A valley degree of freedom (DOF) in transition metal dichalcogenides with broken inversion symmetry can be controlled through spin and orbital DOFs owing to their valley-contrasting characters. Another important aspect of the spin and orbital DOFs is that they affect quasiparticle scattering processes that govern the valley lifetime. Here we combine quasiparticle-interference (QPI) imaging experiments and theoretical simulations to study the roles of the spin and orbital DOFs in 3R-NbS2. We find that the QPI signal arising from an inter-valley scattering is noticeably weaker than that caused by an intra-valley scattering. We show that this behavior is predominantly associated with the orbital DOF, signifying the different spin and orbital structures of spin-split bands at each valley. These findings provide important insights into understanding the valley-related transport properties.
Using both two orbital and five orbital models, we investigate the quasiparticle interference (QPI) patterns in the superconducting (SC) state of iron-based superconductors. We compare the results for nonmagnetic and magnetic impurities in sign-changed s-wave $cos(k_x)cdotcos(k_y)$ and sign-unchanged $|cos(k_x)cdotcos(k_y)|$ SC states. While the patterns strongly depend on the chosen band structures, the sensitivity of peaks around $(pmpi,0)$ and $(0,pmpi)$ wavevectors on magnetic or non-magnetic impurity, and sign change or sign unchanged SC orders is common in two models. Our results strongly suggest that QPI may provide direct information of band structures and evidence of the pairing symmetry in the SC states.
In the presence of spin-orbit coupling, electron scattering off impurities depends on both spin and orbital angular momentum of electrons -- spin-orbit scattering. Although some transport properties are subject to spin-orbit scattering, experimental techniques directly accessible to this effect are limited. Here we show that a signature of spin-orbit scattering manifests itself in quasiparticle interference (QPI) imaged by spectroscopic-imaging scanning tunneling microscopy. The experimental data of a polar semiconductor BiTeI are well reproduced by numerical simulations with the $T$-matrix formalism that include not only scalar scattering normally adopted but also spin-orbit scattering stronger than scalar scattering. To accelerate the simulations, we extend the standard efficient method of QPI calculation for momentum-independent scattering to be applicable even for spin-orbit scattering. We further identify a selection rule that makes spin-orbit scattering visible in the QPI pattern. These results demonstrate that spin-orbit scattering can exert predominant influence on QPI patterns and thus suggest that QPI measurement is available to detect spin-orbit scattering.
The cuprate high-temperature superconductors are known to host a wide array of effects due to interactions and disorder. In this work, we look at some of the consequences of these effects which can be visualized by scanning tunneling spectroscopy. These interaction and disorder effects can be incorporated into a mean-field description by means of a self-energy appearing in the Greens function. We first examine the quasiparticle scattering interference spectra in the superconducting state at optimal doping as temperature is increased. Assuming agreement with angle-resolved photoemission experiments which suggest that the scattering rate depends on temperature, resulting in the filling of the $d$-wave gap, we find that the peaks predicted by the octet model become progressively smeared as temperature is increased. When the scattering rate is of the same order of magnitude as the superconducting gap, the spectral function shows Fermi-arc-like patterns, while the power spectrum of the local density of states shows the destruction of the octet-model peaks. We next consider the normal state properties of the optimally-doped cuprates. We model this by adding a marginal Fermi liquid self-energy to the normal-state propagator, and consider the dependence of the QPI spectra on frequency, temperature, and doping. We demonstrate that the MFL self-energy leads to a smearing of the caustics appearing in the normal-state QPI power spectrum as either temperature or frequency is increased at fixed doping. The smearing is found to be more prominent in the MFL case than in an ordinary Fermi liquid. We also consider the case of a marginal Fermi liquid with a strongly momentum-dependent self-energy which gives rise to a visible nodal-antinodal dichotomy at the normal state, and discuss how the spectra as seen in ARPES and STS differ from both an isotropic metal and a broadened $d$-wave superconductor.
Time-resolved spontaneous Raman spectroscopy serves as a probe for incoherent quasiparticle and collective excitation dynamics, and allows to distinguish symmetry changes across a photoinduced phase transition through the inelastic light scattering selection rules. Largely unexplored is the role of the Raman resonance enhancement in the time-domain, and the transient interaction between scattering from quasiparticles and collective excitations, with the latter interaction leading to a Fano interference. In this work, we report on the observation of a phonon Raman tensor quench and Fano interference after strong photoexcitation of an intrinsic semiconductor. We observed a dynamic phonon scattering rate asymmetry and spectral asymmetry through simultaneous detection of both the anti-Stokes and Stokes response. The asymmetric phonon scattering rate is ascribed to the combined effect of the transient phonon population and the reduction of the phonon Raman tensor resulting from the photoexcited hole population. This same hole population results in a strong enhancement of the Fano spectral asymmetry.
We report the first observation of coherent surface states on cubic perovskite oxide SrVO3(001) thin films through spectroscopic imaging scanning tunneling microscopy. A direct link between the observed atomic-scale interference patterns and the formation of a dxy-derived surface state is supported by first-principles calculations. Furthermore, we show that the apical oxygens on the topmost VO2 plane play a critical role in controlling the spectral weight of the observed coherent surface state.