility at CERN. Four samples in form of self-sustaining metallic discs isotopically enriched in $^{155}$Gd and $^{157}$Gd were used. The measurements were carried out at the experimental area (EAR1) at 185 m from the neutron source, with an array of 4 C$_6$D$_6$ liquid scintillation detectors. The capture cross sections of $^{155}$Gd and $^{157}$Gd at neutron kinetic energy of 0.0253 eV have been estimated to be 62.2(2.2) kb and 239.8(9.3) kb, respectively, thus up to 6% different relative to the ones reported in the nuclear data libraries. A resonance shape analysis has been performed in the resolved resonance region up to 180 eV and 300 eV, respectively, in average resonance parameters have been found in good agreement with evaluations. Above these energies the observed resonance-like structures in the cross section have been tentatively characterised in terms of resonance energy and area up to 1 keV.
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In order to measure the total cross section for thermal neutrons, a photoneutron source (PNS, phase 1) has been developed for the acquisition of nuclear data for the Thorium Molten Salt Reactor (TMSR) at the Shanghai Institute of Applied Physics (SINAP). PNS is an electron LINAC pulsed neutron facility that uses the time-of-flight (TOF) technique. It records the neutron TOF and identifies neutrons and $gamma$-rays by using a digital signal processing technique. The background is obtained by using a combination of employing 12.8 cm boron-loaded polyethylene(PEB) (5$%$ w.t.) to block the flight path and Monte Carlo methods. The neutron total cross sections of natural beryllium are measured in the neutron energy region from 0.007 to 0.1 eV. The present measurement result is compared with the fold Harvey data with the response function of PNS.
The total cross sections for the $^{152}$Gd(p,$gamma$)$^{153}$Tb and $^{152}$Gd(p,n)$^{152}$Tb reactions have been measured by the activation method at effective center-of-mass energies mbox{$3.47 leq E_mathrm{c.m.}^mathrm{eff}leq 7.94$ MeV} and mbox{$4.96 leq E_mathrm{c.m.}^mathrm{eff} leq 7.94$ MeV}, respectively. The targets were prepared by evaporation of 30.6% isotopically enriched $^{152}$Gd oxide on aluminum backing foils, and bombarded with proton beams provided by a cyclotron accelerator. The cross sections were deduced from the observed $gamma$-ray activity, which was detected off-line by a HPGe detector in a low background environment. The results are presented and compared with predictions of statistical model calculations. This comparison supports a modified optical proton+$^{152}$Gd potential suggested earlier.
The cross section of the $^{23}$Na($n, gamma$)$^{24}$Na reaction has been measured via the activation method at the Karlsruhe 3.7 MV Van de Graaff accelerator. NaCl samples were exposed to quasistellar neutron spectra at $kT=5.1$ and 25 keV produced via the $^{18}$O($p, n$)$^{18}$F and $^{7}$Li($p, n$)$^{7}$Be reactions, respectively. The derived capture cross sections $langlesigmarangle_{rm kT=5 keV}=9.1pm0.3$ mb and $langlesigmarangle_{rm kT=25 keV}=2.03 pm 0.05$ mb are significantly lower than reported in literature. These results were used to substantially revise the radiative width of the first $^{23}$Na resonance and to establish an improved set of Maxwellian average cross sections. The implications of the lower capture cross section for current models of $s$-process nucleosynthesis are discussed.
The 62Ni(n,gamma)63Ni(t_1/2=100+-2 yrs) reaction plays an important role in the control of the flow path of the slow neutron-capture (s-) nucleosynthesis process. We have measured for the first time the total cross section of this reaction for a quasi-Maxwellian (kT = 25 keV) neutron flux. The measurement was performed by fast-neutron activation, combined with accelerator mass spectrometry to detect directly the 63Ni product nuclei. The experimental value of 28.4+-2.8 mb, fairly consistent with a recent theoretical estimate, affects the calculated net yield of 62Ni itself and the whole distribution of nuclei with 62<A <90 produced by the weak s-process in massive stars.
The cross sections of the 162Er(a,g,)166Yb and 162Er(a,n)165Yb reactions have been measured for the first time. The radiative alpha capture reaction cross section was measured from Ec.m. = 16.09 down to Ec.m. = 11.21 MeV, close to the astrophysically relevant region (which lies between 7.8 and 11.48 MeV at 3 GK stellar temperature). The 162Er(a,n)165Yb reaction was studied above the reaction threshold between Ec.m. = 12.19 and 16.09 MeV. The fact that the 162Er(a,g)166Yb cross sections were measured below the (a,n) threshold at first time in this mass region opens the opportunity to study directly the a-widths required for the determination of astrophysical reaction rates. The data clearly show that compound nucleus formation in this reaction proceeds differently than previously predicted.
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