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Register a new userOptical amplitude and phase modulation dynamics at the single-photon level in a quantum dot ridge waveguide
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The amplitude and phase of a materials nonlinear optical response provide insight into the underlying electronic dynamics that determine its optical properties. Phase-sensitive nonlinear spectroscopy techniques are widely implemented to explore these dynamics through demodulation of the complex optical signal field into its quadrature components; however, complete reconstruction of the optical response requires measuring both the amplitude and phase of each quadrature, which is often lost in standard detection methods. Here, we implement a heterodyne-detection scheme to fully reconstruct the amplitude and phase response of spectral hole-burning from InAs/GaAs charged quantum dots. We observe an ultra-narrow absorption profile and a corresponding dispersive lineshape of the phase, which reflect the nanosecond optical coherence time of the charged exciton transition. Simultaneously, the measurements are sensitive to electron spin relaxation dynamics on a millisecond timescale, as this manifests as a magnetic-field dependent delay of the amplitude and phase modulation. Appreciable amplitude modulation depth and nonlinear phase shift up to 0.09$timespi$ radians (16$deg$) are demonstrated, providing new possibilities for quadrature modulation at faint photon levels with several independent control parameters, including photon number, modulation frequency, detuning, and externally applied fields.
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We exploit the nonlinearity arising from the spin-photon interaction in an InAs quantum dot to demonstrate phase shifts of scattered light pulses at the single-photon level. Photon phase shifts of close to 90 degrees are achieved using a charged quantum dot in a micropillar cavity. We also demonstrate a photon phase switch by using a spin-pumping mechanism through Raman transitions in an in-plane magnetic field. The experimental findings are supported by a theoretical model which explores the dynamics of the system. Our results demonstrate the potential of quantum dot-induced nonlinearities for quantum information processing.
Strong nonlinear interactions between photons enable logic operations for both classical and quantum-information technology. Unfortunately, nonlinear interactions are usually feeble and therefore all-optical logic gates tend to be inefficient. A quantum emitter deterministically coupled to a propagating mode fundamentally changes the situation, since each photon inevitably interacts with the emitter, and highly correlated many-photon states may be created . Here we show that a single quantum dot in a photonic-crystal waveguide can be utilized as a giant nonlinearity sensitive at the single-photon level. The nonlinear response is revealed from the intensity and quantum statistics of the scattered photons, and contains contributions from an entangled photon-photon bound state. The quantum nonlinearity will find immediate applications for deterministic Bell-state measurements and single-photon transistors and paves the way to scalable waveguide-based photonic quantum-computing architectures.
Sources of single photons are key elements in the study of basic quantum optical concepts and applications in quantum information science. Among the different sources available, semiconductor quantum dots excel with their straight forward integrability in semiconductor based on-chip solutions and the potential that photon emission can be triggered on demand. Usually, the photon emission event is part of a cascaded biexciton-exciton emission scheme. Important properties of the emitted photon such as polarization and time of emission are either probabilistic in nature or pre-determined by electronic properties of the system. In this work, we study the direct two-photon emission from the biexciton. We show that emission through this higher-order transition provides a much more versatile approach to generate a single photon. In the scheme we propose, the two-photon emission from the biexciton is enabled by a laser field (or laser pulse) driving the system into a virtual state inside the band gap. From this intermediate virtual state, the single photon of interest is then spontaneously emitted. Its properties are determined by the driving laser pulse, enabling all-optical on-the-fly control of polarization state, frequency, and time of emission of the photon.
We measure the detuning-dependent dynamics of a quasi-resonantly excited single quantum dot coupled to a micropillar cavity. The system is modeled with the dissipative Jaynes-Cummings model where all experimental parameters are determined by explicit measurements. We observe non-Markovian dynamics when the quantum dot is tuned into resonance with the cavity leading to a non-exponential decay in time. Excellent agreement between experiment and theory is observed with no free parameters providing the first quantitative description of an all-solid-state cavity QED system based on quantum dot emitters.
Planar nanostructures allow near-ideal extraction of emission from a quantum emitter embedded within, thereby realizing deterministic single-photon sources. Such a source can be transformed into M single-photon sources by implementing active temporal-to-spatial mode demultiplexing. We report on the realization of such a demultiplexed source based on a quantum dot embedded in a nanophotonic waveguide. Efficient outcoupling (>60%) from the waveguide into a single mode optical fiber is obtained with high-efficiency grating couplers. As a proof-of-concept, active demultiplexing into M=4 spatial channels is demonstrated by the use of electro-optic modulators with an end-to-end efficiency of >81% into single-mode fibers. Overall we demonstrate four-photon coincidence rates of >1 Hz even under non-resonant excitation of the quantum dot. The main limitation of the current source is the residual population of other exciton transitions that corresponds to a finite preparation efficiency of the desired transition. We quantitatively extract a preparation efficiency of 15% using the second-order correlation function measurements. The experiment highlights the applicability of planar nanostructures as efficient multiphoton sources through temporal-to-spatial demultiplexing and lays out a clear path way of how to scale up towards demonstrating quantum advantages with the quantum dot sources.
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