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A Zeeman slower for diatomic molecules

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 Added by Mirco Siercke Ph.D.
 Publication date 2017
  fields Physics
and research's language is English




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We present a novel slowing scheme for beams of laser-coolable diatomic molecules reminiscent of Zeeman slowing of atomic beams. The scheme results in efficient compression of the 1-dimensional velocity distribution to velocities trappable by magnetic or magneto-optical traps. 3D Monte Carlo simulations for the prototype molecule $^{88}mathrm{Sr}^{19}mathrm{F}$ and experiments in an atomic testbed demonstrate a performance comparable to traditional atomic Zeeman slowing and an enhancement of flux below v=35 m/s by a factor of $approx 20$ compared to white-light slowing. This is the first experimentally shown continuous and dissipative slowing technique in molecule-like level structures, promising to provide the missing link for the preparation of large ultracold molecular ensembles.



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We present a thorough analysis of a Zeeman slower for sodium atoms made of permanent magnets in a Halbach configuration. Due to the orientation of the magnetic field, the polarisation of the slowing laser beam cannot be purely circular leading to optical leakages into dark states. To circumvent this effect, we propose an atomic state preparation stage able to significantly increase the performances of the Zeeman slower. After a careful theoretical analysis of the problem, we experimentally implement an optical pumping stage leading to an increase of the magneto-optical trap loading rate by 3.5. Such method is easy to set up and could be extended to other Zeeman slower architectures.
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