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Register a new userNanoscale Magnetic Imaging using Circularly Polarized High-Harmonic Radiation
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Authors
Ofer Kfir
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This work demonstrates nanoscale magnetic imaging using bright circularly polarized high-harmonic radiation. We utilize the magneto-optical contrast of worm-like magnetic domains in a Co/Pd multilayer structure, obtaining quantitative amplitude and phase maps by lensless imaging. A diffraction-limited spatial resolution of 49 nm is achieved with iterative phase reconstruction enhanced by a holographic mask. Harnessing the unique coherence of high harmonics, this approach will facilitate quantitative, element-specific and spatially-resolved studies of ultrafast magnetization dynamics, advancing both fundamental and applied aspects of nanoscale magnetism.
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We numerically demonstrate that a planar slab made of magnetic Weyl semimetal (a class of topological materials) can emit high-purity circularly polarized (CP) thermal radiation over a broad mid- and long-wave infrared wavelength range for a significant portion of its emission solid angle. This effect fundamentally arises from the strong infrared gyrotropy or nonreciprocity of these materials which primarily depends on the momentum separation between Weyl nodes in the band structure. We clarify the dependence of this effect on the underlying physical parameters and highlight that the spectral bandwidth of CP thermal emission increases with increasing momentum separation between the Weyl nodes. We also demonstrate using recently developed thermal discrete dipole approximation (TDDA) computational method that finite-size bodies of magnetic Weyl semimetals can emit spectrally broadband CP thermal light, albeit over smaller portion of the emission solid angle compared to the planar slabs. Our work identifies unique fundamental and technological prospects of magnetic Weyl semimetals for engineering thermal radiation and designing efficient CP light sources.
High-harmonic generation in two-colour ($omega-2omega$) counter-rotating circularly polarised laser fields opens the path to generate isolated attosecond pulses and attosecond pulse trains with controlled ellipticity. The generated harmonics have alternating helicity, and the ellipticity of the generated attosecond pulse depends sensitively on the relative intensities of two adjacent, counter-rotating harmonic lines. For the $s$-type ground state, such as in Helium, the successive harmonics have nearly equal amplitude, yielding isolated attosecond pulses and attosecond pulse trains with linear polarisation, rotated by 120$^{{circ}}$ from pulse to pulse. In this work, we suggest a solution to overcome the limitation associated with the $s$-type ground state. It is based on modifying the three propensity rules associated with the three steps of the harmonic generation process: ionisation, propagation, and recombination. We control the first step by seeding high harmonic generation with XUV light tuned well below the ionisation threshold, which generates virtual excitations with the angular momentum co-rotating with the $omega$-field. We control the propagation step by increasing the intensity of the $omega$-field relative to the $2omega$-field, further enhancing the chance of the $omega$-field being absorbed versus the $2omega$-field, thus favouring the emission co-rotating with the seed and the $omega-$field. We demonstrate our proposed control scheme using Helium atom as a target and solving time-dependent Schr{o}dinger equation in two and three-dimensions.
Topological states of light represent counterintuitive optical modes localized at boundaries of finite-size optical structures that originate from the properties of the bulk. Being defined by bulk properties, such boundary states are insensitive to certain types of perturbations, thus naturally enhancing robustness of photonic circuitries. Conventionally, the N-dimensional bulk modes correspond to (N-1)-dimensional boundary states. The higher-order bulk-boundary correspondence relates N-dimensional bulk to boundary states with dimensionality reduced by more than 1. A special interest lies in miniaturization of such higher-order topological states to the nanoscale. Here, we realize nanoscale topological corner states in metasurfaces with C6-symmetric honeycomb lattices. We directly observe nanoscale topology-empowered edge and corner localizations of light and enhancement of light-matter interactions via a nonlinear imaging technique. Control of light at the nanoscale empowered by topology may facilitate miniaturization and on-chip integration of classical and quantum photonic devices.
High-order harmonic generation in the presence of a chirped THz pulse is investigated numerically with a complete 3D non-adiabatic model. The assisting THz pulse illuminates the HHG gas cell laterally inducing quasi-phase-matching. We demonstrate that it is possible to compensate the phase mismatch during propagation and extend the macroscopic cutoff of a propagated strong IR pulse to the single-dipole cutoff. We obtain two orders of magnitude increase in the harmonic efficiency of cutoff harmonics ($approx$170 eV) using a THz pulse of constant wavelength, and a further factor of 3 enhancement when a chirped THz pulse is used.
Circularly-polarized extreme UV and X-ray radiation provides valuable access to the structural, electronic and magnetic properties of materials. To date, this capability was available only at large-scale X-ray facilities such as synchrotrons. Here we demonstrate the first bright, phase-matched, extreme UV circularly-polarized high harmonics and use this new light source for magnetic circular dichroism measurements at the M-shell absorption edges of Co. We show that phase matching of circularly-polarized harmonics is unique and robust, producing a photon flux comparable to the linearly polarized high harmonic sources that have been used very successfully for ultrafast element-selective magneto-optic experiments. This work thus represents a critical advance that makes possible element-specific imaging and spectroscopy of multiple elements simultaneously in magnetic and other chiral media with very high spatial and temporal resolution, using tabletop-scale setups.
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