No Arabic abstract
The determination of the longitudinal spin Seebeck effect (LSSE) coefficient is currently plagued by a large uncertainty due to the poor reproducibility of the experimental conditions used in its measurement. In this work we present a detailed analysis of two different methods used for the determination of the LSSE coefficient. We have performed LSSE experiments in different laboratories, by using different setups and employing both the temperature difference method and the heat flux method. We found that the lack of reproducibility can be mainly attributed to the thermal contact resistance between the sample and the thermal baths which generate the temperature gradient. Due to the variation of the thermal resistance, we found that the scaling of the LSSE voltage to the heat flux through the sample rather than to the temperature difference across the sample greatly reduces the uncertainty. The characteristics of a single YIG/Pt LSSE device obtained with two different setups was $(1.143pm0.007)cdot 10^{-7}$ Vm/W and $(1.101pm0.015)cdot 10^{-7}$ Vm/W with the heat flux method and $(2.313pm0.017)cdot 10^{-7}$ V/K and $(4.956pm0.005)cdot 10^{-7}$ V/K with the temperature difference method. This shows that systematic errors can be considerably reduced with the heat flux method.
Using a simplified microscopic model of coupled spin and lattice excitations in a ferromagnetic insulator we evaluate the magnetic-field dependence of the spin Seebeck effect at low temperatures. The model includes Heisenberg exchange coupling, a harmonic lattice potential, and a pseudo-dipolar exchange interaction. Our approach goes beyond previous work [Phys. Rev. B 98, 134421 (2018)] in that it does not rely on the a priori assumption of a fast equilibration of the magnon and phonon distributions. Our theory shows that singular features in the magnetic-field dependence of the spin Seebeck effect at low temperatures observed by Kikkawa et al. [Phys. Rev. Lett. 117, 207203 (2016)] are independent of the relative strength of magnon-impurity and phonon-impurity scattering.
We found a giant Seebeck effect in semiconducting single-wall carbon nanotube (SWCNT) films, which exhibited a performance comparable to that of commercial Bi2Te3 alloys. Carrier doping of semiconducting SWCNT films further improved the thermoelectric performance. These results were reproduced well by first-principles transport simulations based on a simple SWCNT junction model. These findings suggest strategies that pave the way for emerging printed, all-carbon, flexible thermoelectric devices.
We develop a Boltzmann transport theory of coupled magnon-phonon transport in ferromagnetic insulators. The explicit treatment of the magnon-phonon coupling within the Boltzmann approach allows us to calculate the low-temperature magnetic-field dependence of the spin-Seebeck voltage. Within the Boltzmann theory we find that this magnetic field dependence shows similar features as found by Flebus et al. [Phys. Rev. B 95, 144420 (2017)] for a strongly coupled magnon phonon system that forms magnon-polarons, and consistent with experimental findings in yttrium iron garnet by Kikkawa et al. [Phys. Rev. Lett. 117, 207203 (2016)]. In addition to the anomalous magnetic-field dependence of the spin Seebeck effect, we also predict a dependence on the system size.
A new measurement technique for the spin Seebeck effect is presented, wherein the normal metal layer used for its detection is exploited simultaneously as a resistive heater and thermometer. We show how the various contributions to the measured total signal can be disentangled, allowing to extract the voltage signal solely caused by the spin Seebeck effect. To this end we performed measurements as a function of the external magnetic field strength and its orientation. We find that the effect scales linearly with the induced rise in temperature, as expected for the spin Seebeck effect.
Since its experimental discovery, many phenomenological theories successfully reproduced the rapid rise from $p$ to $1+p$ found in the Hall number $n_H$ at the critical doping $p^*$ of the pseudogap in superconducting cuprates. Further comparison with experiments is now needed in order to narrow down candidates. In this paper, we consider three previously successful phenomenological theories in a unified formalism---an antiferromagnetic mean field (AF), a spiral incommensurate antiferromagnetic mean field (sAF), and the Yang-Rice-Zhang (YRZ) theory. We find a rapid rise in the specific heat and a rapid drop in the Seebeck coefficient for increasing doping across the transition in each of those models. The predicted rises and drops are locked, not to~$p^*$, but to the doping where anti-nodal electron pockets, characteristic of each model, appear at the Fermi surface shortly before~$p^*$. While such electron pockets are still to be found in experiments, we discuss how they could provide distinctive signatures for each model. We also show that the range of doping where those electron pockets would be found is strongly affected by the position of the van~Hove singularity.