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Register a new userResonating valence bonds and spinon pairing in the Dicke model
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Added by
Ramachandran Ganesh
Publication date
2018
fields
Physics
and research's language is
English
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Resonating valence bond (RVB) states are a class of entangled quantum many body wavefunctions with great significance in condensed matter physics. We propose a scheme to synthesize a family of RVB states using a cavity QED setup with two-level atoms (with states $vert 0 rangle$ and $vert 1 rangle$) coupled to a common photon mode. In the lossy cavity limit, starting with an initial state of $M$ atoms excited and $N$ atoms in the ground state, we show that this setup can be configured as a Stern Gerlach experiment. A measurement of photon emission collapses the wavefunction of atoms onto an RVB state composed of resonating long-ranged singlets of the form $frac{1}{sqrt{2}}[vert 0 1 rangle - vert 1 0 rangle]$. Each emitted photon reduces the number of singlets by unity, replacing it with a pair of lone spins or `spinons. As spinons are formed coherently in pairs, they are analogous to Cooper pairs in a superconductor. To simulate pair fluctuations, we propose a protocol in which photons are allowed to escape the cavity undetected. This leads to a mixed quantum state with a fluctuating number of spinon pairs -- an inchoate superconductor. Remarkably, in the limit of large system sizes, this protocol reveals an underlying quantum phase transition. Upon tuning the initial spin polarization ($M-N$), the emission exhibits a continuous transition from a dark state to a bright state. This is reflected in the spinon pair number distribution which can be tuned from sub-poissonian to super-poissonian regimes. This opens an exciting route to simulate RVB states and superconductivity.
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Dickes original thought experiment with two spins coupled to a photon mode has recently been experimentally realized. We propose extending this experiment to N spins and show that it naturally gives rise to highly entangled states. In particular, it gives rise to dark states which have resonating valence bond (RVB) character. We first consider a system of N two level spins in a cavity with only one spin in the excited state. This initial state is a linear combination of a dark state and a bright state. We point out the dark state is a coherent superposition of singlets with resonating valence bond character. We show that the coupling to the photon mode takes the spin system into a mixed state with an entangled density matrix. We next consider an initial state with half of the spins in the excited state. We show that there is a non-zero probability for this to collapse into a dark state with RVB character. In the lossy cavity limit, if no photon is detected within several decay time periods, we may deduce that the spin system has collapsed onto the dark RVB state. We show that the probability for this scales as 2/N, making it possible to generate RVB states of 20 spins or more.
Since its proposal by Anderson, resonating valence bonds (RVB) formed by a superposition of fluctuating singlet pairs have been a paradigmatic concept in understanding quantum spin liquids (QSL). Here, we show that excitations related to singlet breaking on nearest-neighbor bonds describe the high-energy part of the excitation spectrum in YbMgGaO4, the effective spin-1/2 frustrated antiferromagnet on the triangular lattice, as originally considered by Anderson. By a thorough single-crystal inelastic neutron scattering (INS) study, we demonstrate that nearest-neighbor RVB excitations account for the bulk of the spectral weight above 0.5 meV. This renders YbMgGaO4 the first experimental system where putative RVB correlations restricted to nearest neighbors are observed, and poses a fundamental question of how complex interactions on the triangular lattice conspire to form this unique many-body state.
The Kagome Heisenberg antiferromagnet is mapped onto an effective Hamiltonian on the star superlattice by Contractor Renormalization. Comparison of ground state energies on large lattices to Density Matrix Renormalization Group justifies truncation of effective interactions at range 3. Within our accuracy, magnetic and translational symmetries are not broken (i.e. a spin liquid ground state). However, we discover doublet spectral degeneracies which signal the onset of p6 - chirality symmetry breaking. This is understood by simple mean field analysis. Experimentally, the p6 chiral order parameter should split the optical phonons degeneracy near the zone center. Addition of weak next to nearest neighbor coupling is discussed.
We apply a variational wave function capable of describing qualitatively and quantitatively the so called resonating valence bond in realistic materials, by improving standard ab initio calculations by means of quantum Monte Carlo methods. In this framework we clearly identify the Kekule and Dewar contributions to the chemical bond of the benzene molecule, and we establish the corresponding resonating valence bond energy of these well known structures ($simeq 0.01$eV/atom). We apply this method to unveil the nature of the chemical bond in undoped graphene and show that this picture remains only within a small resonance length of few atomic units.
A central idea in strongly correlated systems is that doping a Mott insulator leads to a superconductor by transforming the resonating valence bonds (RVBs) into spin-singlet Cooper pairs. Here, we argue that a spin-triplet RVB (tRVB) state, driven by spatially, or orbitally anisotropic ferromagnetic interactions can provide the parent state for triplet superconductivity. We apply this idea to the iron-based superconductors, arguing that strong onsite Hunds interactions develop intra-atomic tRVBs between the t$_{2g}$ orbitals. On doping, the presence of two iron atoms per unit cell allows these inter-orbital triplets to coherently delocalize onto the Fermi surface, forming a fully gapped triplet superconductor. This mechanism gives rise to a unique staggered structure of onsite pair correlations, detectable as an alternating $pi$ phase shift in a scanning tunnelling Josephson microscope.
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