No Arabic abstract
On-chip single-photon sources are key components for integrated photonic quantum technologies. Semiconductor quantum dots can exhibit near-ideal single-photon emission but this can be significantly degraded in on-chip geometries owing to nearby etched surfaces. A long-proposed solution to improve the indistinguishablility is by using the Purcell effect to reduce the radiative lifetime. However, until now only modest Purcell enhancements have been observed. Here we use pulsed resonant excitation to eliminate slow relaxation paths, revealing a highly Purcell-shortened radiative lifetime (22.7 ps) in a waveguide-coupled quantum dot-photonic crystal cavity system. This leads to near-lifetime-limited single-photon emission which retains high indistinguishablility (93.9%) on a timescale in which 20 photons may be emitted. Nearly background-free pulsed resonance fluorescence is achieved under $pi$-pulse excitation, enabling demonstration of an on-chip, on-demand single-photon source with very high potential repetition rates.
We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7pm0.8)~%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4pm1.5)~%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical excitation, which enables us to deterministically populate the excited QD state. In this configuration, we probe the single photon statistics of the device yielding $g^{(2)}(0)=0.072pm0.011$ at a QD-cavity detuning of $75~mu$eV.
Operating reconfigurable quantum circuits with single photon sources is a key goal of photonic quantum information science and technology. We use an integrated waveguide device comprising of directional couplers and a reconfigurable thermal phase controller to manipulate single photons emitted from a chromium related colour centre in diamond. Observation of both a wave-like interference pattern and particle-like sub-Poissionian autocorrelation functions demonstrates coherent manipulation of single photons emitted from the chromium related centre and verifies wave particle duality.
We propose related schemes to generate arbitrarily shaped single photons, i.e. photons with an arbitrary temporal profile, and coherent state superpositions using simple optical elements. The first system consists of two coupled cavities, a memory cavity and a shutter cavity, containing a second order optical nonlinearity and electro-optic modulator (EOM) respectively. Photodetection events of the shutter cavity output herald preparation of a single photon in the memory cavity, which may be stored by immediately changing the optical length of the shutter cavity with the EOM after detection. On-demand readout of the photon, with arbitrary shaping, can be achieved through modulation of the EOM. The second scheme consists of a memory cavity with two outputs which are interfered, phase shifted, and measured. States that closely approximate a coherent state superposition can be produced through postselection for sequences of detection events, with more photon detection events leading to a larger superposition. We furthermore demonstrate that `No-Knowledge Feedback can be easily implemented in this system and used to preserve the superposition state, as well as provide an extra control mechanism for state generation.
We introduce a filter using a noise-free quantum buffer with large optical bandwidth that can both filter temporal-spectral modes, as well as inter-convert them and change their frequency. We show that such quantum buffers optimally filter out temporal-spectral noise; producing identical single-photons from many distinguishable noisy single-photon sources with the minimum required reduction in brightness. We then experimentally demonstrate a noise-free quantum buffer in a warm atomic system that is well matched to quantum dots and can outperform all intensity (incoherent) filtering schemes for increasing indistinguishability.
Silicon carbide has recently been developed as a platform for optically addressable spin defects. In particular, the neutral divacancy in the 4H polytype displays an optically addressable spin-1 ground state and near-infrared optical emission. Here, we present the Purcell enhancement of a single neutral divacancy coupled to a photonic crystal cavity. We utilize a combination of nanolithographic techniques and a dopant-selective photoelectrochemical etch to produce suspended cavities with quality factors exceeding 5,000. Subsequent coupling to a single divacancy leads to a Purcell factor of ~50, which manifests as increased photoluminescence into the zero-phonon line and a shortened excited-state lifetime. Additionally, we measure coherent control of the divacancy ground state spin inside the cavity nanostructure and demonstrate extended coherence through dynamical decoupling. This spin-cavity system represents an advance towards scalable long-distance entanglement protocols using silicon carbide that require the interference of indistinguishable photons from spatially separated single qubits.