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Register a new userQuantum frequency conversion and strong coupling of photonic modes using four-wave mixing in integrated microresonators
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Single photon-level quantum frequency conversion has recently been demonstrated using silicon nitride microring resonators. The resonance enhancement offered by such systems enables high-efficiency translation of quantum states of light across wide frequency ranges at sub-watt pump powers. Using a quantum-mechanical Hamiltonian formalism, we present a detailed theoretical analysis of the conversion dynamics in these systems, and show that they are capable of converting single- and multi-photon quantum states. Analytic formulas for the conversion efficiency, spectral conversion probability density, and pump power requirements are derived which are in good agreement with previous theoretical and experimental results. We show that with only modest improvement to the state of the art, efficiencies exceeding 95% are achievable using less than 100 mW of pump power. At the critical driving strength that yields maximum conversion efficiency, the spectral conversion probability density is shown to exhibit a flat-topped peak, indicating a range of insensitivity to the spectrum of a single photon input. Two alternate theoretical approaches are presented to study the conversion dynamics: a dressed mode approach that yields a better intuitive picture of the conversion process, and a study of the temporal dynamics of the participating modes in the resonator, which uncovers a regime of Rabi-like coherent oscillations of single photons between two different frequency modes. This oscillatory regime arises from the strong coupling of distinct frequency modes mediated by coherent pumps.
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We investigate the effect of 2-beam coupling in different imaging geometries in generating intensity-difference squeezing from four-wave mixing (4WM) in Rb atomic vapors. A recently-introduced dual-seeding technique can cancel out the classical noise in a seeded four-wave mixing process. This dual-seeding technique, however, can introduce new complications that involve 2-beam coupling between different seeded spatial modes in the atomic vapor and can ruin squeezing at frequencies on the order of the atomic linewidth and below. This complicates some forms of quantum imaging using these systems. Here we show that seeding the 4WM process with skew rays can eliminate the excess noise caused by 2-beam coupling. To avoid 2-beam coupling in bright, seeded images, it is important to re-image the object in the gain medium, instead of focussing through it.
We review our recent work on tunable, ultrahigh quality factor whispering-gallery-mode bottle microresonators and highlight their applications in nonlinear optics and in quantum optics experiments. Our resonators combine ultra-high quality factors of up to Q = 3.6 times 10^8, a small mode volume, and near-lossless fiber coupling, with a simple and customizable mode structure enabling full tunability. We study, theoretically and experimentally, nonlinear all-optical switching via the Kerr effect when the resonator is operated in an add-drop configuration. This allows us to optically route a single-wavelength cw optical signal between two fiber ports with high efficiency. Finally, we report on progress towards strong coupling of single rubidium atoms to an ultra-high Q mode of an actively stabilized bottle microresonator.
Chalcogenide glass (ChG) is an attractive material for integrated nonlinear photonics due to its wide transparency and high nonlinearity, and its capability of being directly deposited and patterned on Silicon wafer substrates. It has a singular Raman effect among amorphous materials. Yet, the Raman lasing performance in high quality and chip integrated ChG microresonators remains unexplored. Here, we demonstrate an engineered Raman lasing dynamic based on home developed photonic integrated high-Q ChG microresonators. With a quality factor above 10^6, we achieve the record-low lasing threshold 3.25 mW among integrated planar photonic platforms. Both the single-mode Raman lasers and a broadband Raman-Kerr comb are observed and characterized, which is dependent on the dispersion of our flexible photonic platform and engineered via tuning the waveguide geometric size. The tunability of such a chipscale Raman laser is also demonstrated through tuning the pump wavelength and tuning the operating temperature on the chip. This allows for the access of single-mode lasing at arbitrary wavelengths in the range 1615-1755 nm. Our results may contribute to the understanding of rich Raman and Kerr nonlinear interactions in dissipative and nonlinear microresonators, and on application aspect, may pave a way to chip-scale efficient Raman lasers that is highly desired in spectroscopic applications in the infrared.
Efficient frequency conversion of photons has important applications in optical quantum technology because the frequency range suitable for photon manipulation and communication usually varies widely. Recently, an efficient frequency conversion system using a double-$Lambda$ four-wave mixing (FWM) process based on electromagnetically induced transparency (EIT) has attracted considerable attention because of its potential to achieve a nearly 100% conversion efficiency (CE). To obtain such a high CE, the spontaneous emission loss in this resonant-type FWM system must be suppressed considerably. A simple solution is to arrange the applied laser fields in a backward configuration. However, the phase mismatch due to this configuration can cause a significant decrease in CE. Here, we demonstrate that the phase mismatch can be effectively compensated by introducing the phase shift obtained by two-photon detuning. Under optimal conditions, we observe a wavelength conversion from 780 to 795 nm with a maximum CE of 91.2(6)% by using this backward FWM system at an optical depth of 130 in cold rubidium atoms. The current work represents an important step toward achieving low-loss, high-fidelity EIT-based quantum frequency conversion.
We show that a simple scheme based on nondegenerate four-wave mixing in a hot atomic vapor behaves like a near-perfect phase-insensitive optical amplifier, which can generate bright twin beams with a measured quantum noise reduction in the intensity difference of more than 8 dB, close to the best optical parametric amplifiers and oscillators. The absence of a cavity makes the system immune to external perturbations, and the strong quantum noise reduction is observed over a large frequency range.
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