No Arabic abstract
We study the mechanical stability of a tunable high-finesse microcavity under ambient conditions and investigate light-induced effects that can both suppress and excite mechanical fluctuations. As an enabling step, we demonstrate the ultra-precise electronic stabilization of a microcavity. We then show that photothermal mirror expansion can provide high-bandwidth feedback and improve cavity stability by almost two orders of magnitude. At high intracavity power, we observe self-oscillations of mechanical resonances of the cavity. We explain the observations by a dynamic photothermal instability, leading to parametric driving of mechanical motion. For an optimized combination of electronic and photothermal stabilization, we achieve a feedback bandwidth of $500,$kHz and a noise level of $1.1 times 10^{-13},$m rms.
Micron-scale optical cavities are produced using a combination of template sphere self-assembly and electrochemical growth. Transmission measurements of the tunable microcavities show sharp resonant modes with a Q-factor>300, and 25-fold local enhancement of light intensity. The presence of transverse optical modes confirms the lateral confinement of photons. Calculations show sub-micron mode volumes are feasible. The small mode volume of these microcavities promises to lead to a wide range of applications in microlasers, atom optics, quantum information, biophotonics and single molecule detection.
Proximity of the metal nanoparticles enhance the plasmonic coupling and shifts the resonance. This article presents a numerical study of the photothermal effect in aggregates of small gold nanorods considering the ordered as well as random aggregates. In the ordered aggregates, there is lateral coupling which causes blueshifts in the plasmonic resonance, while in the random aggregates there are redshifts in the plasmonic resonance. The plasmon response of latter could be tailored up to the second infrared biological therapeutic window. It has been observed that the aggregates show higher absorption power and therefore, higher temperature rise compared to the single gold nanorod or monodispersive nanorods. The absorption resonance peak position of the random aggregate depends on the incident and polarization angles of the incident light. The aggregation of the nanoparticles often inherently occurs in the biological medium which affects the photothermal process. This study helps to understand the photothermal heating of nanoparticle aggregates and the use of the optimal light source concerning the absorption peak of the aggregates suspension for therapeutic uses.
Third-order nonlinear optical effects in photonic microcavities are studied. Significant light defocusing in the thin nonlinear microcavity spacer was observed. The polarization self-action effect was detected, when the large nonlinear polarization rotation angle arises when exciting the microcavity mode, being proportional to the radiation intensity.
We report on measurements and modeling of the mode structure of tunable Fabry-Perot optical microcavities with imperfect mirrors. We find that non-spherical mirror shape and finite mirror size lead to loss, mode deformation, and shifted resonance frequencies at particular mirror separations. For small mirror diameters, the useful cavity length is limited to values significantly below the expected stability range. We explain the observations by resonant coupling between different transverse modes of the cavity and mode-dependent diffraction loss. A model based on resonant state expansion that takes into account the measured mirror profile can reproduce the measurements and identify the parameter regime where detrimental effects of mode mixing are avoided.
Scattering induced mode splitting in active microcavities is demonstrated. Below the lasing threshold, quality factor enhancement by optical gain allows resolving, in the wavelength-scanning transmission spectrum, the resonance dips of the split modes which otherwise would not be detected in a passive resonator. In the lasing regime, mode splitting manifests itself as two lasing modes with extremely narrow linewidths. Mixing of these laser modes in a detector leads to a heterodyne beat signal whose frequency corresponds to the amount of splitting. Lasing regime not only allows ultrahigh sensitivity for mode-splitting measurements but also provides an easily accessible scheme by eliminating the need for wavelength scanning around resonant modes. Mode splitting in active microcavities has immediate impact in enhancing the sensitivity of sub-wavelength scatterer detection and in studying light-matter interactions in strong coupling regime.