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Register a new userControlling a quantum gas of polar molecules in an optical lattice
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The production of molecules from dual species atomic quantum gases has enabled experiments that employ molecules at nanoKelvin temperatures. As a result, every degree of freedom of these molecules is in a well-defined quantum state and exquisitely controlled. These ultracold molecules open a new world of precision quantum chemistry in which quantum statistics, quantum partial waves, and even many-body correlations can play important roles. Moreover, to investigate the strongly correlated physics of many interacting molecular dipoles, we can mitigate lossy chemical reactions by controlling the dimensionality of the system using optical lattices formed by interfering laser fields. In a full three-dimensional optical lattice, chemistry can be turned on or off by tuning the lattice depth, which allows us to configure an array of long-range interacting quantum systems with rich internal structure. Such a system represents an excellent platform for gaining fundamental insights to complex materials based on quantum simulations and also for quantum information processing in the future.
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Ultracold polar molecules, with their long-range electric dipolar interactions, offer a unique platform for studying correlated quantum many-body phenomena such as quantum magnetism. However, realizing a highly degenerate quantum gas of molecules with a low entropy per particle has been an outstanding experimental challenge. In this paper, we report the synthesis of a low entropy molecular quantum gas by creating molecules at individual sites of a three-dimensional optical lattice that is initially loaded from a low entropy mixture of K and Rb quantum gases. We make use of the quantum statistics and interactions of the initial atom gases to load into the optical lattice, simultaneously and with good spatial overlap, a Mott insulator of bosonic Rb atoms and a single-band insulator of fermionic K atoms. Then, using magneto-association and optical state transfer, we efficiently produce ground-state molecules in the lattice at those sites that contained one Rb and one K atom. The achieved filling fraction of 25% indicates an entropy as low as $2.2,k_B$ per molecule. This low-entropy molecular quantum gas opens the door to novel studies of transport and entanglement propagation in a many-body system with long-range dipolar interactions.
Control over all internal and external degrees of freedom of molecules at the level of single quantum states will enable a series of fundamental studies in physics and chemistry. In particular, samples of ground-state molecules at ultralow temperatures and high number densities will allow novel quantum-gas studies and future applications in quantum information science. However, high phase-space densities for molecular samples are not readily attainable as efficient cooling techniques such as laser cooling are lacking. Here we produce an ultracold and dense sample of molecules in a single hyperfine level of the rovibronic ground state with each molecule individually trapped in the motional ground state of an optical lattice well. Starting from a zero-temperature atomic Mott-insulator state with optimized double-site occupancy, weakly-bound dimer molecules are efficiently associated on a Feshbach resonance and subsequently transferred to the rovibronic ground state by a stimulated four-photon process with >50 % efficiency. The molecules are trapped in the lattice and have a lifetime of 8 s. Our results present a crucial step towards Bose-Einstein condensation of ground-state molecules and, when suitably generalized to polar heteronuclear molecules, the realization of dipolar quantum-gas phases in optical lattices.
Ultracold polar molecules provide an excellent platform to study quantum many-body spin dynamics, which has become accessible in the recently realized low entropy quantum gas of polar molecules in an optical lattice. To obtain a detailed understanding for the molecular formation process in the lattice, we prepare a density distribution where lattice sites are either empty or occupied by a doublon composed of a bosonic atom interacting with a fermionic atom. By letting this disordered, out-of-equilibrium system evolve from a well-defined initial condition, we observe clear effects on pairing that arise from inter-species interactions, a higher partial wave Feshbach resonance, and excited Bloch-band population. When only the lighter fermions are allowed to tunnel in the three-dimensional (3D) lattice, the system dynamics can be well described by theory. However, in a regime where both fermions and bosons can tunnel, we encounter correlated dynamics that is beyond the current capability of numerical simulations. Furthermore, we show that we can probe the microscopic distribution of the atomic gases in the lattice by measuring the inelastic loss of doublons. These techniques realize tools that are generically applicable to heteronuclear diatomic systems in optical lattices and can shed light on molecule production as well as dynamics of a Bose-Fermi mixture.
In this work, we discuss the emergence of $p$-wave superfluids of identical fermions in 2D lattices. The optical lattice potential manifests itself in an interplay between an increase in the density of states on the Fermi surface and the modification of the fermion-fermion interaction (scattering) amplitude. The density of states is enhanced due to an increase of the effective mass of atoms. In deep lattices, for short-range interacting atoms, the scattering amplitude is strongly reduced compared to free space due to a small overlap of wavefunctions of fermions sitting in the neighboring lattice sites, which suppresses the $p$-wave superfluidity. However, we show that for a moderate lattice depth there is still a possibility to create atomic $p$-wave superfluids with sizable transition temperatures. The situation is drastically different for fermionic polar molecules. Being dressed with a microwave field, they acquire a dipole-dipole attractive tail in the interaction potential. Then, due to a long-range character of the dipole-dipole interaction, the effect of the suppression of the scattering amplitude in 2D lattices is absent. This leads to the emergence of a stable topological $p_x+ip_y$ superfluid of identical microwave-dressed polar molecules.
Spin-polarized samples and spin mixtures of quantum degenerate fermionic atoms are prepared in selected excited Bloch bands of an optical chequerboard square lattice. For the spin-polarized case, extreme band lifetimes above $10,$s are observed, reflecting the suppression of collisions by Paulis exclusion principle. For spin mixtures, lifetimes are reduced by an order of magnitude by two-body collisions between different spin components, but still remarkably large values of about one second are found. By analyzing momentum spectra, we can directly observe the orbital character of the optical lattice. The observations demonstrated here form the basis for exploring the physics of Fermi gases with two paired spin components in orbital optical lattices, including the regime of unitarity.
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