No Arabic abstract
Nuclear level densities and $gamma$-ray strength functions have been extracted for $^{59, 60}rm{Ni}$, using the Oslo method on data sets from the $^{60}$Ni($^{3}$He,$^{3}$He$^{prime}gamma$)$^{60}$Ni and $^{60}$Ni($^{3}$He,$alphagamma$)$^{59}$Ni reactions. Above the neutron separation energy, S$_n$, we have measured the $gamma$-ray strength functions for $^{61}$Ni and $^{60}$Ni in photoneutron experiments. The low-energy part of the $^{59,60}$Ni $gamma$-ray strength functions show an increase for decreasing $gamma$ energies. The experimental $gamma$-ray strength functions are compared with $M1$ $gamma$-ray strength functions calculated within the shell model. The $E1$ $gamma$-ray strength function of $^{60}$Ni has been calculated using the QTBA framework. The QTBA calculations describe the data above $E_{gamma}approx$ 7 MeV, while the shell-model calculations agree qualitatively with the low energy part of the $gamma$-ray strength function. Hence, we give a plausible explanation of the observed shape of the $gamma$-decay strength.
Neutron-capture reactions on very neutron-rich nuclei are essential for heavy-element nucleosynthesis through the rapid neutron-capture process, now shown to take place in neutron-star merger events. For these exotic nuclei, radiative neutron capture is extremely sensitive to their $gamma$-emission probability at very low $gamma$ energies. In this work, we present measurements of the $gamma$-decay strength of $^{70}$Ni over the wide range $1.3 leq E_{gamma} leq 8 $ MeV. A significant enhancement is found in the $gamma$-decay strength for transitions with $E_gamma < 3$ MeV. At present, this is the most neutron-rich nucleus displaying this feature, proving that this phenomenon is not restricted to stable nuclei. We have performed $E1$-strength calculations within the quasiparticle time-blocking approximation, which describe our data above $E_gamma simeq 5$ MeV very well. Moreover, large-scale shell-model calculations indicate an $M1$ nature of the low-energy $gamma$ strength. This turns out to be remarkably robust with respect to the choice of interaction, truncation and model space, and we predict its presence in the whole isotopic chain, in particular the neutron-rich $^{72,74,76}mathrm{Ni}$.
The $E0$ transition strength in the $2^+_2 rightarrow 2^+_1$ transitions of $^{58,60,62}$Ni have been determined for the first time following a series of measurements at the Australian National University (ANU) and the University of Kentucky (UK). The CAESAR Compton-suppressed HPGe array and the Super-e solenoid at ANU were used to measure the $delta(E2/M1)$ mixing ratio and internal conversion coefficient of each transition following inelastic proton scattering. Level half-lives, $delta(E2/M1)$ mixing ratios and $gamma$-ray branching ratios were measured at UK following inelastic neutron scattering. The new spectroscopic information was used to determine the $E0$ strengths. These are the first $2^+ rightarrow 2^+$ $E0$ transition strengths measured in nuclei with spherical ground states and the $E0$ component is found to be unexpectedly large; in fact, these are amongst the largest $E0$ transition strengths in medium and heavy nuclei reported to date.
Excited states in $^{58,60,62}$Ni were populated via inelastic proton scattering at the Australian National University as well as via inelastic neutron scattering at the University of Kentucky Accelerator Laboratory. The Super-e electron spectrometer and the CAESAR Compton-suppressed HPGe array were used in complementary experiments to measure conversion coefficients and $delta(E2/M1)$ mixing ratios, respectively, for a number of $2^+ rightarrow 2^+$ transitions. The data obtained were combined with lifetimes and branching ratios to determine $E0$, $M1$, and $E2$ transition strengths between $2^+$ states. The $E0$ transition strengths between $0^+$ states were measured using internal conversion electron spectroscopy and compare well to previous results from internal pair formation spectroscopy. The $E0$ transition strengths between the lowest-lying $2^+$ states were found to be consistently large for the isotopes studied.
The results of the study of gamma-transition description in fast neutron capture and photofission are presented. Recent experimental data were used, namely, the spectrum of prompt gamma-rays in the energy range 2{div}18 MeV from 14-MeV neutron capture in natural Ni and isomeric ratios in primary fragments of photofission of the isotopes of U, Np and Pu by bremsstrahlung with end-point energies $E_e$= 10.5, 12 and 18 MeV. The data are compared with the theoretical calculations performed within EMPIRE 3.2 and TALYS 1.6 codes. The mean value of angular momenta and their distributions were determined in the primary fragments $^{84}$Br, $^{97}$Nb, $^{90}$Rb, $^{131,133}$Te, $^{132}$Sb, $^{132,134}$I, $^{135}$Xe of photofissions. An impact of the characteristics of nuclear excited states on the calculation results is studied using different models for photon strength function and nuclear level density.
The $^{58}$Ni$(n,gamma)^{59}$Ni cross section was measured with a combination of the activation technique and accelerator mass spectrometry (AMS). The neutron activations were performed at the Karlsruhe 3.7 MV Van de Graaff accelerator using the quasi-stellar neutron spectrum at $kT=25$ keV produced by the $^7$Li($p,n$)$^7$Be reaction. The subsequent AMS measurements were carried out at the 14 MV tandem accelerator of the Maier-Leibnitz-Laboratory in Garching using the Gas-filled Analyzing Magnet System (GAMS). Three individual samples were measured, yielding a Maxwellian-averaged cross section at $kT=30$ keV of $langlesigmarangle_{30text{keV}}$= 30.4 (23)$^{syst}$(9)$^{stat}$ mbarn. This value is slightly lower than two recently published measurements using the time-of-flight (TOF) method, but agrees within the uncertainties. Our new results also resolve the large discrepancy between older TOF measurements and our previous value.