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Register a new userEfficient, designable, and broad-bandwidth optical extinction via aspect-ratio-tailored silver nanodisks
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Subwavelength resonators, ranging from single atoms to metallic nanoparticles, typically exhibit a narrow-bandwidth response to optical excitations. We computationally design and experimentally synthesize tailored distributions of silver nanodisks to extinguish light over broad and varied frequency windows. We show that metallic nanodisks are two-to-ten-times more efficient in absorbing and scattering light than common structures, and can approach fundamental limits to broadband scattering for subwavelength particles. We measure broadband extinction per volume that closely approaches theoretical predictions over three representative visible-range wavelength windows, confirming the high efficiency of nanodisks and demonstrating the collective power of computational design and experimental precision for developing new photonics technologies.
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Area-selective atomic layer deposition is a key technology for modern microelectronics as it eliminates alignment errors inherent to conventional approaches by enabling material deposition only in specific areas. Typically, the selectivity originates from surface modifications of the substrate that allow or block precursor adsorption. The control of the deposition process currently remains a major challenge as the selectivity of the no-growth areas is lost quickly. Here, we show that surface modifications of the substrate strongly manipulate the surface diffusion. The selective deposition of TiO$_2$ on poly (methyl methacrylate) and SiO$_2$ yields localized nanostructures with tailored aspect ratios. Controlling the surface diffusion allows to tune such nanostructures as it boosts the growth rate at the interface of the growth and no-growth areas. Kinetic Monte-Carlo calculations reveal that species move from high to low diffusion areas. Further, we identify the catalytic activity of TiCl$_4$ during the formation of carboxylic acid on poly (methyl methacrylate) as the reaction mechanism responsible for the loss of selectivity, and show that process optimization leads to higher selectivity. Our work enables the precise control of area-selective atomic layer deposition on the nanoscale, and offers new strategies in area-selective deposition processes by exploiting surface diffusion effects.
We investigate the dynamics of high aspect ratio nanowires trapped axially in a single gradient force optical tweezers. A power spectrum analysis of the Brownian dynamics reveals a broad spectral resonance of the order of a kHz with peak properties that are strongly dependent on the input trapping power. Modelling of the dynamical equations of motion of the trapped nanowire that incorporate non-conservative effects through asymmetric coupling between translational and rotational degrees of freedom provides excellent agreement with the experimental observations. An associated observation of persistent cyclical motion around the equilibrium trapping position using winding analysis provides further evidence for the influence of non-conservative forces.
Taking advantages of ultra-narrow bandwidth and high noise rejection performance of the Faraday anomalous dispersion optical filter (FADOF), simultaneously with the coherent amplification of atomic stimulated emission, a stimulated amplified Faraday anomalous dispersion optical filter (SAFADOF) at cesium 1470 nm is realized. The SAFADOF is able to significantly amplify very weak laser signals and reject noise in order to obtain clean signals in strong background. Experiment results show that, for a weak signal of 50 pW, the gain factor can be larger than 25000 (44 dB) within a bandwidth as narrow as 13 MHz. Having this ability to amplify weak signals with low background contribution, the SAFADOF finds outstanding potential applications in weak signal detections.
We present shape-independent upper limits to the power--bandwidth product for a single resonance in an optical scatterer, with the bound depending only on the material susceptibility. We show that quasistatic metallic scatterers can nearly reach the limits, and we apply our approach to the problem of designing $N$ independent, subwavelength scatterers to achieve flat, broadband response even if they individually exhibit narrow resonant peaks.
Putting the DRAM on the same package with a processor enables several times higher memory bandwidth than conventional off-package DRAM. Yet, the latency of in-package DRAM is not appreciably lower than that of off-package DRAM. A promising use of in-package DRAM is as a large cache. Unfortunately, most previous DRAM cache designs mainly optimize for hit latency and do not consider off-chip bandwidth efficiency as a first-class design constraint. Hence, as we show in this paper, these designs are suboptimal for use with in-package DRAM. We propose a new DRAM cache design, Banshee, that optimizes for both in- and off-package DRAM bandwidth efficiency without degrading access latency. The key ideas are to eliminate the in-package DRAM bandwidth overheads due to costly tag accesses through virtual memory mechanism and to incorporate a bandwidth-aware frequency-based replacement policy that is biased to reduce unnecessary traffic to off-package DRAM. Our extensive evaluation shows that Banshee provides significant performance improvement and traffic reduction over state-of-the-art latency-optimized DRAM cache designs.
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