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Register a new userNear-field collection of fluorescence of quantum dots with a fiber-integrated multimode plasmonic probe
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Strong light-matter interaction and high-efficiency optical collection of fluorescence from quantum emitters are crucial topics in quantum and nanophotonic fields. High-quality cavities, dispersive photonic crystal waveguides and even plasmonic structures have been used to enhance the interaction with quantum emitters, thus realize efficient collection of the fluorescence. In this work, a new method is proposed to collect the fluorescence of quantum dots (QDs) with a fiber-integrated multimode silver nanowire (AgNW) waveguide. Fluorescence lifetime measurement is performed to investigate the coupling between QDs and different plasmonic modes. Compared with far-field collection method, the AgNW-fiber probe can realize near-unity collection efficiency theoretically. This fiber-integrated plasmonic probe may be useful in the area of nanophotonics and also promising for quantum information devices.
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Plasmonic nanopatch antennas that incorporate dielectric gaps hundreds of picometers to several nanometers thick have drawn increasing attention over the past decade because they confine electromagnetic fields to grossly sub-diffraction limited volumes. Substantial control over the optical properties of excitons and color centers confined within these plasmonic cavities has already been demonstrated with far-field optical spectroscopies, but near-field optical spectroscopies are essential to an improved understanding of the plasmon-emitter interaction at the nanoscale. Here, we characterize the intensity and phase-resolved plasmonic response of isolated nanopatch antennas with cathodoluminescence microscopy. Further, we explore the distinction between optical and electron-beam spectroscopies of coupled plasmon-exciton heterostructures to identify constraints and opportunities for future nanoscale characterization and control of hybrid nanophotonic structures. While we observe substantial Purcell enhancement in time-resolved photoluminescence spectroscopies, negligible Purcell enhancement is observed in cathodoluminescence spectroscopies of hybrid nanophotonic structures. The substantial differences in measured Purcell enhancement for electron-beam and laser excitation can be understood as a result of the different selection rules for these complementary experiments. These results provide a fundamentally new understanding of near-field plasmon-exciton interactions in nanopatch antennas that is essential to myriad emerging quantum photonic devices.
Photonic quantum technologies call for scalable quantum light sources that can be integrated, while providing the end user with single and entangled photons on-demand. One promising candidate are strain free GaAs/AlGaAs quantum dots obtained by droplet etching. Such quantum dots exhibit ultra low multi-photon probability and an unprecedented degree of photon pair entanglement. However, different to commonly studied InGaAs/GaAs quantum dots obtained by the Stranski-Krastanow mode, photons with a near-unity indistinguishability from these quantum emitters have proven to be elusive so far. Here, we show on-demand generation of near-unity indistinguishable photons from these quantum emitters by exploring pulsed resonance fluorescence. Given the short intrinsic lifetime of excitons confined in the GaAs quantum dots, we show single photon indistinguishability with a raw visibility of $V_{raw}=(94.2pm5.2),%$, without the need for Purcell enhancement. Our results represent a milestone in the advance of GaAs quantum dots by demonstrating the final missing property standing in the way of using these emitters as a key component in quantum communication applications, e.g. as an entangled source for quantum repeater architectures.
One of the outstanding challenges for ion trap quantum information processing is to accurately detect the states of many ions in a scalable fashion. In the particular case of surface traps, geometric constraints make imaging perpendicular to the surface appealing for light collection at multiple locations with minimal cross-talk. In this report we describe an experiment integrating Diffractive Optic Elements (DOEs) with surface electrode traps, connected through in-vacuum multi-mode fibers. The square DOEs reported here were all designed with solid angle collection efficiencies of 3.58%; with all losses included a detection efficiency of 0.388% (1.02% excluding the PMT loss) was measured with a single Ca+ ion. The presence of the DOE had minimal effect on the stability of the ion, both in temporal variation of stray electric fields and in motional heating rates.
We experimentally study the competition between Kerr beam self-cleaning and Raman beam cleanup in a multimode air-silica microstructure optical fiber. Kerr beam self-cleaning of the pump is observed for a certain range of input powers only. Raman Stokes beam generation and cleanup lead to both depletion and degradation of beam quality for the pump. The interplay of modal four-wave mixing and Raman scattering in the infrared domain lead to the generation of a multimode supercontinuum ranging from 500 nm up to 1800 nm.
We experimentally isolate and directly observe multimode solitons in few-mode graded-index fiber. By varying the input energy and modal composition of the launched pulse, we observe a continuous variation of multimode solitons with different spatiotemporal properties. They exhibit an energy-volume relation that is distinct from those of single-mode and fully spatiotemporal solitons.
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