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Register a new userStatic and Dynamic Properties of Two Dimensional Coulomb Clusters
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We study the temperature dependence of static and dynamic responses of Coulomb interacting particles in two-dimensional traps across the thermal crossover from an amorphous solid- to liquid-like behaviors. While static correlations, that investigate the translational and bond orientational order in the confinements, show the footprints of hexatic-like phase at low temperature, dynamics of the particles slow down considerably in this state -- reminiscent of a supercooled liquid. Using density correlations, we probe intriguing signatures of long-lived inhomogeneities due to the interplay of the irregularity in the confinement and long-range Coulomb interactions. The relaxation at multiple time scales show stretched-exponential decay of spatial correlations in irregular traps. Temperature dependence of characteristic time scales, depicting the structural relaxation of the system, show striking similarities with those observed for the glassy systems indicating that, some of the key signatures of supercooled liquids emerge in confinements with lower spatial symmetries.
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We study various properties of the vibrational normal modes for Coulomb-interacting particles in two-dimensional irregular confinement using numerical simulations. By analyzing the participation ratio and spectral statistics, we characterize the vibrational modes for Coulomb clusters as localized, quasi-localized and delocalized. We also study a novel correlation function to understand the spatial structure of these different kinds of modes and subsequently extract the associated characteristic length scales. We further demonstrate that, at any given temperature, particles exhibiting larger displacement over a time interval comparable to the structural relaxation time, are strongly correlated with the low-frequency quasi-localized modes of the inherent structure corresponding to the initial configuration. Establishing this correlation for Coulomb clusters paves the path to identify the particular feature of the initial configuration that determines the previously observed heterogeneous dynamics of the particles at low temperatures in these systems.
We study heat conduction mediated by longitudinal phonons in one dimensional disordered harmonic chains. Using scaling properties of the phonon density of states and localization in disordered systems, we find non-trivial scaling of the thermal conductance with the system size. Our findings are corroborated by extensive numerical analysis. We show that a system with strong disorder, characterized by a `heavy-tailed probability distribution, and with large impedance mismatch between the bath and the system satisfies Fouriers law. We identify a dimensionless scaling parameter, related to the temperature scale and the localization length of the phonons, through which the thermal conductance for different models of disorder and different temperatures follows a universal behavior.
Two-dimensional materials can be strongly influenced by their surroundings. A dielectric environment screens and reduces the Coulomb interaction between electrons in the two-dimensional material. Since the Coulomb interaction is responsible for the insulating state of Mott materials, dielectric screening provides direct access to the Mottness. Our many-body calculations reveal the spectroscopic fingerprints of Coulomb engineering. We demonstrate eV-scale changes to the position of the Hubbard bands and show a Coulomb engineered insulator-to-metal transition. Based on this theoretical analysis, we discuss prerequisites for an effective experimental realization of Coulomb engineering.
We discuss the onset of many body localisation in a one-dimensional system composed of a XXZ quantum spin chain and a Bose-Hubbard model linearly coupled together. We consider two complementary setups depending whether spatial disorder is initially imprinted on spins or on bosons; in both cases, we explore the conditions for the disordered portion of the system to localise by proximity of the other clean half. Assuming that the dynamics of one of the two parts develops on shorter time scales than the other, we can adiabatically eliminate the fast degrees of freedom, and derive an effective hamiltonian for the systems remainder using projection operator techniques. Performing a locator expansion on the strength of the many-body interaction term or on the hopping amplitude of the effective hamiltonian thus derived, we present results on the stability of the many body localised phases induced by proximity effect. We also briefly comment on the feasibility of the proposed model through modern quantum optics architectures, with the long-term perspective to realize experimentally, in composite open systems, Anderson or many-body localisation proximity effects.
Using molecular dynamics simulations we investigate the dependence of the structural and vibrational properties of the surfaces of sodo-silicate glasses on the sodium content as well as the nature of the surface. Two types of glass surfaces are considered: A melt-formed surface (MS) in which a liquid with a free surface has been cooled down into the glass phase and a fracture surface (FS) obtained by tensile loading of a glass sample. We find that the MS is more abundant in Na and non-bridging oxygen atoms than the FS and the bulk glass, whereas the FS has higher concentration of structural defects such as two-membered rings and under-coordinated Si than the MS. We associate these structural differences to the production histories of the glasses and the mobility of the Na ions. It is also found that for Na-poor systems the fluctuations in composition and local atomic charge density decay with a power-law as a function of distance from the surface while Na-rich systems show an exponential decay with a typical decay length of $approx2.3$~AA. The vibrational density of states shows that the presence of the surfaces leads to a decrease of the characteristic frequencies in the system. The two-membered rings give rise to a pronounce band at $approx880$~cm$^{-1}$ which is in good agreement experimental observations.
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