No Arabic abstract
We report results of a muon spin relaxation ($mu$SR) study of YFe$_2$Al$_{10}$, a quasi-2D nearly-ferromagnetic metal in which unconventional quantum critical behavior is observed. No static Fe$^{2+}$ magnetism, with or without long-range order, is found down to 19~mK@. The dynamic muon spin relaxation rate~$lambda$ exhibits power-law divergences in temperature and magnetic field, the latter for fields that are too weak to affect the electronic spin dynamics directly. We attribute this to the proportionality of $lambda(omega_mu,T)$ to the dynamic structure factor~$S(omega_mu,T)$, where $omega_mu approx 10^5$--$10^7~mathrm{s}^{-1}$ is the muon Zeeman frequency. These results suggest critical divergences of $S(omega_mu,T)$ in both temperature and frequency. Power-law scaling and a 2D dissipative quantum XY (2D-DQXY) model both yield forms for $S(omega,T)$ that agree with neutron scattering data ($omega approx 10^{12}~mathrm{s}^{-1}$). Extrapolation to $mu$SR frequencies agrees semi-quantitatively with the observed temperature dependence of $lambda(omega_mu,T)$, but predicts frequency independence for $omega_mu ll T$ in extreme disagreement with experiment. We conclude that the quantum critical spin dynamics of YFe$_2$Al$_{10}$ are not well understood at low frequencies.
By means of nuclear spin-lattice relaxation rate 1/T1, we follow the spin dynamics as a function of the applied magnetic field in two gapped one-dimensional quantum antiferromagnets: the anisotropic spin-chain system NiCl2-4SC(NH2)2 and the spin-ladder system (C5H12N)2CuBr4. In both systems, spin excitations are confirmed to evolve from magnons in the gapped state to spinons in the gapples Tomonaga-Luttinger-liquid state. In between, 1/T1 exhibits a pronounced, continuous variation, which is shown to scale in accordance with quantum criticality. We extract the critical exponent for 1/T1, compare it to the theory, and show that this behavior is identical in both studied systems, thus demonstrating the universality of quantum critical behavior.
We report magnetization, specific heat, and NMR investigations on YFe2Al10 over a wide range in temperature and magnetic field and zero field (NQR) measurements. Magnetic susceptibility, specific heat and spin-lattice relaxation rate divided by T (1/T1T) follow a weak power law (T^-0.4) temperature dependence, which is a signature of critical fluctuations of Fe moments. The value of the Sommerfeld-Wilson ratio and linear relation between 1/T1T and chi(T) suggest the existence of ferromagnetic correlations in this system. No magnetic ordering down to 50 mK in Cp(T) and the unusual temperature and field scaling of the bulk and NMR data are associated with a magnetic instability which drives the system to quantum criticality. The magnetic properties of the system are tuned by field wherein ferromagnetic fluctuations are suppressed and a crossover from quantum critical to FL behavior is observed with increasing magnetic field.
We demonstrate that quantum-critical spin dynamics can be probed in high magnetic fields using muon-spin relaxation ($mu^{+}$SR). Our model system is the strong-leg spin ladder bis(2,3-dimethylpyridinium) tetrabromocuprate (DIMPY). In the gapless Tomonaga-Luttinger liquid phase we observe finite-temperature scaling of the $mu^{+}$SR $1/T_1$ relaxation rate which allows us to determine the Luttinger parameter $K$. We discuss the benefits and limitations of local probes compared with inelastic neutron scattering.
We study the Neel-paramagnetic quantum phase transition in two-dimensional dimerized $S=1/2$ Heisenberg antiferromagnets using finite-size scaling of quantum Monte Carlo data. We resolve the long standing issue of the role of cubic interactions arising in the bond-operator representation when the dimer pattern lacks a certain symmetry. We find non-monotonic (monotonic) size dependence in the staggered (columnar) dimerized model, where cubic interactions are (are not) present. We conclude that there is an irrelevant field in the staggered model that is not present in the columnar case, but, at variance with previous claims, it is not the leading irrelevant field. The new exponent is $omega_2 approx 1.25$ and the prefactor of the correction $L^{-omega_2}$ is large and comes with a different sign from that of the formally leading conventional correction with exponent $omega_1 approx 0.78$. Our study highlights the possibility of competing scaling corrections at quantum critical points.
When the quantum critical transverse-field Ising chain is perturbed by a longitudinal field, a quantum integrable model emerges in the scaling limit with massive excitations described by the exceptional $E_{8}$ Lie algebra. Using the corresponding analytical form factors of the quantum $E_{8}$ integrable model, we systematically study the spin dynamic structure factor of the perturbed quantum critical Ising chain, where particle channels with total energy up to 5$m_1$ ($m_1$ being the mass of the lightest $E_{8}$ particle) are exhausted. In addition to the significant single-particle contributions to the dynamic spectrum, each two-particle channel with different masses is found to exhibit an edge singularity at the threshold of the total mass and decays with an inverse square root of energy, which is attributed to the singularity of the two-particle density of states at the threshold. The singularity is absent for particles with equal masses due to a cancellation mechanism involving the structure of the form factors. As a consequence, the dynamic structure factor displays a cascade of bumping peaks in the continuum region with clear singular features which can serve as a solid guidance for the material realization of the quantum $E_{8}$ model.