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Register a new userThe Triplet Resonating Valence Bond State and Superconductivity in Hunds Metals
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A central idea in strongly correlated systems is that doping a Mott insulator leads to a superconductor by transforming the resonating valence bonds (RVBs) into spin-singlet Cooper pairs. Here, we argue that a spin-triplet RVB (tRVB) state, driven by spatially, or orbitally anisotropic ferromagnetic interactions can provide the parent state for triplet superconductivity. We apply this idea to the iron-based superconductors, arguing that strong onsite Hunds interactions develop intra-atomic tRVBs between the t$_{2g}$ orbitals. On doping, the presence of two iron atoms per unit cell allows these inter-orbital triplets to coherently delocalize onto the Fermi surface, forming a fully gapped triplet superconductor. This mechanism gives rise to a unique staggered structure of onsite pair correlations, detectable as an alternating $pi$ phase shift in a scanning tunnelling Josephson microscope.
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We apply a variational wave function capable of describing qualitatively and quantitatively the so called resonating valence bond in realistic materials, by improving standard ab initio calculations by means of quantum Monte Carlo methods. In this framework we clearly identify the Kekule and Dewar contributions to the chemical bond of the benzene molecule, and we establish the corresponding resonating valence bond energy of these well known structures ($simeq 0.01$eV/atom). We apply this method to unveil the nature of the chemical bond in undoped graphene and show that this picture remains only within a small resonance length of few atomic units.
We have performed Diffusion Quantum Monte Carlo simulations of Li clusters showing that Resonating-Valence-Bond (RVB) pairing correlations between electrons provide a substantial contribution to the cohesive energy. The RVB effects are identified in terms of electron transfers from s- to p-like character, constituting a possible explanation for the breakdown of the Fermi liquid picture observed in recent high resolution Compton scattering experiments for bulk Li.
The trimer resonating valence bond (tRVB) state consisting of an equal-weight superposition of trimer coverings on a square lattice is proposed. A model Hamiltonian of the Rokhsar-Kivelson type for which the tRVB becomes the exact ground state is written. The state is shown to have $9^g$ topological degeneracy on genus g surface and support $Z_3$ vortex excitations. Correlation functions show exponential behavior with a very short correlation length consistent with the gapped spectrum. The classical problem of the degeneracy of trimer configurations is investigated by the transfer matrix method.
Resonating valence bond (RVB) theory of high Tc superconductivity, an electron correlation based mechanism, began as an insightful response by Anderson, to Bednorz and Mullers discovery of high Tc superconductivity in cuprates in late 1986. Shortly a theoretical framework for quantum spin liquids and superconductivity was developed. This theory adresses a formidable strong coupling quantum manybody problem, in modern times. It is built on certain key experimental facts: i) survival of a dynamical Mott localization in a metallic state, ii) proliferation of bond singlets and iii) absence of fermi liquid quasi particles. After summarising RVB theory I will provide an aerial view of, mostly, new superconductors where I believe that, to a large degree RVB mechanism is at work and indicate prospects for even higher Tcs.
Dickes original thought experiment with two spins coupled to a photon mode has recently been experimentally realized. We propose extending this experiment to N spins and show that it naturally gives rise to highly entangled states. In particular, it gives rise to dark states which have resonating valence bond (RVB) character. We first consider a system of N two level spins in a cavity with only one spin in the excited state. This initial state is a linear combination of a dark state and a bright state. We point out the dark state is a coherent superposition of singlets with resonating valence bond character. We show that the coupling to the photon mode takes the spin system into a mixed state with an entangled density matrix. We next consider an initial state with half of the spins in the excited state. We show that there is a non-zero probability for this to collapse into a dark state with RVB character. In the lossy cavity limit, if no photon is detected within several decay time periods, we may deduce that the spin system has collapsed onto the dark RVB state. We show that the probability for this scales as 2/N, making it possible to generate RVB states of 20 spins or more.
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