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Register a new userSeries of broad resonances in atomic three-body systems
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We re-examine the series of resonances found earlier in atomic three-body systems by solving the Faddeev-Merkuriev integral equations. These resonances are rather broad and line-up at each threshold with gradually increasing gaps, the same way for all thresholds and irrespective of the spatial symmetry. We relate these resonances to the Gailitis mechanism, which is a consequence of the polarization potential.
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It is demonstrated that in photoabsorption by endohedral atoms some atomic Giant resonances are almost completely destroyed while the others are totally preserved due to different action on it of the fullerenes shell. As the first example we discuss the 4d10 Giant resonance in Xe@C60 whereas as the second serves the Giant autoionization resonance in Eu@C60. The qualitative difference comes from the fact that photoelectrons from the 4d Giant resonance has small energies (tens of eV) and are strongly reflected by the C60 fullerenes shell. As to the Eu@C60, Giant autoionization leads to fast photoelectrons (about hundred eV) that go out almost untouched by the C60 shell. As a result of the outgoing electrons energy difference the atomic Giant resonances will be largely destroyed in A@C60 while the Giant autoionization resonance will be almost completely preserved. Thus, on the way from Xe@C60 Giant resonance to Eu@C60 Giant autoionization resonance the oscillation structure should disappear. Similar will be the decrease of oscillations on the way from pure Giant to pure Giant autoionization resonances for the angular anisotropy parameters. At Giant resonance frequencies the role of polarization of the fullerenes shell by the incoming photon beam is inessential. Quite different is the situation for the outer electrons in Eu@C60, the photoionization of which will be also considered.
Laser-driven rescattering of electrons is the basis of many strong-field phenomena in atoms and molecules. Here, we will show how this mechanism operates in extended atomic systems, giving rise to effective energy absorption. Rescattering from extended systems can also lead to energy loss, which in its extreme form results in non-linear photo-association. Intense-laser interaction with atomic clusters is discussed as an example. We explain fast electron emission, seen in experimental and numerically obtained spectra, by rescattering of electrons at the highly charged cluster.
Three-body resonances in atomic systems are calculated as complex-energy solutions of Faddeev-type integral equations. The homogeneous Faddeev-Merkuriev integral equations are solved by approximating the potential terms in a Coulomb-Sturmian basis. The Coulomb-Sturmian matrix elements of the three-body Coulomb Greens operator has been calculated as a contour integral of two-body Coulomb Greens matrices. This approximation casts the integral equation into a matrix equation and the complex energies are located as the complex zeros of the Fredholm determinant. We calculated resonances of the e-Ps system at higher energies and for total angular momentum L=1 with natural and unnatural parity
In molecular collisions, resonances occur at specific energies where the colliding particles temporarily form quasi-bound complexes, resulting in rapid variations in the energy dependence of scattering cross sections. Experimentally, it has proven challenging to observe such scattering resonances, especially in differential cross sections. We report the observation of resonance fingerprints in the state-to-state differential cross sections for inelastic NO-He collisions in the 13 to 19 cm$^{-1}$ energy range with 0.3 cm$^{-1}$ resolution. The observed structures were in excellent agreement with quantum scattering calculations. They were analyzed by separating the resonance contributions to the differential cross sections from the background through a partitioning of the multichannel scattering matrix. This revealed the partial wave composition of the resonances, and their evolution during the collision.
We reconsider the homogeneous Faddeev-Merkuriev integral equations for three-body Coulombic systems with attractive Coulomb interactions and point out that the resonant solutions are contaminated with spurious resonances. The spurious solutions are related to the splitting of the attractive Coulomb potential into short- and long-range parts, which is inherent in the approach, but arbitrary to some extent. By varying the parameters of the splitting the spurious solutions can easily be ruled out. We solve the integral equations by using the Coulomb-Sturmian separable expansion approach. This solution method provides an exact description of the threshold phenomena. We have found several new S-wave resonances in the e- e+ e- system in the vicinity of thresholds.
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