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Register a new userPairing Symmetry Studied from Impurity Effects in the Undoped Superconductor T-La$_{1.8}$Eu$_{0.2}$CuO$_4$
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We have investigated the effects of magnetic Ni and nonmagnetic Zn impurities on the superconductivity in undoped T-La$_{1.8}$Eu$_{0.2}$CuO$_4$ (T-LECO) with the Nd$_2$CuO$_4$-type structure, using the polycrystalline bulk samples, to clarify the pairing symmetry. It has been found that both suppression rates of the superconducting transition temperature $T_mathrm{c}$ by Ni and Zn impurities are nearly the same and are very similar to those in the optimally doped and overdoped regimes of hole-doped T-La$_{2-x}$Sr$_{x}$CuO$_4$ with the K$_2$NiF$_4$-type structure. These results strongly suggest that the superconductivity in undoped T-LECO is of the $d$-wave symmetry and is mediated by the spin fluctuation.
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We performed Cu {it K}-edge X-ray absorption fine structure measurements on T-type La$_{1.8}$Eu$_{0.2}$CuO$_4$ (LECO) and Nd$_2$CuO$_4$ (NCO) to investigate the variation in the electronic state associated with the emergence of superconductivity due to annealing. The X-ray absorption near-edge structure spectra of as-sintered (AS) LECO are quite similar to those of AS NCO, indicating that the ground state of AS T-type LECO is a Mott insulator. We found a significant variation of the electronic state at the Cu sites in LECO due to annealing. The electron density after annealing ($n_{rm AN}$) was evaluated for both superconducting LECO and non-superconducting NCO and found to be 0.40 and 0.05 electrons per Cu, respectively. In LECO but not in NCO, extended X-ray absorption fine structure analysis revealed a softening in the strength of the Cu-O bond in the CuO$_2$ plane due to annealing, which is consistent with the screening effect on phonons in the metallic state. Since the amounts of oxygen loss due to annealing ($delta$) for LECO and NCO are comparable with each other, these results suggest distinct electron-doping processes in the two compounds. That electron-doping in NCO approximately follows the relation $n_{rm AN}=2delta$ can be understood if electrons are doped through oxygen deficiency, but the anneal-induced metallic nature and large $n_{rm AN}$ of LECO suggest a variation of the electronic band structure causes self-doping of carriers. The origin of the difference in doping processes due to annealing is discussed in connection with the size of the charge transfer gap.
We performed neutron powder diffraction measurements on the as-sintered (AS) and oxygen-reduced (OR) La$_{1.8}$Eu$_{0.2}$CuO$_{4+alpha-delta}$ (LECO). The structural parameters for oxygens in AS and OR samples refined by the Rietveld analysis are almost identical to those of the reference system, Pr$_{2}$CuO$_{4+alpha-delta}$. Thus, the two systems are comparable in terms of the structural changes in oxygens due to the annealing, although superconductivity appears only in LECO.
We use resonant inelastic x-ray scattering to investigate charge-stripe correlations in La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. By differentiating elastic from inelastic scattering, it is demonstrated that charge-stripe correlations precede both the structural low-temperature tetragonal phase and the transport-defined pseudogap onset. The scattering peak amplitude from charge stripes decays approximately as $T^{-2}$ towards our detection limit. The in-plane integrated intensity, however, remains roughly temperature independent. Therefore, although the incommensurability shows a remarkably large increase at high temperature, our results are interpreted via a single scattering constituent. In fact, direct comparison to other stripe-ordered compounds (La$_{1.875}$Ba$_{0.125}$CuO$_4$, La$_{1.475}$Nd$_{0.4}$Sr$_{0.125}$CuO$_4$ and La$_{1.875}$Sr$_{0.125}$CuO$_4$) suggests a roughly constant integrated scattering intensity across all these compounds. Our results therefore provide a unifying picture for the charge-stripe ordering in La-based cuprates. As charge correlations in La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$ extend beyond the low-temperature tetragonal and pseudogap phase, their emergence heralds a spontaneous symmetry breaking in this compound.
We report an ultrahigh resolution resonant inelastic x-ray scattering (RIXS) study of the in-plane bond-stretching phonon mode in stripe-ordered cuprate La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. Phonon softening and lifetime shortening are found around the charge ordering wave vector. In addition to these self-energy effects, the electron-phonon coupling is probed by its proportionality to the RIXS cross section. We find an enhancement of the electron-phonon coupling around the charge-stripe ordering wave vector upon cooling into the low-temperature tetragonal structure phase. These results suggest that in addition to electronic correlations, electron-phonon coupling contributes significantly to the emergence of long-range charge-stripe order in cuprates.
The Meissner effect has been directly demonstrated by depth-resolved muon spin rotation measurements in high-quality thin films of the T-structured cuprate, T-La$_{1.9}$Y$_{0.1}$CuO$_4$, to confirm bulk superconductivity ($T_csimeq21$ K) in its {sl undoped} state. The gradual expelling of an external magnetic field is observed over a depth range of $sim$100 nm in films with a thickness of 275(15) nm, from which the penetration depth is deduced to be 466(22) nm. Based on this result, we argue that the true ground state of the parent compound of the $n$-type cuprates is not a Mott insulator but a strongly correlated metal with colossal sensitivity to apical oxygen impurities.
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