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Register a new userEnhancing diamond color center fluorescence via optimized plasmonic nanorod configuration
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A novel numerical methodology has been developed, which makes possible to optimize arbitrary emitting dipole and plasmonic nano-resonator configuration with an arbitrary objective function. By selecting quantum efficiency as the objective function that has to be maximized at preselected Purcell factor criteria, optimization of plasmonic nanorod based configurations has been realized to enhance fluorescence of NV and SiV color centers in diamond. Gold and silver nanorod based configurations have been optimized to enhance excitation and emission separately, as well as both processes simultaneously, and the underlying nanophotonical phenomena have been inspected comparatively. It has been shown that considerable excitation enhancement is achieved by silver nanorods, while nanorods made of both metals are appropriate to enhance emission. More significant improvement can be achieved via silver nanorods at both wavelengths of both color centers. It has been proven that theoretical limits originating from metal dielectric properties can be approached by simultaneous optimization, which results in configurations determined by preferences corresponding to the emission. Larger emission enhancement is achieved via both metals in case of SiV center compared to the NV center. Gold and silver nanorod based configurations making possible to improve SiV centers quantum efficiency by factors of 1.18 and 5.25 are proposed, which have potential applications in quantum information processing.
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Silicon-vacancy color centers in nanodiamonds are promising as fluorescent labels for biological applications, with a narrow, non-bleaching emission line at 738,nm. Two-photon excitation of this fluorescence offers the possibility of low-background detection at significant tissue depth with high three-dimensional spatial resolution. We have measured the two-photon fluorescence cross section of a negatively-charged silicon vacancy (SiV$^-$) in ion-implanted bulk diamond to be $0.74(19) times 10^{-50}{rm cm^4;s/photon}$ at an excitation wavelength of 1040,nm. In comparison to the diamond nitrogen vacancy (NV) center, the expected detection threshold of a two-photon excited SiV center is more than an order of magnitude lower, largely due to its much narrower linewidth. We also present measurements of two- and three-photon excitation spectra, finding an increase in the two-photon cross section with decreasing wavelength, and discuss the physical interpretation of the spectra in the context of existing models of the SiV energy-level structure.
Hyperbolic plasmonic metamaterials provide numerous opportunities for designing unusual linear and nonlinear optical properties. We show that the modal overlap of fundamental and second-harmonic light in an anisotropic plasmonic metamaterial slab results in the broadband enhancement of radiated second-harmonic intensity by up to 2 orders of magnitudes for TM- and TE-polarized fundamental light, compared to a smooth Au film under TM-polarised illumination. The results open up possibilities to design tuneable frequency-doubling metamaterial with the goal to overcome limitations associated with classical phase matching conditions in thick nonlinear crystals.
Scalable quantum photonic networks require coherent excitation of quantum emitters. However, many solid-state systems can undergo a transition to a dark shelving state that inhibits the fluorescence. Here we demonstrate that a controlled gating using a weak non-resonant laser, the resonant excitation can be recovered and amplified for single germanium vacancies (GeVs). Employing the gated resonance excitation, we achieve optically stable resonance fluorescence of GeV centers. Our results are pivotal for the deployment of diamond color centers as reliable building blocks for scalable solid state quantum networks.
Configuration of three different concave silver core-shell nanoresonators was numerically optimized to enhance the excitation and emission of embedded silicon vacancy (SiV) diamond color centers simultaneously. According to the tradeoff between the radiative rate enhancement and quantum efficiency (QE) conditional optimization was performed to ensure ~2-3-4 and 5-fold apparent cQE enhancement of SiV color centers with ~10% intrinsic QE. The enhancement spectra, as well as the near-field and charge distribution were inspected to uncover the physics underlying behind the optical responses. The conditionally optimized coupled systems were qualified by the product of the radiative rate enhancements at the excitation and emission, which is nominated as Px factor. The optimized spherical core-shell nanoresonator containing a centralized emitter is capable of enhancing considerably the emission via bonding dipolar resonance. The Px factor is 529-fold with 49.7% cQE at the emission. Decentralization of the emitter leads to appearance of higher order multipolar modes, which is not advantageous caused by their nonradiative nature. Transversal and longitudinal dipolar resonances of the optimized ellipsoidal core-shell resonator were tuned to the excitation and emission, respectively. The simultaneous enhancements result in 6.2x10^5 Px factor with 50.6% cQE at the emission. Rod-shaped concave core-shell nanoresonators exploit similarly transversal and longitudinal dipolar resonances, moreover they enhance the fluorescence more significantly due to their antenna-like geometry. Px factor of 8.34x10^5 enhancement is achievable while the cQE is 50.3% at the emission. The enhancement can result in 2.03x10^6-fold Px factor, when the criterion regarding the minimum QE is set to 20%.
We experimentally demonstrate a simple and robust optical fibers based method to achieve simultaneously efficient excitation and fluorescence collection from Nitrogen-Vacancy (NV) defects containing micro-crystalline diamond. We fabricate a suitable micro-concave (MC) mirror that focuses scattered excitation laser light into the diamond located at the focal point of the mirror. At the same instance, the mirror also couples the fluorescence light exiting out of the diamond crystal in the opposite direction of the optical fiber back into the optical fiber within its light acceptance cone. This part of fluorescence would have been otherwise lost from reaching the detector. Our proof-of-principle demonstration achieves a 25 times improvement in fluorescence collection compared to the case of not using any mirrors. The increase in light collection favors getting high signal-to-noise ratio (SNR) optically detected magnetic resonance (ODMR) signals hence offers a practical advantage in fiber-based NV quantum sensors. Additionally, we compacted the NV sensor system by replacing some bulky optical elements in the optical path with a 1x2 fiber optical coupler in our optical system. This reduces the complexity of the system and provides portability and robustness needed for applications like magnetic endoscopy and remote-magnetic sensing.
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