No Arabic abstract
Spectral dispersion of ultrashort pulses allows simultaneous focusing of light in both space and time creating so-called spatio-temporal foci. Such space-time coupling may be combined with existing holographic techniques to give a further dimension of control when generating focal light fields. It is shown that a phase-only hologram placed in the pupil plane of an objective and illuminated by a spatially chirped ultrashort pulse can be used to generate three dimensional arrays of spatio-temporally focused spots. Exploiting the pulse front tilt generated at focus when applying simultaneous spatial and temporal focusing (SSTF), it is possible to overlap neighbouring foci in time to create a smooth intensity distribution. The resulting light field displays a high level of axial confinement, with experimental demonstrations given through two-photon microscopy and non-linear laser fabrication of glass.
We present an apparatus that converts every pulse of a pulsed light source to a pulse train in which the intensities of the different pulses are samples of the spatial or temporal frequency spectrum of the original pulse. In this way, the spectrum of the incident light can be measured by following the temporal response of a single detector. The apparatus is based on multiple round-trips inside a 2f- cavity-like mirror arrangement in which the spectrum is spread on the back focal plane, where after each round-trip a small section of the spectrum is allowed to escape. The apparatus is fibre-free, offers easy wavelength range tunability, and a prototype built achieves over 10% average efficiency in the near infra red. We demonstrate the application of the prototype for the efficient measurement of the joint spectrum of a non-degenerate bi-photon source in which one of the photons is in the near infra red.
The ultrafast response of metals to light is governed by intriguing non-equilibrium dynamics involving the interplay of excited electrons and phonons. The coupling between them gives rise to nonlinear diffusion behavior on ultrashort timescales. Here, we use scanning ultrafast thermo-modulation microscopy to image the spatio-temporal hot-electron diffusion in a thin gold film. By tracking local transient reflectivity with 20 nm and 0.25 ps resolution, we reveal two distinct diffusion regimes, consisting of an initial rapid diffusion during the first few picoseconds after optical excitation, followed by about 100-fold slower diffusion at longer times. We simulate the thermo-optical response of the gold film with a comprehensive three-dimensional model, and identify the two regimes as hot-electron and phonon-limited thermal diffusion, respectively.
The concepts of Fourier optics were established in France in the 1940s by Pierre-Michel Duffieux, and laid the foundations of an extensive series of activities in the French research community that have touched on nearly every aspect of contemporary optics and photonics. In this paper, we review a selection of results where applications of the Fourier transform and transfer functions in optics have been applied to yield significant advances in unexpected areas of optics, including the spatial shaping of complex laser beams in amplitude and in phase, real-time ultrafast measurements, novel ghost imaging techniques, and the development of parallel processing methodologies for photonic artificial intelligence.
Light emitted from a source into a scene can undergo complex interactions with scene surfaces of different material types before being reflected. During this transport, every surface reflection is encoded in the properties of the photons that reach the detector, including time, direction, intensity, wavelength and polarization. Conventional imaging systems capture intensity by integrating over all other dimensions of the light, hiding this rich scene information. Existing methods are capable of untangling these measurements into their spatial and temporal dimensions, fueling geometric scene understanding tasks. However, examining material properties jointly with geometric properties is an open challenge that could enable unprecedented capabilities beyond geometric scene understanding, allowing for material-dependent scene understanding and imaging through complex transport. In this work, we close this gap, and propose a computational light transport imaging method that captures the spatially- and temporally-resolved complete polarimetric response of a scene. Our method hinges on a 7D tensor theory of light transport. We discover low-rank structure in the polarimetric tensor dimension and propose a data-driven rotating ellipsometry method that learns to exploit redundancy of polarimetric structure. We instantiate our theory with two prototypes: spatio-polarimetric imaging and coaxial temporal-polarimetric imaging. This allows us, for the first time, to decompose scene light transport into temporal, spatial, and complete polarimetric dimensions that unveil scene properties hidden to conventional methods. We validate the applicability of our method on diverse tasks, including shape reconstruction with subsurface scattering, seeing through scattering media, untangling multi-bounce light transport, breaking metamerism, and decomposition of crystals.
The shortest light pulses produced to date are of the order of a few tens of attoseconds, with central frequencies in the extreme ultraviolet range and bandwidths exceeding tens of eV. They are often produced as a train of pulses separated by half the driving laser period, leading in the frequency domain to a spectrum of high, odd-order harmonics. As light pulses become shorter and more spectrally wide, the widely-used approximation consisting in writing the optical waveform as a product of temporal and spatial amplitudes does not apply anymore. Here, we investigate the interplay of temporal and spatial properties of attosecond pulses. We show that the divergence and focus position of the generated harmonics often strongly depend on their frequency, leading to strong chromatic aberrations of the broadband attosecond pulses. Our argumentation uses a simple analytical model based on Gaussian optics, numerical propagation calculations and experimental harmonic divergence measurements. This effect needs to be considered for future applications requiring high quality focusing while retaining the broadband/ultrashort characteristics of the radiation.