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Theoretical derivation of laser-dressed atomic states by using a fractal space

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 Added by Guillaume Duchateau
 Publication date 2017
  fields Physics
and research's language is English




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The derivation of approximate wave functions for an electron submitted to both a coulomb and a time-dependent laser electric fields, the so-called Coulomb-Volkov (CV) state, is addressed. Despite its derivation for continuum states does not exhibit any particular problem within the framework of the standard theory of quantum mechanics (QM), difficulties arise when considering an initially bound atomic state. Indeed the natural way of translating the unperturbed momentum by the laser vector potential is no longer possible since a bound state does not exhibit a plane wave form including explicitely a momentum. The use of a fractal space permits to naturally define a momentum for a bound wave function. Within this framework, it is shown how the derivation of laser-dressed bound states can be performed. Based on a generalized eikonal approach, a new expression for the laser-dressed states is also derived, fully symmetric relative to the continuum or bound nature of the initial unperturbed wave function. It includes an additional crossed term in the Volkov phase which was not obtained within the standard theory of quantum mechanics. The derivations within this fractal framework have highlighted other possible ways to derive approximate laser-dressed states in QM. After comparing the various obtained wave functions, an application to the prediction of the ionization probability of hydrogen targets by attosecond XUV pulses within the sudden approximation is provided. This approach allows to make predictions in various regimes depending on the laser intensity, going from the non-resonant multiphoton absorption to tunneling and barrier-suppression ionization.

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Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra-violet) -- IR (infrared) measurement, the XUV photon energy is scanned between SI{20.4}{electronvolt} and the ionization threshold at SI{24.6}{electronvolt}, revealing electric dipole-forbidden transitions for a temporally overlapping IR pulse ($sim!SI{e12}{wattper centimetersquared}$). The interpretation of the experimental results is supported by numerically solving the time-dependent Schrodinger equation in a single-active-electron approximation.
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