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Magneto-electric spectroscopy of Andreev bound states in Josephson quantum dots

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 Added by Nils Wentzell
 Publication date 2016
  fields Physics
and research's language is English




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We theoretically investigate the behavior of Andreev levels in a single-orbital interacting quantum dot in contact to superconducting leads, focusing on the effect of electrostatic gating and applied magnetic field, as relevant for recent experimental spectroscopic studies. In order to account reliably for spin-polarization effects in presence of correlations, we extend here two simple and complementary approaches that are tailored to capture effective Andreev levels: the static functional renormalization group (fRG) and the self-consistent Andreev bound states (SCABS) theory. We provide benchmarks against the exact large-gap solution as well as NRG calculations and find good quantitative agreement in the range of validity. The large flexibility of the implemented approaches then allows us to analyze a sizeable parameter space, allowing to get a deeper physical understanding into the Zeeman field, electrostatic gate, and flux dependence of Andreev levels in interacting nanostructures.



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We demonstrate several new electron transport phenomena mediated by Andreev bound states (ABSs) that form on three-terminal carbon nanotube (CNT) QDs, with one superconducting (S) contact in the center and two adjacent normal metal (N) contacts. Three-terminal spectroscopy allows us to identify the coupling to the N contacts as the origin of the Andreev resonance (AR) linewidths and to determine the critical coupling strengths to S, for which a ground state transition S-QD systems can occur. We ascribe replicas of the lowest-energy ABS resonance to transitions between the ABS and odd-parity excited QD states, a process called excited state ABS resonances. In the conductance between the two N contacts we find a characteristic pattern of positive and negative differential subgap conductance, which we explain by considering two nonlocal processes, the creation of Cooper pairs in S by electrons from both N terminals, and a novel mechanism called resonant ABS tunneling. In the latter, electrons are transferred via the ABS without creating Cooper pairs in S. The three-terminal geometry also allows spectroscopy experiments with different boundary conditions, for example by leaving S floating. Surprisingly, we find that, depending on the boundary conditions, the experiments either show single-particle Coulomb blockade resonances, ABS characteristics, or both in the same measurements, seemingly contradicting the notion of ABSs replacing the single particle states as eigenstates of the QD. We qualitatively explain these results as originating from the finite time scale required for the coherent oscillations between the superposition states after a single electron tunneling event. These experiments demonstrate that three-terminal experiments on a single complex quantum object can also be useful to investigate charge dynamics otherwise not accessible due to the very high frequencies.
The superconducting proximity effect in semiconductor nanowires has recently enabled the study of new superconducting architectures, such as gate-tunable superconducting qubits and multiterminal Josephson junctions. As opposed to their metallic counterparts, the electron density in semiconductor nanosystems is tunable by external electrostatic gates providing a highly scalable and in-situ variation of the device properties. In addition, semiconductors with large $g$-factor and spin-orbit coupling have been shown to give rise to exotic phenomena in superconductivity, such as $varphi_0$ Josephson junctions and the emergence of Majorana bound states. Here, we report microwave spectroscopy measurements that directly reveal the presence of Andreev bound states (ABS) in ballistic semiconductor channels. We show that the measured ABS spectra are the result of transport channels with gate-tunable, high transmission probabilities up to $0.9$, which is required for gate-tunable Andreev qubits and beneficial for braiding schemes of Majorana states. For the first time, we detect excitations of a spin-split pair of ABS and observe symmetry-broken ABS, a direct consequence of the spin-orbit coupling in the semiconductor.
We present a microscopic theory for the current through a tunnel Josephson junction coupled to a non-linear environment, which consists of an Andreev two-level system coupled to a harmonic oscillator. It models a recent experiment [Bretheau, Girit, Pothier, Esteve, and Urbina, Nature (London) 499, 312 (2013)] on photon spectroscopy of Andreev bound states in a superconducting atomic-size contact. We find the eigenenergies and eigenstates of the environment and derive the current through the junction due to inelastic Cooper pair tunneling. The current-voltage characteristic reveals the transitions between the Andreev bound states, the excitation of the harmonic mode that hybridizes with the Andreev bound states, as well as multi-photon processes. The calculated spectra are in fair agreement with the experimental data.
We study an analytical model of a Rashba nanowire that is partially covered by and coupled to a thin superconducting layer, where the uncovered region of the nanowire forms a quantum dot. We find that, even if there is no topological superconducting phase possible, there is a trivial Andreev bound state that becomes pinned exponentially close to zero energy as a function of magnetic field strength when the length of the quantum dot is tuned with respect to its spin-orbit length such that a resonance condition of Fabry-Perot type is satisfied. In this case, we find that the Andreev bound state remains pinned near zero energy for Zeeman energies that exceed the characteristic spacing between Andreev bound state levels but that are smaller than the spin-orbit energy of the quantum dot. Importantly, as the pinning of the Andreev bound state depends only on properties of the quantum dot, we conclude that this behavior is unrelated to topological superconductivity. To support our analytical model, we also perform a numerical simulation of a hybrid system while explicitly incorporating a thin superconducting layer, showing that all qualitative features of our analytical model are also present in the numerical results.
The spectrum of a segment of InAs nanowire, confined between two superconducting leads, was measured as function of gate voltage and superconducting phase difference using a third normal-metal tunnel probe. Sub-gap resonances for odd electron occupancy---interpreted as bound states involving a confined electron and a quasiparticle from the superconducting leads, reminiscent of Yu-Shiba-Rusinov states---evolve into Kondo-related resonances at higher magnetic fields. An additional zero bias peak of unknown origin is observed to coexist with the quasiparticle bound states.
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