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Free-Space Quantum Electrodynamics with a single Rydberg superatom

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 Publication date 2017
  fields Physics
and research's language is English




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The interaction of a single photon with an individual two-level system is the textbook example of quantum electrodynamics. Achieving strong coupling in this system so far required confinement of the light field inside resonators or waveguides. Here, we demonstrate strong coherent coupling between a single Rydberg superatom, consisting of thousands of atoms behaving as a single two-level system due to the Rydberg blockade, and a propagating light pulse containing only a few photons. The strong light-matter coupling in combination with the direct access to the outgoing field allows us to observe for the first time the effect of the interactions on the driving field at the single photon level. We find that all our results are in quantitative agreement with the predictions of the theory of a single two-level system strongly coupled to a single quantized propagating light mode. The demonstrated coupling strength opens the way towards interfacing photonic and atomic qubits and preparation of propagating non-classical states of light, two crucial building blocks in future quantum networks.



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We experimentally investigate the collective decay of a single Rydberg superatom, formed by an ensemble of thousands of individual atoms supporting only a single excitation due to the Rydberg blockade. Instead of observing a constant decay rate determined by the collective coupling strength to the driving field, we show that the enhanced emission of the single stored photon into the forward direction of the coupled optical mode depends on the dynamics of the superatom before the decay. We find that the observed decay rates are reproduced by an expanded model of the superatom which includes coherent coupling between the collective bright state and subradiant states.
We propose to implement the Jaynes-Cummings model by coupling a few-micrometer large atomic ensemble to a quantized cavity mode and classical laser fields. A two-photon transition resonantly couples the single-atom ground state |g> to a Rydberg state |e> via a non-resonant intermediate state |i>, but due to the interaction between Rydberg atoms only a single atom can be resonantly excited in the ensemble. This restricts the state space of the ensemble to the collective ground state |G> and the collectively excited state |E> with a single Rydberg excitation distributed evenly on all atoms. The collectively enhanced coupling of all atoms to the cavity field with coherent coupling strengths which are much larger than the decay rates in the system leads to the strong coupling regime of the resulting effective Jaynes-Cummings model. We use numerical simulations to show that the cavity transmission can be used to reveal detailed properties of the Jaynes-Cummings ladder of excited states, and that the atomic nonlinearity gives rise to highly non-trivial photon emission from the cavity. Finally, we suggest that the absence of interactions between remote Rydberg atoms may, due to a combinatorial effect, induce a cavity-assisted excitation blockade whose range is larger than the typical Rydberg dipole-dipole interaction length.
111 - D. Petrosyan , K. M{o}lmer 2018
We propose an efficient free-space scheme to create single photons in a well-defined spatiotemporal mode. To that end, we first prepare a single source atom in an excited Rydberg state. The source atom interacts with a large ensemble of ground-state atoms via a laser-mediated dipole-dipole exchange interaction. Using an adiabatic passage with a chirped laser pulse, we produce a spatially extended spin wave of a single Rydberg excitation in the ensemble, accompanied by the transition of the source atom to another Rydberg state. The collective atomic excitation can then be converted to a propagating optical photon via a coherent coupling field. In contrast to previous approaches, our single-photon source does not rely on the strong coupling of a single emitter to a resonant cavity, nor does it require the heralding of collective excitation or complete Rydberg blockade of multiple excitations in the atomic ensemble.
We propose a hybrid optomechanical quantum system consisting of a moving membrane strongly coupled to an ensemble of N atoms with a Rydberg state. Due to the strong van-der-Waals interaction between the atoms, the ensemble forms an effective two-level system, a Rydberg superatom, with a collectively enhanced atom-light coupling. Using this superatom imposed collective enhancement strong coupling between membrane and superatom is feasible for parameters within the range of current experiments. The quantum interface to couple the membrane and the superatom can be a pumped single mode cavity, or a laser field in free space, where the Rydberg superatom and the membrane are spatially separated. In addition to the coherent dynamics, we study in detail the impact of the typical dissipation processes, in particular the radiative decay as a source for incoherent superpositions of atomic excitations. We identify the conditions to suppress these incoherent dynamics and thereby a parameter regime for strong coupling. The Rydberg superatom in this hybrid system serves as a toolbox for the nanomechanical resonator allowing for a wide range of applications such as state transfer, sympathetic cooling and non-classical state preparation. As an illustration, we show that a thermally occupied membrane can be prepared in a non-classical state without the necessity of ground state cooling.
We report on the experimental observation of non-trivial three-photon correlations imprinted onto initially uncorrelated photons through interaction with a single Rydberg superatom. Exploiting the Rydberg blockade mechanism, we turn a cold atomic cloud into a single effective emitter with collectively enhanced coupling to a focused photonic mode which gives rise to clear signatures in the connected part of the three-body correlation function of the out-going photons. We show that our results are in good agreement with a quantitative model for a single, strongly coupled Rydberg superatom. Furthermore, we present an idealized but exactly solvable model of a single two-level system coupled to a photonic mode, which allows for an interpretation of our experimental observations in terms of bound states and scattering states.
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