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Controlling surface charge and spin density oscillations by Dirac plasmon interaction in thin topological insulators

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 Added by Ruben Esteban
 Publication date 2017
  fields Physics
and research's language is English




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We study the selective excitation at infrared and THz frequencies of optical and acoustic plasmonic modes supported by thin topological insulators. These modes are characterized by effective net charge or net spin density, respectively, and we study their excitation by combining many-body and electromagnetic calculations. We first show that non-locality can significantly modify the plasmonic response: it changes the energy of propagating plasmons up to tens of percent. We then discuss how, by changing the distance between a dipolar source and a semi-infinite 10 nm thin film, it is possible to control the excitation of acoustic and optical propagating plasmons, which can propagate over a distance of several plasmonic wavelengths. Furthermore, we consider 10 nm thin TI nanodisks and study the excitation of acoustic and optical localized plasmon modes by a point dipole source and plane wave illumination, respectively. The resonant plasmonic modes appear at frequencies that strongly depends on the size of the disk, and that can be potentially tuned by applying electrostatic gating to modify the Fermi Energy of the conductive 2-dimensional layer that forms at the interfaces of the TI. We observe a spectral shift from ~29 $mu$m to ~34 $mu$m by changing the Fermi Energy from 250meV to 350meV. Last, the electromagnetic energy of these plasmonics modes can be confined to very small regions, of effective volume ~(120 nm)^3 for the smaller disk considered, much less than the free-space wavelength cubed $lambda$^3 ~(35000 nm)^3. The strong confinement is desirable for achieving very efficient coupling with nearby systems. Our detailed study thus shows that thin topological insulators are a promising system to control both the spin and charge oscillations associated with the plasmonic resonances, with possible applications to fast, compact and electrically-controlled spintronics devices.



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We investigate the spin and charge densities of surface states of the three-dimensional topological insulator $Bi_2Se_3$, starting from the continuum description of the material [Zhang {em et al.}, Nat. Phys. 5, 438 (2009)]. The spin structure on surfaces other than the 111 surface has additional complexity because of a misalignment of the contributions coming from the two sublattices of the crystal. For these surfaces we expect new features to be seen in the spin-resolved ARPES experiments, caused by a non-helical spin-polarization of electrons at the individual sublattices as well as by the interference of the electron waves emitted coherently from two sublattices. We also show that the position of the Dirac crossing in spectrum of surface states depends on the orientation of the interface. This leads to contact potentials and surface charge redistribution at edges between different facets of the crystal.
We have investigated the nature of surface states in the Bi2Te3 family of three-dimensional topological insulators using first-principles calculations as well as model Hamiltonians. When the surface Dirac cone is warped due to Dresselhaus spin-orbit coupling in rhombohedral structures, the spin acquires a finite out-of-plane component. We predict a novel in-plane spin-texture of the warped surface Dirac cone with spins not perpendicular to the electron momentum. Our k.p model calculation reveals that this novel in-plane spin-texture requires high order Dresselhaus spin-orbit coupling terms.
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One of the most fascinating challenges in Physics is the realization of an electron-based counterpart of quantum optics, which requires the capability to generate and control single electron wave packets. The edge states of quantum spin Hall (QSH) systems, i.e. two-dimensional (2D) topological insulators realized in HgTe/CdTe and InAs/GaSb quantum wells, may turn the tide in the field, as they do not require the magnetic field that limits the implementations based on quantum Hall effect. Here we show that an electric pulse, localized in space and/or time and applied at a QSH edge, can photoexcite electron wavepackets by intra-branch electrical transitions, without invoking the bulk states or the Zeeman coupling. Such wavepackets are spin-polarised and propagate in opposite directions, with a density profile that is independent of the initial equilibrium temperature and that does not exhibit dispersion, as a result of the linearity of the spectrum and of the chiral anomaly characterising massless Dirac electrons. We also investigate the photoexcited energy distribution and show how, under appropriate circumstances, minimal excitations (Levitons) are generated. Furthermore, we show that the presence of a Rashba spin-orbit coupling can be exploited to tailor the shape of photoexcited wavepackets. Possible experimental realizations are also discussed.
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