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The increasing need to store large amounts of information with an ultra-dense, reliable, low power and low cost memory device is driving aggressive efforts to improve upon current perpendicular magnetic recording technology. However, the difficulties in fabricating small grain recording media while maintaining thermal stability and a high signal-to-noise ratio motivate development of alternative methods, such as the patterning of magnetic nano-islands and utilizing energy-assist for future applications. In addition, both from sensor and memory perspective three-dimensional spintronic devices are highly desirable to overcome the restrictions on the functionality in the planar structures. Here we demonstrate a three-dimensional magnetic-memory (magnetic page memory) based on thermally assisted and stray-field induced transfer of domains in a vertical stack of magnetic nanowires with perpendicular anisotropy. Using spin-torque induced domain shifting in such a device with periodic pinning sites provides additional degrees of freedom by allowing lateral information flow to realize truly three-dimensional integration.
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Recent progress in nanofabrication and additive manufacturing have facilitated the building of nanometer-scale three-dimensional structures, that promise to lead to an emergence of new functionalities within a number of fields, compared to state-of-the-art two dimensional systems. In magnetism, the move to three-dimensional systems offers the possibility for novel magnetic properties not available in planar systems, as well as enhanced performance, both of which are key for the development of new technological applications. In this review paper we will focus our attention on three-dimensional magnetic systems and how their magnetic configuration can be retrieved using X-ray magnetic nanotomography.
Cylindrical magnetic nanowires with large transversal magnetocrystalline anisotropy have been shown to sustain non-trivial magnetic configurations resulting from the interplay of spatial confinement, exchange, and anisotropies. Exploiting these peculiar 3D spin configurations and their solitonic inhomogeneities are prospected to improve magnetization switching in future spintronics, such as power-saving magnetic memory and logic applications. Here we employ holographic vector field electron tomography to reconstruct the remanent magnetic states in CoNi nanowires with 10 nm resolution in 3D, with a particular focus on domain walls between remanent states and ubiquitous real-structure effects stemming from irregular morphology and anisotropy variations. By tuning the applied magnetic field direction, both longitudinal and transverse multi-vortex states of different chiralities and peculiar 3D features such as shifted vortex cores are stabilized. The chiral domain wall between the longitudinal vortices of opposite chiralities exhibits a complex 3D shape characterized by a push out of the central vortex line and a gain in exchange and anisotropy energy. A similar complex 3D texture, including bent vortex lines, forms at the domain boundary between transverse-vortex states and longitudinal configurations. Micromagnetic simulations allow an understanding of the origin of the observed complex magnetic states.
Magnetic hopfion is three-dimensional (3D) topological soliton with novel spin structure that would enable exotic dynamics. Here we study the current driven 3D dynamics of a magnetic hopfion with unit Hopf index in a frustrated magnet. Attributed to spin Berry phase and symmetry of the hopfion, the phase space entangles multiple collective coordinates, thus the hopfion exhibits rich dynamics including longitudinal motion along the current direction, transverse motion perpendicular to the current direction, rotational motion and dilation. Furthermore, the characteristics of hopfion dynamics is determined by the ratio between the non-adiabatic spin transfer torque parameter and the damping parameter. Such peculiar 3D dynamics of magnetic hopfion could shed light on understanding the universal physics of hopfions in different systems and boost the prosperous development of 3D spintronics.
Recent acoustic and electrical-circuit experiments have reported the third-order (or octupole) topological insulating phase, while its counterpart in classical magnetic systems is yet to be realized. Here we explore the collective dynamics of magnetic vortices in three-dimensional breathing cuboids, and find that the vortex lattice can support zero-dimensional corner states, one-dimensional hinge states, two-dimensional surface states, and three-dimensional bulk states, when the ratio of alternating intralayer and interlayer bond lengths goes beyond a critical value. We show that only the corner states are stable against external frustrations because of the topological protection. Full micromagnetic simulations verify our theoretical predictions with good agreement.
Magnetic resonance imaging (MRI) has revolutionized biomedical science by providing non-invasive, three-dimensional biological imaging. However, spatial resolution in conventional MRI systems is limited to tens of microns, which is insufficient for imaging on molecular and atomic scales. Here we demonstrate an MRI technique that provides sub-nanometer spatial resolution in three dimensions, with single electron-spin sensitivity. Our imaging method works under ambient conditions and can measure ubiquitous dark spins, which constitute nearly all spin targets of interest and cannot otherwise be individually detected. In this technique, the magnetic quantum-projection noise of dark spins is measured using a single nitrogen-vacancy (NV) magnetometer located near the surface of a diamond chip. The spatial distribution of spins surrounding the NV magnetometer is imaged with a scanning magnetic-field gradient. To evaluate the performance of the NV-MRI technique, we image the three-dimensional landscape of dark electronic spins at and just below the diamond surface and achieve an unprecedented combination of resolution (0.8 nm laterally and 1.5 nm vertically) and single-spin sensitivity. Our measurements uncover previously unidentified electronic spins on the diamond surface, which can potentially be used as resources for improved magnetic imaging of samples proximal to the NV-diamond sensor. This three-dimensional NV-MRI technique is immediately applicable to diverse systems including imaging spin chains, readout of individual spin-based quantum bits, and determining the precise location of spin labels in biological systems.
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