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Register a new userQuantum gas of rovibronic ground-state molecules in an optical lattice
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Authors
Johann G. Danzl
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Control over all internal and external degrees of freedom of molecules at the level of single quantum states will enable a series of fundamental studies in physics and chemistry. In particular, samples of ground-state molecules at ultralow temperatures and high number densities will allow novel quantum-gas studies and future applications in quantum information science. However, high phase-space densities for molecular samples are not readily attainable as efficient cooling techniques such as laser cooling are lacking. Here we produce an ultracold and dense sample of molecules in a single hyperfine level of the rovibronic ground state with each molecule individually trapped in the motional ground state of an optical lattice well. Starting from a zero-temperature atomic Mott-insulator state with optimized double-site occupancy, weakly-bound dimer molecules are efficiently associated on a Feshbach resonance and subsequently transferred to the rovibronic ground state by a stimulated four-photon process with >50 % efficiency. The molecules are trapped in the lattice and have a lifetime of 8 s. Our results present a crucial step towards Bose-Einstein condensation of ground-state molecules and, when suitably generalized to polar heteronuclear molecules, the realization of dipolar quantum-gas phases in optical lattices.
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The production of molecules from dual species atomic quantum gases has enabled experiments that employ molecules at nanoKelvin temperatures. As a result, every degree of freedom of these molecules is in a well-defined quantum state and exquisitely controlled. These ultracold molecules open a new world of precision quantum chemistry in which quantum statistics, quantum partial waves, and even many-body correlations can play important roles. Moreover, to investigate the strongly correlated physics of many interacting molecular dipoles, we can mitigate lossy chemical reactions by controlling the dimensionality of the system using optical lattices formed by interfering laser fields. In a full three-dimensional optical lattice, chemistry can be turned on or off by tuning the lattice depth, which allows us to configure an array of long-range interacting quantum systems with rich internal structure. Such a system represents an excellent platform for gaining fundamental insights to complex materials based on quantum simulations and also for quantum information processing in the future.
Ultracold polar molecules, with their long-range electric dipolar interactions, offer a unique platform for studying correlated quantum many-body phenomena such as quantum magnetism. However, realizing a highly degenerate quantum gas of molecules with a low entropy per particle has been an outstanding experimental challenge. In this paper, we report the synthesis of a low entropy molecular quantum gas by creating molecules at individual sites of a three-dimensional optical lattice that is initially loaded from a low entropy mixture of K and Rb quantum gases. We make use of the quantum statistics and interactions of the initial atom gases to load into the optical lattice, simultaneously and with good spatial overlap, a Mott insulator of bosonic Rb atoms and a single-band insulator of fermionic K atoms. Then, using magneto-association and optical state transfer, we efficiently produce ground-state molecules in the lattice at those sites that contained one Rb and one K atom. The achieved filling fraction of 25% indicates an entropy as low as $2.2,k_B$ per molecule. This low-entropy molecular quantum gas opens the door to novel studies of transport and entanglement propagation in a many-body system with long-range dipolar interactions.
Spin-polarized samples and spin mixtures of quantum degenerate fermionic atoms are prepared in selected excited Bloch bands of an optical chequerboard square lattice. For the spin-polarized case, extreme band lifetimes above $10,$s are observed, reflecting the suppression of collisions by Paulis exclusion principle. For spin mixtures, lifetimes are reduced by an order of magnitude by two-body collisions between different spin components, but still remarkably large values of about one second are found. By analyzing momentum spectra, we can directly observe the orbital character of the optical lattice. The observations demonstrated here form the basis for exploring the physics of Fermi gases with two paired spin components in orbital optical lattices, including the regime of unitarity.
Non-standard Bose-Hubbard models can exhibit rich ground state phase diagrams, even when considering the one-dimensional limit. Using a self-consistent Gutzwiller diagonalisation approach, we study the mean-field ground state properties of a long-range interacting atomic gas in a one-dimensional optical lattice. We first confirm that the inclusion of long-range two-body interactions to the standard Bose-Hubbard model introduces density wave and supersolid phases. However, the introduction of pair and density-dependent tunnelling can result in new phases with two-site periodic density, single-particle transport and two-body transport order parameters. These staggered phases are potentially a mean-field signature of the known novel twisted superfluids found via a DMRG approach [PRA textbf{94}, 011603(R) (2016)]. We also observe other unconventional phases, which are characterised by sign staggered order parameters between adjacent lattice sites.
We report on the efficient design of quantum optimal control protocols to manipulate the motional states of an atomic Bose-Einstein condensate (BEC) in a one-dimensional optical lattice. Our protocols operate on the momentum comb associated with the lattice. In contrast to previous works also dealing with control in discrete and large Hilbert spaces, our control schemes allow us to reach a wide variety of targets by varying a single parameter, the lattice position. With this technique, we experimentally demonstrate a precise, robust and versatile control: we optimize the transfer of the BEC to a single or multiple quantized momentum states with full control on the relative phase between the different momentum components. This also allows us to prepare the BEC in a given eigenstate of the lattice band structure, or superposition thereof.
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